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Measures of Nonclassical Correlations and Quantum-Enhanced Interferometry

Matthias Lang

Published Jan 1, 2015• 0 citations
OpenAlex

Abstract

In the first part of this dissertation a framework for categorizing entropic measures of nonclassical correlations in bipartite quantum states is presented. The measures are based on the difference between a quantum entropic quantity and the corresponding classical quantity obtained from measurements on the two systems. Three types of entropic quantities are used, and three different measurement strategies are applied to these quantities. Many of the resulting measures of nonclassical correlations have been proposed previously. Properties of the various measures are explored, and results of evaluating the measures for two-qubit quantum states are presented. To demonstrate how these measures differ from entanglement we move to the set of Bell-diagonal states for two qubits, which can be depicted as a tetrahedron in three dimensions. We consider the level surfaces of entanglement and of the correlation measures from our framework for Bell-diagonal states. This provides a complete picture of the structure of entanglement and discord for this simple case and, in particular, of their nonanalytic behavior under decoherence. The pictorial approach also indicates how to show that all of the proposed correlation measures are neither convex nor concave. In the second part we look at two practical interferometric setups that use nonclassical states of light to enhance their performance. First we consider an interferometer powered by laser light (a coherent state) into one input port and ask the following question: what is the best state to inject into the second input port, given a constraint on the mean number of photons this state can carry, in order to optimize the interferometer's phase sensitivity? This question is the practical question for high-sensitivity interferometry. We answer the question by considering the quantum Cram\'er-Rao bound for such a setup. The answer is squeezed vacuum. Then we analyze the ultimate bounds on the phase sensitivity of an interferometer, given the constraint that the state input to the interferometer's initial 50:50 beam splitter B is a product state of the two input modes. Requiring a product state is a natural restriction: if one were allowed to input an arbitrary, entangled two-mode state $|\Xi \rangle$ to the beam splitter, one could generally just as easily input the state $B|\Xi \rangle$ directly into the two modes after the beam splitter, thus rendering the beam splitter unnecessary. We find optimal states for a fixed photon number and for a fixed mean photon number. Our results indicate that entanglement is not a crucial resource for quantum-enhanced interferometry. Initially the analysis for both of these setups is performed for the idealized case of a lossless interferometer. Then the analysis is extended to the more realistic scenario where the interferometer suffers from photon losses.

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In the first part of this dissertation a framework for categorizing entropic measures of nonclassical correlations in bipartite quantum states is presented. The measures are based on the difference between a quantum entropic quantity and the corresponding classical quantity obtained from measurements on the two systems. Three types of entropic quantities are used, and three different measurement strategies are applied to these quantities. Many of the resulting measures of nonclassical correlations have been proposed previously. Properties of the various measures are explored, and results of evaluating the measures for two-qubit quantum states are presented. To demonstrate how these measures differ from entanglement we move to the set of Bell-diagonal states for two qubits, which can be depicted as a tetrahedron in three dimensions. We consider the level surfaces of entanglement and of the correlation measures from our framework for Bell-diagonal states. This provides a complete picture of the structure of entanglement and discord for this simple case and, in particular, of their nonanalytic behavior under decoherence. The pictorial approach also indicates how to show that all of the proposed correlation measures are neither convex nor concave. In the second part we look at two practical interferometric setups that use nonclassical states of light to enhance their performance. First we consider an interferometer powered by laser light (a coherent state) into one input port and ask the following question: what is the best state to inject into the second input port, given a constraint on the mean number of photons this state can carry, in order to optimize the interferometer's phase sensitivity? This question is the practical question for high-sensitivity interferometry. We answer the question by considering the quantum Cram'er-Rao bound for such a setup. The answer is squeezed vacuum. Then we analyze the ultimate bounds on the phase sensitivity of an interferometer, given the constraint that the state input to the interferometer's initial 50:50 beam splitter B is a product state of the two input modes. Requiring a product state is a natural restriction: if one were allowed to input an arbitrary, entangled two-mode state ∣Ξ⟩|\Xi \rangle∣Ξ⟩ to the beam splitter, one could generally just as easily input the state B∣Ξ⟩B|\Xi \rangleB∣Ξ⟩ directly into the two modes after the beam splitter, thus rendering the beam splitter unnecessary. We find optimal states for a fixed photon number and for a fixed mean photon number. Our results indicate that entanglement is not a crucial resource for quantum-enhanced interferometry. Initially the analysis for both of these setups is performed for the idealized case of a lossless interferometer. Then the analysis is extended to the more realistic scenario where the interferometer suffers from photon losses.
Quantum-enhanced interferometers utilize non-classical states of light in order to surpass the limitations imposed by classical physics on phase measurement sensitivity and resolution. We review key scientific developments in this growing field of research and derive fundamental metrology concepts, namely the Cram\'{e}r-Rao bound and the Fisher information, which are used to analyze the metrological performance of quantum states of light. We propose a supersensitive quantum interferometry protocol that can be amplified to the macroscopic realm (i.e. the mean number of photons of the probe state can reach approximately 100,000 photons) using contemporary techniques of spontaneous parametric down conversion. The parity measurement on the output field asymptotically saturates the quantum Cram\'{e}r-Rao bound, which scales like the Heisenberg limit. We uncover the role of photon statistics on phase sensitivity and rule out the necessity of mode entanglement for quantum-enhanced interferometry. Based on these insights we outline a practical metrology technique (independent of mode entanglement) that measures a phase delay of a single-mode anti-squeezing operation. This scheme can also be scaled macroscopically using contemporary techniques and is shown to significantly surpass the shot-noise limit (SNL) in the presence of realistic losses. Finally, the physical resources that enable quantum-enhanced interferometry is studied by analyzing the quantum Fisher information (QFI) using the first quantization and the second quantization formalisms of quantum mechanics. It is shown that increasing the intra-mode correlations of an interferometer (as quantified by the second order Glauber coherence function) can be conducive to attaining a quantum advantage in phase estimation; whereas, introducing mode entanglement can reduce phase sensitivity. Using the first quantization description, we derive a formula for the QFI that shows explicitly how the Heisenberg scaling term depends on particle entanglement.
We analyze the ultimate bounds on the phase sensitivity of an interferometer, given the constraint that the state input to the interferometer's initial 50:50 beam splitter BBB is a product state of the two input modes. Requiring a product state is a natural restriction: If one were allowed to input an arbitrary, entangled two-mode state $|\ensuremath{\Xi}\ensuremath{\rangle}$ to the beam splitter, one could generally just as easily input the state $B|\ensuremath{\Xi}\ensuremath{\rangle}$ directly into the two modes after the beam splitter, thus rendering the beam splitter unnecessary. We find optimal states for a fixed photon number and for a fixed mean photon number.
This is a two-part thesis strung together by a common underlying theme—quantum correlations. We present some new characterizations and quantifications of quantum correlations and an application of one such correlation—entanglement—for quantum technology. In Part I of the thesis, we use a Rényi generalization of the quantum conditional mutual information (QCMI) to define and study new measures of quantum entanglement and quantum discord. In particular, using a quantity derived from a Rényi QCMI, we introduce: a) the geometric squashed entanglement, a faithful entanglement measure, which is a lower bound on the squashed entanglement and which reduces to the geometric measure of entanglement for pure quantum states, b) the surprisal of measurement recoverability, a discord-like measure, which is similarly a lower bound on the quantum discord. The surprisal of measurement recoverability enhances our understanding of quantum discord in terms of the ability to recover one share of a bipartite quantum system after it has been measured. In Part II, we discuss entanglement-enhanced quantum sensing. In particular, we consider optical interferometric sensors that use photon-number parity detection. Using the quantum and classical Cramér-Rao bounds (QCRB and CCRB) on phase precision as the figures of merit, we characterize a class of two-mode pure states for which photon-number parity measurement is optimal for phase estimation. These states turn out to be a subset of the class of path-symmetric states—a class for which photon-number counting-based measurements are known to be optimal. Further, we gauge the performance of the particular interferometry based on coherent light mixed with squeezed vacuum light and photon-number parity measurement. We show that photon-number parity is an optimal measurement for the above state in the sense that the detection scheme is capable of achieving the best phase precision offered by the state (given by its QCRB). The state by itself is also known to be capable of optimal phase precision for any state in linear interferometry for a given photon budget, called the Heisenberg limit. Thus, we demonstrate Heisenberg-limited phase estimation for the state with photon-number parity detection.
This thesis fathoms the possibilities and limitations of measurements in quantum optics. After a short introduction to the general aspects of measurements in quantum mechanics, it presents three examples of a measurement process in concrete applications to quantum optics. For one, while operators describing quantities of interest might have a simple theoretical form, it is often hard to actually implement a measurement of their expectation values experimentally. This situation is encountered in the first part which is devoted to the measurement of quantum statistical properties of a light beam. In contrast to classical optics, these statistics are not fully determined by first- and second-order correlations. Instead, higher-order correlations, usually described by non-Hermitian operators, are necessary to characterize the quantum state completely. A particular example is the N-photon Fock state, for which only a measurement of the Nth-order correlations allows for a full characterization. Here, we present a new method how to measure an important class of Nth-order correlations for arbitrary N in a single spatial mode with two polarizations with limited experimental resources. The second part is again centered around the realization of specific measurement operators for photon correlation measurements. However, in contrast to the previous chapter, these measurements are not an end in their own, but are designed to create specific quantum states as a consequence of the measurement process: A suitable measurement of photons emitted by a number of atoms allows to transfer the atoms into long-lived entangled states. We find that with this method it is possible to entangle two remote atomic qubits to an arbitrary and well-defined degree. Furthermore, we show how to generate two families of quantum states in an arbitrary number of remote atomic qubits: one family consists of all -- symmetric and non-symmetric -- total angular momentum eigenstates in N remote qubits, the other is a family of cluster states. It is also systematically investigated whether the technique of quantum state engineering by projective measurements allows for the creation of any arbitrary state. We find explicit solutions for the case of two and three qubits, while it is shown that no solution exist for N > 6. We conclude the section by proving that with some changes in the setup, this measurement-based quantum state engineering technique allows to create the same states among the scattered photons themselves rather than among the emitting atoms. The last part is devoted to the amount of information one is able to gain about a given system when performing a measurement. The corresponding limits of information are investigated at the example of the duality that arises in a two-way interferometer between the visibility of the interference pattern and the knowledge about the path of the interfering object. We show that there exist correlations between the phase difference the interfering object acquires on its way through the interferometer and the amount of which-way information retrievable from certain observables of the which-way detector. In this way, the which-way information becomes a phase-dependent quantity. In particular, we find that for certain values of the phase shift, the amount of extractable which-way information can be larger than allowed by phase-independent measurement. This property is put to use to find the optimal observable for the which-way detector readout in dependence on the phase of the interfering object. Following this strategy, we are able to gain more which-way information than previously thought possible.
How can we characterize different types of correlation between quantum systems? Since correlations cannot be generated locally, we take any real function of a multipartite state which cannot increase under local operations to measure a correlation. Correlation measures that can be expressed as an optimization of a linear combination of entropies are particularly useful, since they can often be interpreted operationally. We systematically study such optimized linear entropic functions, and by enforcing monotonicity under local processing we identify four cones of correlation measures for bipartite quantum states. This yields two new optimized measures of bipartite quantum correlation that are particularly simple, which have the additional property of being additive.
We consider an interferometer powered by laser light (a coherent state) into one input port and ask the following question: what is the best state to inject into the second input port, given a constraint on the mean number of photons this state can carry, in order to optimize the interferometer's phase sensitivity? This question is the practical question for high-sensitivity interferometry. We answer the question by considering the quantum Cramér-Rao bound for such a setup. The answer is squeezed vacuum.