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Advances in Natural Sciences Nanoscience and Nanotechnology

Observation of green lasing at 537 nm from Er-ions by coupled photon–atom modes in a random cavity

Van Hoi Pham, Thuy Chi, Huy Bui, The Anh Nguyen, Thuy Van Nguyen

Published Mar 1, 2011• 1 citation
Publisher

Abstract

Abstract We present new results of a laser phenomenon that gives rise to a narrow green emission mode in a random photonic-crystal cavity based on an Er-doped glass–air gap–polymer with a 976 nm diode laser pump. Lasing occurs at 537 nm, which does not respond to the resonant radiative transition 2 H 11/2→4 I 15/2; 4 S 3/2→4 I 15/2 in Erbium ions. This effect can be seen as photon–atom coupling in the context of the interaction between a single atom and/or a few atoms and resonant optical media, such as cavities or photonic crystals. Experimental results show that the random lasing mode directly originates from the coupled photon–atom mode inside the random cavity. The measured Q-factor is of 2100–2800 for a random cavity with an air gap of 600–1700 nm between Er-doped glass fiber and a coated polymer layer.

DOI
10.1088/2043-6262/2/1/015004

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Optics Letters•Dec 1, 1992•35 citations
Abstract We present new results of a laser phenomenon that gives rise to a narrow green emission mode in a random photonic-crystal cavity based on an Er-doped glass–air gap–polymer with a 976 nm diode laser pump. Lasing occurs at 537 nm, which does not respond to the resonant radiative transition 2 H 11/2→4 I 15/2; 4 S 3/2→4 I 15/2 in Erbium ions. This effect can be seen as photon–atom coupling in the context of the interaction between a single atom and/or a few atoms and resonant optical media, such as cavities or photonic crystals. Experimental results show that the random lasing mode directly originates from the coupled photon–atom mode inside the random cavity. The measured Q-factor is of 2100–2800 for a random cavity with an air gap of 600–1700 nm between Er-doped glass fiber and a coated polymer layer.
Summary form only given: Amplification in rare-earth doped solid state planar optical structures has attracted a lot of interest in recent years due to the fact that the rare earth ions show sharp absorption and emission bands and relatively long luminescence lifetimes. In particular the erbium (Er) ion is very attractive because of its intra 4f-transition from the first excited state to the ground state around 1.53 mum (4I13/2-4I15/2). The main problem of the erbium doped waveguide amplifiers (EDWAs) is that high values of the Er3+concentration are required to reach high gain figures in a compact length, but in this way the concentration quenching effects become very considerable and detrimental to the optical gain, since they reduce the population in the first excited state. A good solution to overcome this dramatic drawback is to consider erbium doped photonic crystal amplifier (EDPCA). In fact the small group velocity of electromagnetic eigenmodes brings about the enhancement of stimulated emission if the photonic crystals are doped by active media as the rare earth ions E3+r or Yt3+. This phenomenon originates from the long interaction time between radiation field and the matter caused by the small group velocity near the edge of the photonic band gap. The efficient confinement of light is achievable not only by tuning the input signal at the band edge of the gap of the photonic crystal but it is also obtainable by introducing local defects inside photonic crystals. The density of electromagnetic states inside a cavity is significantly modified and the spontaneous emission of atoms in a cavity can be either enhanced or inhibited. Erbium doped silica-titania one-dimensional photonic crystal microcavities have been analyzed by solving the erbium rate equations and the Maxwell equations by means of an auxiliary differential equation finite difference time domain technique. Since the performance of optical amplifiers depends on the populations of the energy levels participating in radiative transitions, determined principally by the distribution and concentration of the rare-earth ions and by the pumping conditions, the relations between these parameters and the transmittance of the EDPCMA have been studied
Light emission at 1.54 microm from an Er-doped amorphous silicon nitride layer coupled to photonic crystal resonators at cryogenic and room temperatures and under varying optical pump powers has been studied. The results demonstrate that small mode volume, high quality factor resonators enhance Er absorption and emission rates at the cavity resonance. Time resolved measurements give 11- to 17-fold Purcell enhancement of spontaneous emission at cryogenic temperatures, and 2.4-fold enhancement at room temperature. Resonances exhibit linewidth narrowing with pump power, signifying absorption bleaching and partial inversion of the Er ions cryogenic temperatures. We estimate that 31% of Er ions are excited at the highest pump power.
Er 3+ ions produce a sharp line emission that has small absorption cross section, long radiative lifetime, and is independent of external perturbations. These optical properties of the Er3+ ions limit the pumping efficiency and tunability of the emission line. In this work we present a study in which Er3+ emission was modified by coupling an ensemble of Er3+ ions to a microcavity resonance. The optical response of an optical cavity that consists of an Er2O3 layer confined between Si/SiO2 distributed Bragg reflectors is studied. When the cavity is in resonance with the optical transition of the Er3+ ions, the resonances in the reflectivity spectra split. The results are explained by a standard semiclassical model of atom–photon coupling.
One-dimensional nanobeam photonic crystal cavities are fabricated in an Er-doped amorphous silicon nitride layer.Photoluminescence from the cavities around 1.54 µm is studied at cryogenic and room temperatures at different optical pump powers.The resonators demonstrate Purcell enhanced absorption and emission rates, also confirmed by time-resolved measurements.Resonances exhibit linewidth narrowing with pump power, signifying absorption bleaching and the onset of stimulated emission in the material at both 5.5 K and room temperature.We estimate from the cavity linewidths that Er has been pumped to transparency at the cavity resonance wavelength.
Erbium is a rare-earth metal that, when incorporated in a solid, can emit light at a wavelength of 1.5 μm. It plays a key role in current day telecommunication technology as the principle ingredient of optical fiber amplifiers. In this thesis the control of the Er spontaneous emission in three different types of microphotonic materials is described. Part I of this thesis focuses on the effect of a metallo-dielectric interface on the spontaneous emission of optical emitters in silica glass. It is shown that Er ions near a Ag interface can couple to surface plasmons (SPs) via a near-field interaction. By coupling SPs out into the far field, large changes in the Er photoluminescence emission distribution, spectra, and polarization can be observed. The excitation of SPs also results in an increase of the Er photoluminescence decay rate. The observed decay rates are in good agreement with calculations based on a classical dipole oscillator model. From the change in photoluminescence decay rate of Si nanocrystals near a Ag interface it is shown that Si nanocrystals can efficiently excite SPs and have an internal quantum efficiency of 77 %. Part II focuses on the effect of a microcavity on the spontaneous emission of Er and describes how ion implantation can be used to dope dielectric microresonators with optically active Er ions. The fabrication and characterization of an Er ion-implanted silica microsphere resonator is described that shows lasing at 1.5 μm when pumped above its lasing threshold. Ion implantation is also used to dope toroidal microcavities on a Si chip with Er. The microtoroids are doped by either pre-implantation into the SiO2 base material, or by post-implantation in a fully fabricated microtoroid. The optical activation of Er ions in the microtoroid is investigated and Er lasing at 1.5 μm is observed for both types of microcavities with the lowest threshold (4.5 μW) for the pre-implanted microtoroids. Part III describes the fabrication of an Er-doped Si-inverse opal photonic crystal. These photonic crystals can potentially have a photonic bandgap that can fully inhibit the spontaneous emission of on optical emitter. Fabrication criteria are derived for such a photonic crystal, based on the lattice parameter, filling fraction, and Si refractive index. In the opal photonic crystal composed of both Si and SiO2 we show that Er ions can be selectively excited in both the Si and SiO2 part of the photonic crystal by changing the excitation wavelength and/or the measurement temperature.