This is a two-part thesis strung together by a common underlying theme—quantum correlations. We present some new characterizations and quantifications of quantum correlations and an application of one such correlation—entanglement—for quantum technology. In Part I of the thesis, we use a Rényi generalization of the quantum conditional mutual information (QCMI) to define and study new measures of quantum entanglement and quantum discord. In particular, using a quantity derived from a Rényi QCMI, we introduce: a) the geometric squashed entanglement, a faithful entanglement measure, which is a lower bound on the squashed entanglement and which reduces to the geometric measure of entanglement for pure quantum states, b) the surprisal of measurement recoverability, a discord-like measure, which is similarly a lower bound on the quantum discord. The surprisal of measurement recoverability enhances our understanding of quantum discord in terms of the ability to recover one share of a bipartite quantum system after it has been measured. In Part II, we discuss entanglement-enhanced quantum sensing. In particular, we consider optical interferometric sensors that use photon-number parity detection. Using the quantum and classical Cramér-Rao bounds (QCRB and CCRB) on phase precision as the figures of merit, we characterize a class of two-mode pure states for which photon-number parity measurement is optimal for phase estimation. These states turn out to be a subset of the class of path-symmetric states—a class for which photon-number counting-based measurements are known to be optimal. Further, we gauge the performance of the particular interferometry based on coherent light mixed with squeezed vacuum light and photon-number parity measurement. We show that photon-number parity is an optimal measurement for the above state in the sense that the detection scheme is capable of achieving the best phase precision offered by the state (given by its QCRB). The state by itself is also known to be capable of optimal phase precision for any state in linear interferometry for a given photon budget, called the Heisenberg limit. Thus, we demonstrate Heisenberg-limited phase estimation for the state with photon-number parity detection.
This is a two-part thesis strung together by a common underlying theme—quantum correlations. We present some new characterizations and quantifications of quantum correlations and an application of one such correlation—entanglement—for quantum technology. In Part I of the thesis, we use a Rényi generalization of the quantum conditional mutual information (QCMI) to define and study new measures of quantum entanglement and quantum discord. In particular, using a quantity derived from a Rényi QCMI, we introduce: a) the geometric squashed entanglement, a faithful entanglement measure, which is a lower bound on the squashed entanglement and which reduces to the geometric measure of entanglement for pure quantum states, b) the surprisal of measurement recoverability, a discord-like measure, which is similarly a lower bound on the quantum discord. The surprisal of measurement recoverability enhances our understanding of quantum discord in terms of the ability to recover one share of a bipartite quantum system after it has been measured. In Part II, we discuss entanglement-enhanced quantum sensing. In particular, we consider optical interferometric sensors that use photon-number parity detection. Using the quantum and classical Cramér-Rao bounds (QCRB and CCRB) on phase precision as the figures of merit, we characterize a class of two-mode pure states for which photon-number parity measurement is optimal for phase estimation. These states turn out to be a subset of the class of path-symmetric states—a class for which photon-number counting-based measurements are known to be optimal. Further, we gauge the performance of the particular interferometry based on coherent light mixed with squeezed vacuum light and photon-number parity measurement. We show that photon-number parity is an optimal measurement for the above state in the sense that the detection scheme is capable of achieving the best phase precision offered by the state (given by its QCRB). The state by itself is also known to be capable of optimal phase precision for any state in linear interferometry for a given photon budget, called the Heisenberg limit. Thus, we demonstrate Heisenberg-limited phase estimation for the state with photon-number parity detection.
One important problem in quantum optics is to resolve an extremely small change of phase shift. The complementarity between photon number and phase sets an ultimate limit, the so-called Heisenberg limit, on the phase measurement sensitivity. The precise phase estimation has many technological applications, such as optical gyroscopes, gravitational wave detection, quantum imaging and sensing. In this thesis I show that the utilization of the parity measurement in the optical interferometry is actually applicable to a wide range of quantum entangled input states. Comparison of the performance of the various quantum states then can be made within such a unified output measurement scheme. Based on such a universal detection scheme, we present a comparison of the phase sensitivity reduction for various quantum states of light in the presence of photon loss. I also provide a simple condition that could be used to check whether an arbitrary state can achieve the Heisenberg limit independently of the detection scheme. It implies that the fidelity between the two output states with zero phase and minimal detectable phase applied respectively should significantly different from unity as the minimal phase shift scaling as 1/N, whereas the average number of input photons N goes to infinity. Next I give several measures to characterize the which-way information in the interference experiment. We define a new distinguishability associated with the fidelity between two density matrices to measure the which-way information. We demonstrate that the changes of mutual entropy as well as the entanglement of formation of the whole system, i.e. the physical system plus the which-way detector can also be used to describe the which-way information. With such quantities, we show that as the fringe visibility of the interference pattern gets larger, the less which-way information is obtained. Finally, I show that coherent light coupled with photon number resolving detectors can provide a super-resolution much below the Rayleigh diffraction limit, with sensitivity no worse than shot-noise in terms of the detected photon power. This scheme would have applications to laser radar, given the difficulty in making entangled states of light, as well as their susceptibility to atmospheric absorption.
In this dissertation we begin with a brief introduction to quantum optics concentrating on the topics of the noise of quantum optical states, quantum estimation theory, quantum interferometry and the atom-field interaction. This background is necessary for understanding the discussions in later chapters. In particular, quantum interferometry, which is optical interferometry when the light source is a quantum mechanical state, plays a central role in this dissertation. In Chapter 2 we discuss the phase estimation sensitivity of quantum metrology when photon loss is present. In Chapter 3 we extend the discussion to include the phase fluctuation of the system caused by the environment. We model our metrological system with the Mach-Zehnder interferometer (MZI) and use a light field in the symmetric number-path entangled state as the source. In both chapters we use the parity operator as the detection scheme and show that it is optimal under pure dephasing. In Chapter 4 we discuss the application of quantum optical states in remote sensing and propose a new scheme for a quantum radar. Again, our scheme consists of a MZI and a coherent light source. It is shown that using only coherent states of light and quantum homodyne detection, super-resolving ranging and angle determination are achievable. Chapter 5 is devoted to the generation of a super-resolving single-photon number-path entangled state which may serve as a proof-of-principle prototype for quantum lithography. The repeated implementation of MZIs is shown to be able to remove photons coherently from both modes of a symmetric number-path entangled state with arbitrarily high photon number. Lastly, in Chapter 6 we introduce the phenomenon known as polarization self-rotation and discuss its potential in generating a squeezed vacuum state, which has a huge impact in quantum interferometry.
In the first part of this dissertation a framework for categorizing entropic measures of nonclassical correlations in bipartite quantum states is presented. The measures are based on the difference between a quantum entropic quantity and the corresponding classical quantity obtained from measurements on the two systems. Three types of entropic quantities are used, and three different measurement strategies are applied to these quantities. Many of the resulting measures of nonclassical correlations have been proposed previously. Properties of the various measures are explored, and results of evaluating the measures for two-qubit quantum states are presented. To demonstrate how these measures differ from entanglement we move to the set of Bell-diagonal states for two qubits, which can be depicted as a tetrahedron in three dimensions. We consider the level surfaces of entanglement and of the correlation measures from our framework for Bell-diagonal states. This provides a complete picture of the structure of entanglement and discord for this simple case and, in particular, of their nonanalytic behavior under decoherence. The pictorial approach also indicates how to show that all of the proposed correlation measures are neither convex nor concave. In the second part we look at two practical interferometric setups that use nonclassical states of light to enhance their performance. First we consider an interferometer powered by laser light (a coherent state) into one input port and ask the following question: what is the best state to inject into the second input port, given a constraint on the mean number of photons this state can carry, in order to optimize the interferometer's phase sensitivity? This question is the practical question for high-sensitivity interferometry. We answer the question by considering the quantum Cram\'er-Rao bound for such a setup. The answer is squeezed vacuum. Then we analyze the ultimate bounds on the phase sensitivity of an interferometer, given the constraint that the state input to the interferometer's initial 50:50 beam splitter B is a product state of the two input modes. Requiring a product state is a natural restriction: if one were allowed to input an arbitrary, entangled two-mode state ∣Ξ⟩ to the beam splitter, one could generally just as easily input the state B∣Ξ⟩ directly into the two modes after the beam splitter, thus rendering the beam splitter unnecessary. We find optimal states for a fixed photon number and for a fixed mean photon number. Our results indicate that entanglement is not a crucial resource for quantum-enhanced interferometry. Initially the analysis for both of these setups is performed for the idealized case of a lossless interferometer. Then the analysis is extended to the more realistic scenario where the interferometer suffers from photon losses.
This paper defines the fidelity of recovery of a tripartite quantum state on systems A,B, and C as a measure of how well one can recover the full state on all three systems if system A is lost and a recovery operation is performed on system C alone. The surprisal of the fidelity of recovery (its negative logarithm) is an information quantity which obeys nearly all of the properties of the conditional quantum mutual information I(A;B∣C), including non-negativity, monotonicity with respect to local operations, duality, invariance with respect to local isometries, a dimension bound, and continuity. We then define a (pseudo) entanglement measure based on this quantity, which we call the ``geometric squashed entanglement.'' We prove that the geometric squashed entanglement is a 1-LOCC monotone (i.e., monotone nonincreasing with respect to local operations and classical communication from Bob to Alice), that it vanishes if and only if the state on which it is evaluated is unentangled, and that it reduces to the geometric measure of entanglement if the state is pure. We also show that it is invariant with respect to local isometries, subadditive, continuous, and normalized on maximally entangled states. We next define the surprisal of measurement recoverability, which is an information quantity in the spirit of quantum discord, characterizing how well one can recover a share of a bipartite state if it is measured. We prove that this discordlike quantity satisfies several properties, including non-negativity, faithfulness on classical-quantum states, invariance with respect to local isometries, a dimension bound, and normalization on maximally entangled states. This quantity, combined with a recent breakthrough of Fawzi and Renner, makes it possible to characterize states with discord nearly equal to zero as being approximate fixed points of entanglement-breaking channels (equivalently, they are recoverable from the state of a measuring apparatus). Finally, we discuss a multipartite fidelity of recovery and several of its properties.
Quantum-enhanced interferometers utilize non-classical states of light in order to surpass the limitations imposed by classical physics on phase measurement sensitivity and resolution. We review key scientific developments in this growing field of research and derive fundamental metrology concepts, namely the Cram\'{e}r-Rao bound and the Fisher information, which are used to analyze the metrological performance of quantum states of light. We propose a supersensitive quantum interferometry protocol that can be amplified to the macroscopic realm (i.e. the mean number of photons of the probe state can reach approximately 100,000 photons) using contemporary techniques of spontaneous parametric down conversion. The parity measurement on the output field asymptotically saturates the quantum Cram\'{e}r-Rao bound, which scales like the Heisenberg limit. We uncover the role of photon statistics on phase sensitivity and rule out the necessity of mode entanglement for quantum-enhanced interferometry. Based on these insights we outline a practical metrology technique (independent of mode entanglement) that measures a phase delay of a single-mode anti-squeezing operation. This scheme can also be scaled macroscopically using contemporary techniques and is shown to significantly surpass the shot-noise limit (SNL) in the presence of realistic losses. Finally, the physical resources that enable quantum-enhanced interferometry is studied by analyzing the quantum Fisher information (QFI) using the first quantization and the second quantization formalisms of quantum mechanics. It is shown that increasing the intra-mode correlations of an interferometer (as quantified by the second order Glauber coherence function) can be conducive to attaining a quantum advantage in phase estimation; whereas, introducing mode entanglement can reduce phase sensitivity. Using the first quantization description, we derive a formula for the QFI that shows explicitly how the Heisenberg scaling term depends on particle entanglement.
The squashed entanglement quantifies the amount of entanglement in a bipartite quantum state, and it satisfies all of the axioms desired for an entanglement measure. The quantum discord is a measure of quantum correlations that are different from those due to entanglement. What these two measures have in common is that they are both based upon the conditional quantum mutual information. In Berta et al (2015 J. Math. Phys. 56 022205), we recently proposed Rényi generalizations of the conditional quantum mutual information of a tripartite state on ABC (with C being the conditioning system), which were shown to satisfy some properties that hold for the original quantity, such as non-negativity, duality, and monotonicity with respect to local operations on the system B (with it being left open to show that the Rényi quantity is monotone with respect to local operations on system A). Here we define a Rényi squashed entanglement and a Rényi quantum discord based on a Rényi conditional quantum mutual information and investigate these quantities in detail. Taking as a conjecture that the Rényi conditional quantum mutual information is monotone with respect to local operations on both systems A and B, we prove that the Rényi squashed entanglement and the Rényi quantum discord satisfy many of the properties of the respective original von Neumann entropy based quantities. In our prior work (Berta et al 2015 Phys. Rev. A 91 022333), we also detailed a procedure to obtain Rényi generalizations of any quantum information measure that is equal to a linear combination of von Neumann entropies with coefficients chosen from the set . Here, we extend this procedure to include differences of relative entropies. Using the extended procedure and a conjectured monotonicity of the Rényi generalizations in the Rényi parameter, we discuss potential remainder terms for well known inequalities such as monotonicity of the relative entropy, joint convexity of the relative entropy, and the Holevo bound.