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Optics and Spectroscopy

Dynamics of interaction between two-level atoms in a laser field and linear stationary optical dimensional resonances

O. N. Gadomskiĭ, Yu. V. Abramov

Published Jul 1, 2003• 0 citations
Publisher

Abstract

Formulas for radiative forces acting on the atoms of a diatomic object in a field of external laser radiation are obtained with allowance made for the interatomic dipole-dipole interaction. It is shown that one can control the motion of the atoms by gradually varying the frequency of external laser radiation due to the presence of optical dimensional resonances in the spectrum of the diatomic object.

DOI
10.1134/1.1595205

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Formulas for radiative forces acting on the atoms of a diatomic object in a field of external laser radiation are obtained with allowance made for the interatomic dipole-dipole interaction. It is shown that one can control the motion of the atoms by gradually varying the frequency of external laser radiation due to the presence of optical dimensional resonances in the spectrum of the diatomic object.
The forces acting on interacting moving atoms exposed to resonant laser radiation are calculated. It is shown that the forces acting on the atoms include the radiation pressure forces as well as the external and internal bias forces. The dependences of the forces on the atomic spacing, polarization, and laser radiation frequency are given. It is found that the internal bias force associated with the interaction of atomic dipoles via the reemitted field may play an important role in the dynamics of dense atomic ensembles in a light field. It is shown that optical size resonances appear in the system of interacting atoms at frequencies differing substantially from transition frequencies in the spectrum of atoms. It is noted that optical size resonances as well as the Doppler frequency shift in the spectrum of interacting atoms play a significant role in the processes of laser-radiation-controlled motion of the atoms.
The existence of linear nonstationary optical resonances in a diatomic nanostructural object with a dipole-dipole atomic interaction has been proved. A new solution to the joint system of modified Bloch optical equations and nonlocal field equations is obtained for time intervals much shorter than the times of phase and energy relaxation. Formulas for effective polarizabilities of the object’s atoms, which have a set of dimensional resonances, are derived. The frequencies of these resonances significantly differ from the eigenfrequencies of the object’s atoms, and their properties depend on the interatomic distance, light-pulse duration, initial atomic inversions, and the orientation of the object’s axis relative to the direction of incidence of the external light wave.
The optical response of a diatomic system excited by monochromatic light is studied. On the basis of a semiclassical approach, the effects of rearrangement of the energy spectrum of the system due to the dipole-dipole interaction and the effects related to variations in the orientation of the atomic dipole moments under the action of microscopic fields are jointly taken into account. The strongest response of the system is shown to occur at dimensional resonance frequencies. The number of observed intensity peaks depends on the position of the observation point with respect to the interatomic axis. The frequencies of the dimensional resonances are compared with other characteristic frequencies of the atomic spectrum.
In quantum optical problems involving the interaction of atoms with laser fields, the atoms are usually considered being stationary during the interaction. Since every photon has a momentum, the atomic momentum (motion) can be changed in the process of absorption and emission of photons. This may force a stationary atom to move or to change momentum of an already moving atom. Therefore, the dynamical behaviour of atoms can be varied by the interaction with a radiation field. For a weak driving field, the influence of this field on the atomic motion can be neglected. However, the intensities of laser fields are generally very strong, and then the motion of the atoms can be considerably changed by the laser field. Here, we discuss this aspect, especially the effect of a driving field on the motion of atoms and the atomic momentum distribution. In particular, we will consider diffraction of atoms by a standing-wave laser field due to an exchange of momentum with the photons of the wave, and radiation force on atoms driven by a running-or standing-wave laser field.
The usual form of electromagnetic forces is given by but for neutral atoms q = 0. The next order of force is the dipole term, but this also vanishes because neutral atoms have no inherent dipole moment. However, a dipole moment can be induced by a field, and this is most efficient if the field is alternating near the atomic resonance frequency. Since these frequencies are typically in the optical range, dipole moments are efficiently induced by shining nearly resonant light on the atoms. Laser cooling and trapping rely on the interaction between laser light and atoms to exert a controllable force on the atoms, and many sophisticated schemes have been developed using the special properties of the interaction. This chapter begins with the simplest schemes for exerting optical forces on atoms, namely a single-frequency light field interacting with a two-level atom. Although this is the simplest possible scheme, it is pedagogically valuable because it shows many of the features that will be encountered further on. The ultimate temperature using such a scheme is limited, but lower temperatures can be achieved with multilevel atoms. This topic is addressed later in the chapter. Two kinds of optical forces When an atom absorbs nearly resonant light, it makes a transition to the excited state, and its subsequent return to the ground state can be either by spontaneous or by stimulated emission. The nature of the optical force that arises from these two different processes is quite different, and will be described separately [1]. The spontaneous emission case is different from the familiar quantum mechanical calculations using state vectors to describe the state of the system, because spontaneous emission causes the state of the system to evolve from a pure state into a mixed state (see Exercise 6.9). Spontaneous emission is an essential ingredient for the dissipative nature of the optical forces in monochromatic light, and the density matrix is needed to describe it (see Chap. 6). When an atom absorbs light, its energy excites the atom and its angular momentum changes the electron's orbit. Both of these are internal atomic properties. However, the linear momentum of the light, can change only the external, translational motion of the atom.