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Journal of the Optical Society of America B

Multiwave diffraction in saturable absorbers

K. Divakara Rao, K. K. Sharma

Published Apr 1, 1995• 6 citations
Publisher

Abstract

We present an analytical description of the degenerate multiwave diffraction of an independent probe beam incident at an arbitrary angle upon a population grating created by two resonant and coherent pump beams in a saturable absorbing medium. We have also undertaken experimental verification of some of the features, using a thin-film sample of Rhodamine 6G-doped boric acid glass. It is found that the three-beam configuration provides a broader angular bandwidth for observing nonlinear effects.

DOI
10.1364/josab.12.000658

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We present an analytical description of the degenerate multiwave diffraction of an independent probe beam incident at an arbitrary angle upon a population grating created by two resonant and coherent pump beams in a saturable absorbing medium. We have also undertaken experimental verification of some of the features, using a thin-film sample of Rhodamine 6G-doped boric acid glass. It is found that the three-beam configuration provides a broader angular bandwidth for observing nonlinear effects.
The optical phase conjugation signal in nearly nondegenerate four wave mixing was studied using a rhodamine 110 doped boric acid glass saturable absorber nonlinear medium. We have demonstrated a narrow band optical filter (2.56±0.15Hz) using an optical phase conjugation signal in the frequency modulation of a weak probe beam in the presence of two strong counterpropagating pump beams in rhodamine 110 doped boric acid glass thin films (10−4m). Both the pump beams and the probe beam are at a wavelength of 488nm (continuous-wave Ar+ laser). The probe beam frequency was detuned with a ramp signal using a piezoelectric transducer mirror.
The temporal evolution of optical nonlinearities is an important element in the choice of materials suitable for applications such as optical switches, real-time optical correlators, and optical memories. In this paper, we report a study of the nonlinear optical properties of a (1) saturable absorber (rhodamine 6G) in solution (water and methanol) and also embedded in a polyvinyl alcohol matrix and (2) a thin film of glass doped with CdSxSe1-x microcrystallites. The temporal response of the phase-conjugate signal obtained by degenerate four-wave mixing, as well as the dynamic of higher-order resonant signals have been investigated by means of a frequency-doubled picosecond Nd:YAG laser. Intensity-dependent relaxation times have been found for some materials. Merit figures (defined as the ratio between the nonlinear susceptibility and its relaxation time) of these media have been considered for different polarization configurations. Physical mechanisms involved in the grating relaxation for these different media will be discussed.
In a highly nonlinear thin film, the presence of the diffracted beams from the pump-probe-beam-induced refractive-index grating modifies considerably the energy coupling between the pump and the probe beams. Using coupled amplitude and phase equations, the roles of various factors such as phases and phase shifts, phase modulations, pump-beam intensity, intensity ratio, interaction length, and losses in the medium in the multiwave-mixing processes are clearly identified. We also present experimental results on the dependence of the probe gain on the pump-probe-beam ratio, the pump intensity, and on the interaction length, using a nematic liquid-crystal film as the nonlinear medium.
We report the energy-transfer efficiency in a saturable absorber nonlinear media by two-coherent-wave coupling using the Doppler shift. Intensity-dependent nondegenerate two-beam coupling has been studied in Rhodamine 110-doped boric acid glass films. Two beams have been described in the limit of a weak probe and a relatively strong pump at the wavelength 488 nm from a continuous-wave Ar+ laser. The results have been interpreted in terms of the four-level description of a saturable absorber. We obtained good agreement between the experimental and the theoretical results. Estimated values of the nonlinear parameters such as the saturation intensity, refractive index, and the response time of the optical nonlinearity have been obtained at different pump beam intensities for the first time, to our knowledge, in the Rhodamine 110-doped film.
Further theoretical observations and a new analysis of stationary degenerate and nearly degenerate optical wave mixing effects in a Kerr-like nonlinear medium are presented. The effects of phase modulations, beam ratio, intensity, wave mixing angle and frequency differences and other physical and optical parameters in multiwave mixing mediated probe gain and their application in ring oscillation devices are analyzed in detail. New experimental studies of the intensity and the angular dependence of the probe beam amplification and side diffractions in liquid crystal provide further insights into the phenomena.