This dissertation deals with theoretical and experimental research on nonclassical, or entangled, states of atoms and photons. In the first part, I describe two approaches to the preparation of entangled states of a large number of atoms. The first approach is based on the transfer of quantum correlations from non-classical light to the atomic spins. I consider three different situations: (a) the atoms are placed in a loss-free cavity and no relaxation of any kind is present; (b) the atoms are placed in a cavity with input and output for the electromagnetic field and the atoms spontaneously decay from the upper state; (c) there is no cavity around the atoms and spontaneous emission is present. I show that in all three situations with judicious choice of parameters, entangled samples of atoms can be produced. The second approach is based on quantum-nondemolition (QND) measurements of collective atomic operators. I describe experiments with pulsed and cw light as the probe, that result in squeezed spin states of atoms. When a rf magnetic field is applied to the atomic sample, sub- shot noise performance of an atomic spin interferometer is demonstrated. In the second part of the thesis I describe investigations of phase properties of two-photon and single-photon states. These experiments make use of spontaneous type-II down-conversion in a nonlinear crystal. First, interferometric measurement of a phase shift at the Heisenberg limit for a two-photon state is described. Next, a violation of Bell-type inequalities in phase space is demonstrated for the quantum optical version of the Einstein-Podolsky-Rosen state. Finally, some recent work directed toward homodyning a single photon against a strong local oscillator field is described.
This dissertation deals with theoretical and experimental research on nonclassical, or entangled, states of atoms and photons. In the first part, I describe two approaches to the preparation of entangled states of a large number of atoms. The first approach is based on the transfer of quantum correlations from non-classical light to the atomic spins. I consider three different situations: (a) the atoms are placed in a loss-free cavity and no relaxation of any kind is present; (b) the atoms are placed in a cavity with input and output for the electromagnetic field and the atoms spontaneously decay from the upper state; (c) there is no cavity around the atoms and spontaneous emission is present. I show that in all three situations with judicious choice of parameters, entangled samples of atoms can be produced. The second approach is based on quantum-nondemolition (QND) measurements of collective atomic operators. I describe experiments with pulsed and cw light as the probe, that result in squeezed spin states of atoms. When a rf magnetic field is applied to the atomic sample, sub- shot noise performance of an atomic spin interferometer is demonstrated. In the second part of the thesis I describe investigations of phase properties of two-photon and single-photon states. These experiments make use of spontaneous type-II down-conversion in a nonlinear crystal. First, interferometric measurement of a phase shift at the Heisenberg limit for a two-photon state is described. Next, a violation of Bell-type inequalities in phase space is demonstrated for the quantum optical version of the Einstein-Podolsky-Rosen state. Finally, some recent work directed toward homodyning a single photon against a strong local oscillator field is described.
The fields of quantum and nonlinear optics have given rise to a variety of nonclassical states of light that have been proven to surpass certain limitations set by classical physics. Namely, certain squeezed and entangled states have been shown to beat the shot-noise limit when making precision phase measurements in interferometry, as well as write lithographic patterns that are smaller than classically allowed by the Rayleigh diffraction limit. Additionally, single-photon sources and entangled photon pairs have given rise to provably secure quantum key distribution for cryptography. Producing these quantum states of light has proven a difficult task. Nonlinear crystals, when pumped by a laser, produce pairs of single photons via the process of spontaneous parametric down conversion (SPDC). This process is mediated by the second order nonlinear susceptibility of the material. When pumped in a high gain regime, these crystals give rise to optical parametric amplification, which is a viable source of squeezed light. The vast majority of research in this area has focused on crystals that are seeded by vacuum in their two modes. This dissertation concerns the field of quantum nonlinear optics. It is an investigation into the processes that occur when nonlinear materials interact with the electromagnetic field on the single photon level. I have focused on seeding nonlinear crystals with quantum states of light, including single photons and entangled states. This process results in various states directly applicable to interferometry, imaging, and cryptography. Another application investigated is an absolute radiance measurement via stimulated parametric down conversion resulting from non-vacuum seeding of a nonlinear crystal. Additionally, other nonlinear processes, including four-wave mixing, nonlinear magneto-optical effects and coherent population trapping in warm atomic vapor involving quantum states of light are investigated. The process of seeding third-order nonlinear interactions, such as in atomic vapors, gives rise to a variety of interesting, nonclassical phenomena such as entangled image transfer and nonlocal imaging. Strong analogies between SPDC and four-wave mixing are drawn. I also experimentally show an all optical pi-only phase shift of one light beam via another in warm Cesium vapor.
The generation of entanglement in atomic systems plays a central topic in the fields of quantum information storage and processing. Moreover, a special category of entangled states of multi-atom ensembles, spin squeezed states, have been proven to lead to considerable improvement in the sensitivity of precision measurements compared to systems involving uncorrelated atoms. A treatment of entanglement in open systems is, however, incomplete without a precise description of the process of decoherence which necessarily accompanies it. The theory of entanglement and decoherence are the two main topics of this thesis. Methods are described for the generation of strong correlations in large atomic ensembles using either cavity quantum electrodynamics or measurement outcome conditioned quantum dynamics. Moreover, the description of loss of entanglement resulting from the coupling to a noise reservoir (electromagnetic vacuum) is explored. A spin squeezing parameter is used throughout this thesis as both a measure of entanglement strength and as an indication of the sensitivity improvement above the so-called standard quantum limit (sensitivity obtained with uncorrelated particles) in metrology. The first scheme considered consists of a single mode cavity field interacting with a collection of atoms for which spin squeezing is produced in both resonant and off-resonant regimes. In the resonant case, transfer of squeezing from a field state to the atoms is analyzed, while in the off-resonant regime squeezing is produced via an effective nonlinear interaction (one-axis twisting Hamiltonian). A second, more experimentally realistic case, is one involving the interaction of free space atoms with laser pulses; a projective measurement of a source field originating from atomic fluctuations provides a means of preparing atomic collective states such as spin squeezed and Schrodinger cat states. A new unravelling is proposed, that employs the detection of photon number in a single output channel and is capable of producing mesoscopic Schrodinger cat states in a single step. As a first step to understanding the role of cooperative decoherence, of importance in the case of dense pencil-shaped atomic ensembles, the collective spin decoherence of a two multilevel atom system is derived. This calculation is also relevant to entanglement loss for two qubits manipulated using with reading/writing pulses. Finally, a scheme is proposed in which arbitrarily strong entanglement can be produced in a four-wave mixing setup, where the preparation of the atoms in a dark state limits the decoherence to negligible values.
In 1935 Einstein, Podolsky and Rosen used the assumption of local realism to conclude in a Gedankenexperiment with two entangled particles that quantum mechanics is not complete. For this reason EPR motivated an extension of quantum mechanics by so-called local hidden variables. Based on this idea in 1964 Bell constructed a mathematical inequality whereby experimental tests could distinguish between quantum mechanics and local-realistic theories. Many experiments have since been done that are consistent with quantum mechanics, disproving the concept of local realism. But all these tests suffered from loopholes allowing a local-realistic explanation of the experimental observations by exploiting either the low detector efficiency or the fact that the detected particles were not observed space-like separated. In this context, of special interest is entanglement between different quantum objects like atoms and photons, because it allows one to entangle distant atoms by the interference of photons. The resulting space-like separation together with the almost perfect detection efficiency of the atoms allows a first loophole-free test of Bell's inequality. The primary goal of the present thesis is the experimental realization of entanglement between a single localized atom and a single spontaneously emitted photon at a wavelength suitable for the transport over long distances. In the experiment a single optically trapped Rb87 atom is excited to a state which has two selected decay channels. In the following spontaneous decay a photon is emitted coherently with equal probability into both decay channels. This accounts for perfect correlations between the polarization state of the emitted photon and the Zeeman state of the atom after spontaneous decay. Because these decay channels are spectrally and in all other degrees of freedom indistinguishable, the spin state of the atom is entangled with the polarization state of the photon. To verify entanglement, appropriate correlation measurements in complementary bases of the photon polarization and the internal quantum state of the atom are performed. It is shown, that the generated atom-photon state yields an entanglement fidelity of 0.82. The experimental results of this work mark an important step towards the generation of entanglement between space-like separated atoms for a first loophole-free test of Bell's inequality. Furthermore entanglement between a single atom and a single photon is an important tool for new quantum communication and information applications, e.g. the remote state preparation of a single atom over large distances.
After they have interacted, quantum particles generally behave as a single nonseparable entangled system. The concept of entanglement plays an essential role in quantum physics. We have performed entanglement experiments with Rydberg atoms and microwave photons in a cavity and tested quantum mechanics in situations of increasing complexity. Entanglement resulted either from a resonant exchange of energy between atoms and the cavity field or from dispersive energy shifts affecting atoms and photons when they were not resonant. With two entangled particles (two atoms or one atom and a photon), we have realized new versions of the Einstein-Podolsky-Rosen situation. The detection of one particle projected the other, at a distance, in a correlated state. This process could be viewed as an elementary measurement, one particle being a ‘‘meter’’ measuring the other. We have performed a ‘‘quantum nondemolition’’ measurement of a single photon, which we detected repeatedly without destroying it. Entanglement is also essential to understand decoherence, the process accounting for the classical appearance of the macroscopic world. A mesoscopic superposition of states (‘‘Schrodinger cat’’) gets rapidly entangled with its environment, losing its quantum coherence. We have prepared a Schrodinger cat made of a few photons and studied the dynamics of its decoherence, in an experiment which constitutes a glimpse at the quantum/classical boundary. We have also investigated entanglement as a resource for the processing of quantum information. By using quantum two-state systems (qubits) instead of classical bits of information, one can perform logical operations exploiting quantum interferences and taking advantage of the properties of entanglement. Manipulating as qubits atoms and photons in a cavity, we have operated a quantum gate and applied it to the generation of a complex three-particle entangled state. We finally discuss the perspectives opened by these experiments for further fundamental studies.
After they have interacted, quantum particles generally behave as a single nonseparable entangled system. The concept of entanglement plays an essential role in quantum physics. We have performed entanglement experiments with Rydberg atoms and microwave photons in a cavity and tested quantum mechanics in situations of increasing complexity. Entanglement resulted either from a resonant exchange of energy between atoms and the cavity field or from dispersive energy shifts affecting atoms and photons when they were not resonant. With two entangled particles (two atoms or one atom and a photon), we have realized new versions of the Einstein-Podolsky-Rosen situation. The detection of one particle projected the other, at a distance, in a correlated state. This process could be viewed as an elementary measurement, one particle being a ``meter'' measuring the other. We have performed a ``quantum nondemolition'' measurement of a single photon, which we detected repeatedly without destroying it. Entanglement is also essential to understand decoherence, the process accounting for the classical appearance of the macroscopic world. A mesoscopic superposition of states (``Schr\"odinger cat'') gets rapidly entangled with its environment, losing its quantum coherence. We have prepared a Schr\"odinger cat made of a few photons and studied the dynamics of its decoherence, in an experiment which constitutes a glimpse at the quantum/classical boundary. We have also investigated entanglement as a resource for the processing of quantum information. By using quantum two-state systems (qubits) instead of classical bits of information, one can perform logical operations exploiting quantum interferences and taking advantage of the properties of entanglement. Manipulating as qubits atoms and photons in a cavity, we have operated a quantum gate and applied it to the generation of a complex three-particle entangled state. We finally discuss the perspectives opened by these experiments for further fundamental studies.
This thesis is a dissemination of the experimental work I have carried out in the last three and a half years, under supervision of Prof. Miles Padgett and Dr. Sonja Franke-Arnold. Presented within are seven unique experiments investigating the orbital angular momentum (OAM) states of light, and the associated spatial modes. Six of these experiments relate to measurements on quantum-entangled photon pairs produced in down-conversion. The first chapter of my thesis is a brief review of the some of the contributions made to the field of research of OAM, both involving classical and quantum states of light. This chapter introduces some of the hallmark experiments within the subject, from which my experimental work reported in this thesis is inspired. The second chapter details the set up of the down conversion experiment, and the experimental techniques used to design a fully functioning quantum measurement system. Most importantly, this includes the holographic techniques used to measure the spatial states of the photon pairs. In addition to holographic measurements, a system to holographically auto-align the down-conversion experiment was developed. Due to the sensitive nature of the experiments presented, this automated system has been crucial to the success of all of the single photon experiments presented within this document. The experimental results are split into three separate categories. The first (Chapter 3) describes measurements investigating the Fourier relationship between OAM and angular position states, both at the classical and quantum levels. The following chapter (Chapter 4) consists of four experiments designed to quantify the degree of entanglement of states of OAM and angular position. This includes the first demonstration of the historic EPR (Einstein-Podolsky-Rosen) paradox for OAM and angle states, violation of a Bell-type inequality for arbitrary OAM states, and characterisation of the density matrices for a range of OAM state-spaces. The final chapter (Chapter 5) reports a new type of ghost imaging using down-converted photon pairs. In this experiment, we violate a Bell inequality within a ghost image, demonstrating the entangled nature of our system and contributing a new element to the long standing contention over quantum vs. classical features within ghost imaging. These experiments have seen a wide range of collaboration. The experimental work on the Fourier relation on single photons was carried out in collaboration with Dr. Anand Kumar Jha (University of Rochester). The work on ghost imaging was performed with collaboration with Prof. Monika Ritsch-Marte (Innsbruck Medical University), and the angular EPR paradox work was carried out in collaboration with Prof. Robert Boyd (Univ. of Rochester) and Prof. David Ireland (Univ. of Glasgow). The work I present here is experimental, however any theoretical developments are in a large part due to the support of Dr. Sonja Franke-Arnold and Prof. Steve Barnett (Univ. of Strathclyde).