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Advances in Natural Sciences Nanoscience and Nanotechnology

Manipulating single atoms and photons using optical nanofibers

K. Hakuta, K. P. Nayak

Published Feb 21, 2012• 11 citations
Publisher

Abstract

Abstract We discuss how optical nanofibers, subwavelength-diameter fibers, can open new perspectives in quantum optical technologies theoretically and experimentally. Discussions are mainly focused on the manipulation of spontaneous emission for atoms around the nanofiber. We show that photons from single quantum emitters can be efficiently channeled into guided modes of the nanofiber. Especially by fabricating a cavity structure of the nanofiber, the channeling efficiency can be improved to exceed 80% although the cavity finesse is moderate. We discuss also how to realize such a nanofiber cavity experimentally.

DOI
10.1088/2043-6262/3/1/015005

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•Jan 1, 2012•1 citation
Abstract We discuss how optical nanofibers, subwavelength-diameter fibers, can open new perspectives in quantum optical technologies theoretically and experimentally. Discussions are mainly focused on the manipulation of spontaneous emission for atoms around the nanofiber. We show that photons from single quantum emitters can be efficiently channeled into guided modes of the nanofiber. Especially by fabricating a cavity structure of the nanofiber, the channeling efficiency can be improved to exceed 80% although the cavity finesse is moderate. We discuss also how to realize such a nanofiber cavity experimentally.
Abstract Recent advances in the coherent control of single quanta of light, photons , is a topic of prime interest, and is discussed under the banner of quantum photonics . In the last decade, the subwavelength diameter waist of a tapered optical fiber, referred to as an optical nanofiber , has opened promising new avenues in the field of quantum optics, paving the way toward a versatile platform for quantum photonics applications. The key feature of the technique is that the optical field can be tightly confined in the transverse direction while propagating over long distances as a guided mode and enabling strong interaction with the surrounding medium in the evanescent region. This feature has led to surprising possibilities to manipulate single atoms and fiber-guided photons, e.g. the efficient channeling of emission from single atoms and solid-state quantum emitters into the fiber-guided modes, high optical depth with a few atoms around the nanofiber, trapping atoms around a nanofiber, and atomic memories for fiber-guided photons. Furthermore, implementing a moderate longitudinal confinement in nanofiber cavities has enabled the strong coupling regime of cavity quantum electrodynamics to be reached, and the long-range dipole–dipole interaction between quantum emitters mediated by the nanofiber offers a platform for quantum nonlinear optics with an ensemble of atoms. In addition, the presence of a longitudinal component of the guided field has led to unique capabilities for chiral light–matter interactions on nanofibers. In this article, we review the key developments of the nanofiber technology toward a vision for quantum photonics on an all-fiber interface.
Optical nanofibers provide a versatile platform for exploring strong light-matter interactions at the single-quantum level, a central goal of quantum optics. Their subwavelength diameter supports tightly confined guided modes with strong evanescent fields, enabling efficient coupling between photons and nearby atoms. By incorporating fiber Bragg gratings, nanofibers can form fully fiber-integrated high-finesse cavities, combining strong atom-photon coupling with efficient and low-loss optical input-output interfacing in the setting of cavity quantum electrodynamics (QED). In parallel, nanofiber systems naturally realize waveguide QED, where atoms interact strongly with propagating photons in a one-dimensional geometry. In this review, we introduce the underlying physical principles, summarize key experimental techniques and representative phenomena, and discuss prospects for applications in quantum information processing, quantum networks, and related quantum technologies.
Tapered optical fiber with subwavelength diameter waist, an optical nanofiber, provides a unique and versatile platform for manipulating atoms and photons. In the guided modes of the nanofibers, the optical field can be tightly confined in the transverse direction while enabling strong interaction with the surrounding medium in the evanescent region. Combining laser-cooled atoms with nanofibers has enabled surprising quantum optics experiments, e.g. the efficient channeling of emission from single atoms into the fiber-guided modes, spectroscopy of near-surface atoms, high optical depth with an array of atoms optically trapped around the nanofiber, atomic memories and Bragg reflectors for fiber-guided photons, chiral light-matter interaction etc. In addition, using moderate longitudinal confinement in nanofiber cavities has enabled strong coupling between a single atom and fiber-guided photons. In this article, I review some of the key experimental demonstrations on the “atom＋nanofiber” platform.
We experimentally demonstrate the efficient channeling of fluorescence photons from single q dots on optical nanofiber into the guided modes by measuring the photon-count rates through the guided and radiation modes simultaneously. We obtain the maximum channeling efficiency to be 22.0(±4.8)% at a fiber diameter of 350 nm for the emission wavelength of 780 nm. The results may open new possibilities in quantum information technologies for generating single photons into single-mode optical fibers.
This thesis presents single photon generation and spectroscopy using quantum dots (q-dots) on optical nanofibers. Optical nanofibers are essentially vacuum-clad silica fibers with sub-wavelength diameter, which can support only the propagation of the fundamental mode through the guided mode. Optical nanofibers are realized using adiabatically tapered single mode optical fibers. Experiments were performed by depositing colloidal core-shell type CdSeTe (ZnS) q-dots on the optical nanofiber surface. A method is developed to deposit single q-dots systematically and reproducibly along the optical nanofiber. In the view point of investigation of fluorescence photon emission characteristics for single q-dots on optical nanofibers, the absolute fluorescence photon-count rates channeled into the nanofiber guided modes and the normalized photon correlations at various excitation laser intensities are measured. The results are able to obtain the product between the fluorescence photon channeling efficiency and the quantum efficiency of the single q-dots. However, the channeling efficiency cannot be determined without accurate information on the quantum efficiency of the single q-dots. Therefore, a method is devised to determine the channeling of fluorescence photons from single q-dots into the guided modes by measuring the fluorescence photon-count rates through the guided and radiation modes simultaneously. By measuring for various nanofiber diameters, a maximum channeling efficiency obtained to be 22.0 (±4.8)% at a fiber diameter of 350 nm for an emission wavelength of 780 nm. The measured results completely reproduce the theoretical predictions within the experimental error. We demonstrate in situ measurements of fluorescence quantum efficiency of single q-dots using the present nanofiber technique. We determine fluorescence quantum efficiency of single q-dots accurately by assuming the theoretical values for the channeling efficiency from the product of the channeling efficiency and the quantum efficiency. We demonstrate that one can pick up one q-dot on the nanofiber with fluorescence quantum efficiency higher than the average value measured for an ensemble. Thus, the optical nanofiber method offers a promising way for generating and manipulating single photons. This work should provide a basis for extending the optical nanofiber method to a general technique in quantum optics, which may open new possibilities in quantum information technologies.