We experimentally demonstrate the efficient channeling of fluorescence photons from single q-dots into single-mode optical fiber, by measuring the photon-count rates through the guided and radiation modes simultaneously for various diameters of nanofiber.
We experimentally demonstrate the efficient channeling of fluorescence photons from single q dots on optical nanofiber into the guided modes by measuring the photon-count rates through the guided and radiation modes simultaneously. We obtain the maximum channeling efficiency to be 22.0(±4.8)% at a fiber diameter of 350 nm for the emission wavelength of 780 nm. The results may open new possibilities in quantum information technologies for generating single photons into single-mode optical fibers.
This thesis presents single photon generation and spectroscopy using quantum dots (q-dots) on optical nanofibers. Optical nanofibers are essentially vacuum-clad silica fibers with sub-wavelength diameter, which can support only the propagation of the fundamental mode through the guided mode. Optical nanofibers are realized using adiabatically tapered single mode optical fibers. Experiments were performed by depositing colloidal core-shell type CdSeTe (ZnS) q-dots on the optical nanofiber surface. A method is developed to deposit single q-dots systematically and reproducibly along the optical nanofiber. In the view point of investigation of fluorescence photon emission characteristics for single q-dots on optical nanofibers, the absolute fluorescence photon-count rates channeled into the nanofiber guided modes and the normalized photon correlations at various excitation laser intensities are measured. The results are able to obtain the product between the fluorescence photon channeling efficiency and the quantum efficiency of the single q-dots. However, the channeling efficiency cannot be determined without accurate information on the quantum efficiency of the single q-dots. Therefore, a method is devised to determine the channeling of fluorescence photons from single q-dots into the guided modes by measuring the fluorescence photon-count rates through the guided and radiation modes simultaneously. By measuring for various nanofiber diameters, a maximum channeling efficiency obtained to be 22.0 (±4.8)% at a fiber diameter of 350 nm for an emission wavelength of 780 nm. The measured results completely reproduce the theoretical predictions within the experimental error. We demonstrate in situ measurements of fluorescence quantum efficiency of single q-dots using the present nanofiber technique. We determine fluorescence quantum efficiency of single q-dots accurately by assuming the theoretical values for the channeling efficiency from the product of the channeling efficiency and the quantum efficiency. We demonstrate that one can pick up one q-dot on the nanofiber with fluorescence quantum efficiency higher than the average value measured for an ensemble. Thus, the optical nanofiber method offers a promising way for generating and manipulating single photons. This work should provide a basis for extending the optical nanofiber method to a general technique in quantum optics, which may open new possibilities in quantum information technologies.
We experimentally investigate the fluorescence photon emission characteristics for single q-dots by using optical nanofibers. We demonstrate that single q-dots can be deposited along an optical nanofiber systematically and reproducibly with a precision of 5 μm. For single q-dots on an optical nanofiber, we measure the fluorescence photon numbers coupled into the nanofiber and the normalized photon correlations, by varying the excitation laser intensity. We estimate the fluorescence photon coupling efficiency into the nanofiber guided modes.
Abstract We discuss how optical nanofibers, subwavelength-diameter fibers, can open new perspectives in quantum optical technologies theoretically and experimentally. Discussions are mainly focused on the manipulation of spontaneous emission for atoms around the nanofiber. We show that photons from single quantum emitters can be efficiently channeled into guided modes of the nanofiber. Especially by fabricating a cavity structure of the nanofiber, the channeling efficiency can be improved to exceed 80% although the cavity finesse is moderate. We discuss also how to realize such a nanofiber cavity experimentally.