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Journal of Experimental and Theoretical Physics

Dynamics of moving interacting atoms in a laser radiation field and optical size resonances

O. N. Gadomskiĭ, A. G. Glukhov

Published Feb 1, 2005• 0 citations
Publisher

Abstract

The forces acting on interacting moving atoms exposed to resonant laser radiation are calculated. It is shown that the forces acting on the atoms include the radiation pressure forces as well as the external and internal bias forces. The dependences of the forces on the atomic spacing, polarization, and laser radiation frequency are given. It is found that the internal bias force associated with the interaction of atomic dipoles via the reemitted field may play an important role in the dynamics of dense atomic ensembles in a light field. It is shown that optical size resonances appear in the system of interacting atoms at frequencies differing substantially from transition frequencies in the spectrum of atoms. It is noted that optical size resonances as well as the Doppler frequency shift in the spectrum of interacting atoms play a significant role in the processes of laser-radiation-controlled motion of the atoms.

DOI
10.1134/1.1884665

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The forces acting on interacting moving atoms exposed to resonant laser radiation are calculated. It is shown that the forces acting on the atoms include the radiation pressure forces as well as the external and internal bias forces. The dependences of the forces on the atomic spacing, polarization, and laser radiation frequency are given. It is found that the internal bias force associated with the interaction of atomic dipoles via the reemitted field may play an important role in the dynamics of dense atomic ensembles in a light field. It is shown that optical size resonances appear in the system of interacting atoms at frequencies differing substantially from transition frequencies in the spectrum of atoms. It is noted that optical size resonances as well as the Doppler frequency shift in the spectrum of interacting atoms play a significant role in the processes of laser-radiation-controlled motion of the atoms.
The present state of research on the cooling of atomic ensembles by means of laser radiation pressure is discussed. First the basic theory of resonance radiation pressure is reviewed. The effect of recoil on the drift and fluctuations of the momentum of an atom interacting with resonance radiation is examined. There is an analysis of the forces acting on an atom in some simple light fields: a traveling plane wave, a Gaussian beam, and counterpropagating Gaussian beams. The review then focuses on the monochromatization of atoms by resonance radiation pressure and related methods for laser cooling of atoms. The roles played by the radiation pressure force and by momentum diffusion in shaping the narrow velocity distributions of the ensemble of atoms are analyzed. The lowest temperature obtainable in the radiation cooling of atoms is estimated. The basic experimental methods for laser cooling of atomic beams are described. Problems of the three-dimensional cooling of atomic ensembles and problems of localizing cold atoms in light fields, steady-state magnetic fields, and electrostatic fields are discussed. The review concludes with a discussion of some applications of cold atoms in high-precision spectroscopy, frequency standards, and atomic physics.
The forces acting on a resonance particle in the fields of laser radiation sources can be large. Acceleration, heating, and cooling of atoms by using these forces are discussed. Since the forces are of a resonance type, one can employ them to separate isotopes and excited atoms from unexcited atoms. Light pressure can play an important role in the spectroscopy of narrow atomic and molecular resonances. The quantum features of the motion of particles in a standing light wave are manifested in a fine structure of the absorption coefficient. This review is concerned with analyzing the resonance light-pressure forces and discussing the application of them in optics and quantum electronics.
We report the investigation of the influence of atomic motion on the fluorescence dynamics of a dilute atomic ensemble driven by resonance pulse radiation. We show that even for sub-Doppler temperatures, the motion of atoms can significantly affect the nature of both superradiation and subradiation. We also demonstrate that, in the case of an ensemble of moving scatterers, it is possible to observe the nonmonotonic time dependence of the fluorescence rate. This leads to the fact that, in certain time intervals, increasing temperature causes not an decrease but an increase of the fluorescence intensity in the cone of coherent scattering. We analyze the role of the frequency diffusion of secondary radiation as a result of multiple light scattering in an optically dense medium. It is shown that spectrum broadening is the main factor which determines radiation trapping upon resonant excitation. Along with broadening, we found a shift and distortion of the shape of the spectrum over time. At later time, after the trapping stage, the dynamics is dominated by close pairs of atoms (dimers). The dynamics of the excited states of these dimers has been studied in detail. It is shown that the change in the lifetime of the given adiabatic term of the diatomic quasimolecule induced by the change in the interatomic distance as well as possible nonadiabatic transitions between sub- and superradiant states caused by atomic motion can lead not to the anticipated weakening of subradiation effect, but to its enhancement.
The usual form of electromagnetic forces is given by but for neutral atoms q = 0. The next order of force is the dipole term, but this also vanishes because neutral atoms have no inherent dipole moment. However, a dipole moment can be induced by a field, and this is most efficient if the field is alternating near the atomic resonance frequency. Since these frequencies are typically in the optical range, dipole moments are efficiently induced by shining nearly resonant light on the atoms. Laser cooling and trapping rely on the interaction between laser light and atoms to exert a controllable force on the atoms, and many sophisticated schemes have been developed using the special properties of the interaction. This chapter begins with the simplest schemes for exerting optical forces on atoms, namely a single-frequency light field interacting with a two-level atom. Although this is the simplest possible scheme, it is pedagogically valuable because it shows many of the features that will be encountered further on. The ultimate temperature using such a scheme is limited, but lower temperatures can be achieved with multilevel atoms. This topic is addressed later in the chapter. Two kinds of optical forces When an atom absorbs nearly resonant light, it makes a transition to the excited state, and its subsequent return to the ground state can be either by spontaneous or by stimulated emission. The nature of the optical force that arises from these two different processes is quite different, and will be described separately [1]. The spontaneous emission case is different from the familiar quantum mechanical calculations using state vectors to describe the state of the system, because spontaneous emission causes the state of the system to evolve from a pure state into a mixed state (see Exercise 6.9). Spontaneous emission is an essential ingredient for the dissipative nature of the optical forces in monochromatic light, and the density matrix is needed to describe it (see Chap. 6). When an atom absorbs light, its energy excites the atom and its angular momentum changes the electron's orbit. Both of these are internal atomic properties. However, the linear momentum of the light, can change only the external, translational motion of the atom.
A theoretical analysis is given of the interaction of a laser field consisting of two orthogonal, linearly polarized, low-power standing waves, with an ensemble of J=1/2 ground-state atoms. The atoms are assumed to move with velocities below the Doppler limit of laser cooling. The two-dimensional light-induced atomic force is calculated for the specific case when the field polarization directions differ by \ensuremath{\pi}/2. The effective optical-pumping time is shown to increase strongly near the nodes of the laser field, leading to a force that can be much larger than that in the one-dimensional case. The force is not isotropic, and can lead to the bunching of the atoms in velocity space.