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Quantum Electronics

Nonlinear mixing in the presence of transparency induced by an additional strong field

Vasily G. Arkhipkin

Published Jan 31, 1995• 3 citations
Publisher

Abstract

It is shown that the use of additional strong laser radiation may result in a resonant increase of the nonlinear susceptibility in the generation of the sum frequency and harmonics, and it may also reduce the absorption of the generated radiation near the centres of the Stark-split components. The phase-matching conditions are also satisfied near these centres. The conversion efficiency is two or three orders of magnitude higher than in the absence of an additional strong radiation field.

DOI
10.1070/qe1995v025n01abeh000289

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It is shown that the use of additional strong laser radiation may result in a resonant increase of the nonlinear susceptibility in the generation of the sum frequency and harmonics, and it may also reduce the absorption of the generated radiation near the centres of the Stark-split components. The phase-matching conditions are also satisfied near these centres. The conversion efficiency is two or three orders of magnitude higher than in the absence of an additional strong radiation field.
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Three-wave frequency mixing is theoretically investigated under simultaneous single- and two-photon resonances; one of the fundamental fields is weak while another one is strong. The influence of field splitting on nonlinear susceptibility is studied for both homogeneously- and Doppler-broadened transitions. We analyzed the role of interference of quantum transitions via quasilevels in absorption and nonlinear generation and its impact on mixing process. The possibility of significant enhancement of nonlinear generation efficiency in optically dense media is demonstrated.