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Journal of Modern Optics

Influence of squeezing bandwidths on resonance fluorescence

Gordon Yeoman, Stephen Mark Barnett

Published Oct 1, 1996• 27 citations
Publisher

Abstract

We present an analytical technique for investigating the behaviour of a coherently driven atom damped by a squeezed vacuum with finite squeezing bandwidth. A master equation and analytic expressions for the fluorescent spectrum are derived for the simple case of a two-level atom exactly resonant with the frequencies of both the squeezed field and the driving field. Suitable choices of driving strength, phase and squeezing source lead to either sub-natural lincwidths of the Rabi sidebands or a sub-natural linewidth of the central spectral peak or indeed sub-natural linewidths of all three spectral peaks when squeezing bandwidths are taken into account. We also establish the remarkable result that in the strong driving regime, the width of the central peak of the fluorescent spectrum depends solely on the squeezing found at the Rabi sideband frequencies.

DOI
10.1080/09500349608232870

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Physical Review A•Oct 1, 1990•56 citations
We present an analytical technique for investigating the behaviour of a coherently driven atom damped by a squeezed vacuum with finite squeezing bandwidth. A master equation and analytic expressions for the fluorescent spectrum are derived for the simple case of a two-level atom exactly resonant with the frequencies of both the squeezed field and the driving field. Suitable choices of driving strength, phase and squeezing source lead to either sub-natural lincwidths of the Rabi sidebands or a sub-natural linewidth of the central spectral peak or indeed sub-natural linewidths of all three spectral peaks when squeezing bandwidths are taken into account. We also establish the remarkable result that in the strong driving regime, the width of the central peak of the fluorescent spectrum depends solely on the squeezing found at the Rabi sideband frequencies.
We examine subnatural phase-dependent linewidths in the fluorescence spectrum of a three-level atom damped by a narrow-bandwidth squeezed vacuum in a cavity. Using the dressed-atom model approach of a strongly driven three-level cascade system, we derive the master equation of the system from which we obtain simple analytical expressions for the fluorescence spectrum. We show that the phase effects depend on the bandwidths of the squeezed vacuum and the cavity relative to the Rabi frequency of the driving fields. When the squeezing bandwidth is much larger than the Rabi frequency, the spectrum consists of five lines with only the central and outer sidebands dependent on the phase. For a squeezing bandwidth much smaller than the Rabi frequency the number of lines in the spectrum and their phase properties depend on the frequency at which the squeezing and cavity modes are centered. When the squeezing and cavity modes are centered on the inner Rabi sidebands, the spectrum exhibits five lines that are completely independent of the squeezing phase with only the inner Rabi sidebands dependent on the squeezing correlations. Matching the squeezing and cavity modes to the outer Rabi sidebands leads to the disappearance of the inner Rabi sidebands and a strong phase dependence of the central line and the outer Rabi sidebands. We find that in this case the system behaves as an individual two-level system that reveals exactly the noise distribution in the input squeezed vacuum.
The resonance fluorescence of a two-level atom driven by a coherent laser field and damped by a finite bandwidth squeezed vacuum is analysed. We extend the Yeoman and Barnett technique to a non-zero detuning of the driving field from the atomic resonance and discuss the role of squeezing bandwidth and the detuning in the level shifts, widths and intensities of the spectral lines. The approach is valid for arbitrary values of the Rabi frequency and detuning but for the squeezing bandwidths larger than the natural line-width in order to satisfy the Markoff approximation. The narrowing of the spectral lines is interpreted in terms of the quadrature-noise spectrum. We find that, depending on the Rabi frequency, detuning and the squeezing phase, different factors contribute to the line narrowing. For a strong resonant driving field there is no squeezing in the emitted field and the fluorescence spectrum exactly reveals the noise spectrum. In this case the narrowing of the spectral lines arises from the noise reduction in the input squeezed vacuum. For a weak or detuned driving field the fluorescence exhibits a large squeezing and, as a consequence, the spectral lines have narrowed linewidths. Moreover, the fluorescence spectrum can be asymmetric about the central frequency despite the symmetrical distribution of the noise. The asymmetry arises from the absorption of photons by the squeezed vacuum which reduces the spontaneous emission. For an appropriate choice of the detuning some of the spectral lines can vanish despite that there is no population trapping. Again this process can be interpreted as arising from the absorption of photons by the squeezed vacuum. When the absorption is large it may compensate the spontaneous emission resulting in the vanishing of the fluorescence lines.
The dynamics of a strongly driven two-level atom are examined for the case that the atom is coupled to a ``two-mode'' squeezed vacuum. The source of squeezed light is taken to be a (frequency) nondegenerate parametric oscillator. We consider the situation in which the Rabi sidebands produced by the coherent driving field coincide with the spectral peaks of the parametric oscillator. Approximate analytical results are presented and checked against numerical simulations of the exact equations. For a suitable choice of relative phase, all three spectral lines in the fluorescence triplet are found to exhibit subnatural linewidths. Significant modifications to the fluorescence spectrum are also possible with a nonzero laser-atom detuning.
The fluorescence spectrum of a strongly driven two-level atom located inside an optical cavity damped by a narrow-bandwidth squeezed vacuum is studied. We use a dressed atom model approach, first applied to squeezed vacuum problems by Yeoman and Barnett, to derive the master equation of the system and discuss the role of the cavity and the squeezed vacuum in the narrowing of the spectral lines and the population trapping effect. We find that in the presence of a single-mode cavity the effect of squeezing on the fluorescence spectrum is more evident in the linewidths of the Rabi sidebands rather than in the linewidth of the central component. Even in the absence of squeezing, the cavity can reduce the linewidth of the central component almost to zero, whereas the Rabi sidebands can be narrowed only to some finite value. In the presence of a two-mode cavity and a two-mode squeezed vacuum the signature of squeezing is evident in the linewidths of all spectral lines. We also establish that the narrowing of the spectral lines is very sensitive to the detuning of the driving field from the atomic resonance. Moreover, we find that the population trapping effect, predicted for the broadband squeezed vacuum case, may appear in a narrow-bandwidth case only if the input squeezed modes are perfectly matched to the cavity modes and if there is non-zero squeezing at the Rabi sidebands.
Fluorescence from a coherently driven two-level atom that is damped by a squeezed vacuum is studied. We show that the mean atomic polarization depends on the relative phases of the squeezed vacuum and the coherent driving field. The fluorescent spectrum is calculated and shows several modifications over the spectrum for normal resonance fluorescence. In particular, the central peak of the Mollow triplet has a linewidth that depends on the phase of the driving field. For strong squeezing this peak can either be much narrower or much broader than the natural linewidth of the atom.
We examine resonance fluorescence of a two-level atom in a squeezed vacuum, under the condition that the squeezing bandwidth is much narrower than the Rabi splitting of the Mollow triplet. For a suitable choice of the relative phase between the squeezed vacuum and coherent driving field, we find significant narrowing of the Rabi peaks and inhibited population decay. These results are in marked contrast to previous broadband squeezing analyses, which predict strong broadening of the Rabi peaks and enhanced population decay. We explore the connection between our work and that on the dynamical suppression of spontaneous emission via strongly driven resonance fluorescence in a cavity [Lewenstein, Mossberg, and Glauber, Phys. Rev. Lett. 59, 775 (1987)]. By modifying this work to incorporate squeezing of the cavity modes, we are able to combine the features of both systems, and thereby predict strong inhibition of the decay of all three components of the Bloch vector in a possible experimental configuration.