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Physical Review A

Effects of finite bandwidth on the resonance fluorescence spectrum inside of a cavity

A. H. Toor, Muhammad Suhail Zubairy

Published Jan 1, 1994• 12 citations
Publisher

Abstract

We have considered the steady-state resonance fluorescence spectrum for a beam of two-level atoms, interacting with a strong driving field with a finite bandwidth inside a cavity. The competitive effects of cavity losses and the finite bandwidth of the intense driving laser beam on the resonance fluorescence spectrum have been discussed. Our results show that the usual three-peaked resonance fluorescence spectrum starts merging back into the central peak as the bandwidth of the driving field increases. Moreover, the asymmetry introduced by the detuning of the driving field having a finite bandwidth is also affected by the cavity losses.

DOI
10.1103/physreva.49.449

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Journal of the Optical Society of America B•Jul 1, 1995•14 citations
We have considered the steady-state resonance fluorescence spectrum for a beam of two-level atoms, interacting with a strong driving field with a finite bandwidth inside a cavity. The competitive effects of cavity losses and the finite bandwidth of the intense driving laser beam on the resonance fluorescence spectrum have been discussed. Our results show that the usual three-peaked resonance fluorescence spectrum starts merging back into the central peak as the bandwidth of the driving field increases. Moreover, the asymmetry introduced by the detuning of the driving field having a finite bandwidth is also affected by the cavity losses.
The resonance fluorescence of a two-level atom driven by a coherent laser field and damped by a finite bandwidth squeezed vacuum is analysed. We extend the Yeoman and Barnett technique to a non-zero detuning of the driving field from the atomic resonance and discuss the role of squeezing bandwidth and the detuning in the level shifts, widths and intensities of the spectral lines. The approach is valid for arbitrary values of the Rabi frequency and detuning but for the squeezing bandwidths larger than the natural line-width in order to satisfy the Markoff approximation. The narrowing of the spectral lines is interpreted in terms of the quadrature-noise spectrum. We find that, depending on the Rabi frequency, detuning and the squeezing phase, different factors contribute to the line narrowing. For a strong resonant driving field there is no squeezing in the emitted field and the fluorescence spectrum exactly reveals the noise spectrum. In this case the narrowing of the spectral lines arises from the noise reduction in the input squeezed vacuum. For a weak or detuned driving field the fluorescence exhibits a large squeezing and, as a consequence, the spectral lines have narrowed linewidths. Moreover, the fluorescence spectrum can be asymmetric about the central frequency despite the symmetrical distribution of the noise. The asymmetry arises from the absorption of photons by the squeezed vacuum which reduces the spontaneous emission. For an appropriate choice of the detuning some of the spectral lines can vanish despite that there is no population trapping. Again this process can be interpreted as arising from the absorption of photons by the squeezed vacuum. When the absorption is large it may compensate the spontaneous emission resulting in the vanishing of the fluorescence lines.
We present an analytical technique for investigating the behaviour of a coherently driven atom damped by a squeezed vacuum with finite squeezing bandwidth. A master equation and analytic expressions for the fluorescent spectrum are derived for the simple case of a two-level atom exactly resonant with the frequencies of both the squeezed field and the driving field. Suitable choices of driving strength, phase and squeezing source lead to either sub-natural lincwidths of the Rabi sidebands or a sub-natural linewidth of the central spectral peak or indeed sub-natural linewidths of all three spectral peaks when squeezing bandwidths are taken into account. We also establish the remarkable result that in the strong driving regime, the width of the central peak of the fluorescent spectrum depends solely on the squeezing found at the Rabi sideband frequencies.
We present analytical results for the steady-state resonance fluorescence spectrum produced by a driven two-level atom excited under two strong coherent fields in the presence of a broadband squeezed vacuum. Here the central frequency of the squeezed vacuum is considered to be resonant as well as off-resonant with the average driving field frequency while maintaining resonance between the atomic transition frequency and the average driving field frequency. We observe a ringing phenomenon in the fluorescence spectrum due to the small frequency difference in the bichromatic field and this phenomenon is found to be sensitive to the detuning of the carrier frequency of squeezed vacuum with respect to the central frequency of the bichromatic field.
The problem of resonance fluorescence from a two-level atom that is driven near resonance by a laser beam of finite bandwidth is tackled via the Heisenberg equations of motion, by a simple generalization of our previous treatment. It is found that the two-time intensity correlation function is again factorizable into a product of the mean light intensities at the two times, each of which is slightly modified under broad-band excitation from its value under monochromatic excitation. The spectrum of the fluorescence is affected rather more drastically, and, in general, becomes asymmetric under broad-band excitation.
The effects of different laser line shapes on the intensity and spectrum of resonance fluorescence from a two-level atom are investigated. The laser model considered is that of an ideal single-mode laser operating high above threshold, with constant amplitude and undergoing phase-frequency fluctuations analogous to Brownian motion. As the correlation time of the frequency fluctuations increases from zero to infinity, the laser line shape changes from Lorentzian to Gaussian in a continuous way. It is shown that for intermediate and strong fields, the average intensity of fluorescence in the case of a resonant broadband Lorentzian line shape is higher than that in the case of a Gaussian line shape with the same bandwidth and total power. This is in contrast to the weak-field case where the higher peak power of the Gaussian line shape makes it more effective than the Lorentzian line shape. It is also shown that in the case of a nonzero frequency correlation time (non-Lorentzian line shape) the intensity of fluorescence undergoes non-Markovian fluctuations. In relation to the spectrum of resonance fluorescence, it is shown that as the line shape is varied from Lorentzian to Gaussian the following changes take place: In the case of off-resonance excitation, the asymmetry of the spectrum decreases. In the case of resonant excitation, the center-peak to side-peak height ratio for the triplet structure increases. Moreover, the recently predicted center-line dip, which develops in the spectrum in the case of broadband excitation when the Rabi frequency and the bandwidth are nearly equal, becomes increasingly deeper.
The resonance fluorescence system of a coherently driven two-level atom in the presence of a broadband squeezed vacuum field whose central frequency is not in resonance with either the driving field frequency or the atomic transition frequency is analyzed. Solutions of the Bloch equations of the system are presented in terms of continued fractions for arbitrary strength of the coherent driving field. Numerical results are presented for the first-harmonic quadrature components of the absorption spectrum and the fluorescent intensity. The effects of the squeezed vacuum field detuning on the absorption spectrum result in hole burning or a dip structure in the weak-field case and two absorption–amplification peaks in the strong-field case. Results are sensitive to the relative phase of the squeezed vacuum.