Matter-wave interferometers are sensitive probes of low energy physics and have been used for precise tests of gravity and quantum mechanics. These applications would benefit from interfering particles of higher mass, but observing the interference of a large particle is challenging due to the need to control its initial state and to avoid decoherence. Here we propose to demonstrate matter-wave interference of a microparticle with an embedded rare-earth ion. Optical transitions of the rare-earth ion will impart momentum to the microparticle's center of mass. The use of a time-symmetric interferometer geometry and a rare-earth ion state with angular momentum $J = 1/2$ will eliminate sensitivity to the initial conditions of the microparticle. We show that the rates of all relevant external decoherence mechanisms either decrease or remain constant as the microparticle mass is increased, allowing decoherence to be avoided by using sufficiently large particles. An apparatus at moderate vacuum levels will support microparticle interferometry with up to $10^3$ photons per beam splitter and millisecond coherence time. This demonstration will establish microparticle interferometry as a new platform for quantum sensing, improving searches for minimal modifications of quantum mechanics by up to three orders of magnitude in the near term and laying the foundation for future gravitational tests.
Matter-wave interferometers are sensitive probes of low energy physics and have been used for precise tests of gravity and quantum mechanics. These applications would benefit from interfering particles of higher mass, but observing the interference of a large particle is challenging due to the need to control its initial state and to avoid decoherence. Here we propose to demonstrate matter-wave interference of a microparticle with an embedded rare-earth ion. Optical transitions of the rare-earth ion will impart momentum to the microparticle's center of mass. The use of a time-symmetric interferometer geometry and a rare-earth ion state with angular momentum J=1/2 will eliminate sensitivity to the initial conditions of the microparticle. We show that the rates of all relevant external decoherence mechanisms either decrease or remain constant as the microparticle mass is increased, allowing decoherence to be avoided by using sufficiently large particles. An apparatus at moderate vacuum levels will support microparticle interferometry with up to 103 photons per beam splitter and millisecond coherence time. This demonstration will establish microparticle interferometry as a new platform for quantum sensing, improving searches for minimal modifications of quantum mechanics by up to three orders of magnitude in the near term and laying the foundation for future gravitational tests.
The wave-particle duality is a key concept of quantum physics and extending quantum superpositions to bodies of increasing mass and complexity has become a key goal to numerous research groups. Such experiments are motivated by the desire to probe and better understand the quantum-classical interface in advanced tests of spontaneous or gravity-induced wave function collapse and in the search for non-linear modifications of quantum theory. High mass interferometry has been proposed to serve in the search for light dark matter via weak recoil decoherence as well as in tests of the weak equivalence principle by comparing a large variety of quantum systems with very distinct internal composition, excitation, mass, shape or angular momentum. Here we discuss the experimental state of the art in high-mass matter-wave interferometry, as well as new perspectives from cluster and nanoparticle physics to push quantum superpositions by 3 to 4 orders of magnitude in mass or up to 6 orders of magnitude in 'macroscopicity'. We discuss different near-field interferometer configurations that shall become useful in near-future demonstrations of quantum phenomena with objects as diverse as proteins, metal clusters and dielectric nanoparticles.
Creating quantum superposition states of bodies with increasing mass and complexity is an exciting and important challenge. Demonstrating such superpositions is vital for understanding how classical observations arise from the underlying quantum physics. Here, we discuss how recent progress in macromolecule interferometry can be combined with the state of the art in cluster physics to push the mass record for matter-wave interference with wide state separation by 3 to 4 orders of magnitude. We show how near-field interferometers in different configurations can achieve this goal for a wide range of particle materials with strongly varying properties. This universality will become important in advanced tests of wave function collapse and of other modifications of quantum mechanics, as well as in the search for light dark matter and in tests of gravity with composite quantum systems.
Matter-wave interferometry is a striking quantum phenomenon that differs fundamentally from classical mechanics. In the quantum regime, matter behaves like a wave and can exist in spatial superpositions, allowing a single quantum object to move along multiple trajectories simultaneously. Similar to optical interferometers, such quantum matter systems act as interferometers themselves, with the differential phase that encodes information about external forces experienced during their evolution. This makes matter-wave interferometry a powerful platform for quantum sensing across various applications: (i) One of the most direct applications is precision measurement. Atomic interferometers can measure local acceleration and have already been implemented in devices such as accelerometers, seismometers, gravimeters, and gradiometers. (ii) Atomic interferometers are proposed as complementary tools for future gravitational-wave observatories, including ongoing projects MIGA, MAGIS-100, AION and ZAIGA. (iii) Matter-wave interferometry also offers a promising platform for probing quantum aspects of gravity. Numerous tabletop proposals aim to test quantum gravity models, investigate collapse mechanisms, study gravity-induced decoherence, and search for gravity-mediated quantum entanglement. The Stern-Gerlach interferometer (SGI) is a type of matter-wave interferometer that manipulates spatial superpositions using magnetic-field gradients. The witness of an SGI can be designed via its spin, enabling more precise measurements of the differential phase. Recent developments in atomic chip technology have enabled the generation of highly controlled magnetic fields on compact platforms, allowing for precise manipulation of spin states and making SGIs experimentally realizable. Robustness is a critical challenge for matter-wave interferometers. In real experiments, various sources of classical noises arise from mechanical vibrations, seismic motions, inertial forces, tidal forces, magnetic field fluctuations and so on. These noises can disturb the spin and spatial degrees of freedom of the test mass, resulting in witness loss of the interferometer. While spin decoherence is relatively well understood and can be formulated by the Bloch-Redfield master equation, the impact on spatial degrees of freedom still requires systematic investigation. This thesis therefore aims to explore witness loss in an SGI induced by stochastic noises acting on spatial degrees of freedom. As investigated by this thesis, the witness gets lost via several mechanisms: (i) Dephasing. The spatial phase is fluctuated by stochastic noise, resulting in a random phase factor eiδϕ, whose ensemble average contributes a decay factor e−Γ to the spin density matrix and leads to a loss of witness. As is demonstrated by the thesis, this decay factor is a linear response to the external noise, with a transfer function as the Fourier transform of the unperturbed classical trajectories. (ii) Humpty-Dumpty problem. The classical trajectories are also disturbed by stochastic noise, resulting in a non-closure problem of the interferometer, known as the Humpty-Dumpty problem. The resulting witness loss is usually characterized by the contrast of the final states ⟨ψ1|ψ2⟩, which equals the phase-space distance |α1 − α2|2 when the test mass is in coherent states. (iii) Position localization decoherence. Due to the randomness of the noise, the spatial wavefunction of the test mass is thus also stochastic, of which the ensemble average experiences decoherence characterized by the power spectrum density of external noise. However, as illustrated by this thesis, this type of decoherence does not affect spin-based witnesses in most practical scenarios. The general theoretical framework is mainly constructed in chapter 3 of this thesis. The subsequent chapters analyze several representative noise sources: (i) Gravitational and electrostatic noise. Molecules in the surrounding gas move randomly due to thermal motion, generating stochastic gravitational accelerations and electrostatic forces that can be expanded in multipole series. Since the random motion follows Maxwell’s distribution and approximately has a cylindrical symmetry, the resulting noise power spectrum density takes the form of Bessel functions. (ii) Inertial acceleration noise. The mechanical support of the experimental apparatus is always fluctuated by vibrational noise, resulting in random inertial force on the test mass. In practice, dephasing can be mitigated through destructive interference by introducing appropriate coupling between different directional components. (iii) Inertial torsion noise. In suspended experiments, the experimental apparatus is fluctuated by torsional noise, leading to another inertial noise on the test mass. The power spectrum density of the inertial torsion noise is formulated by the selfconvolution of the original noise, resulting in the peak frequencies that are doubled. Taken together, these analyses build a comprehensive picture of how stochastic noise affects the spatial dynamics of an SGI and leads to the loss of spin-based witnesses. Future work may include more realistic noise sources such as magnetic noise and trap-potential noise. These insights will be valuable for future experimental implementations, particularly in precision sensing for quantum gravity, where preserving coherence and maintaining reliable witness signals are essential.
Abstract The quantum superposition principle is a fundamental concept of physics 1 and the basis of numerous quantum technologies 2,3 . Yet, it is still often regarded counterintuitive because we do not observe its key features on the macroscopic scales of our daily lives. It is, therefore, interesting to ask how quantum properties persist or change as we increase the size and complexity of objects 4 . A model test for this question can be realized by matter-wave interferometry, in which the motion of individual massive particles becomes delocalized and needs to be described by a wave function that spans regions far larger than the particle itself 5 . Over the years, this has been explored with a series of objects of increasing mass and complexity 6–9 and a growing community aims at pushing this to ever larger limits. Here we present an experimental platform that extends matter-wave interference to large metal clusters, a qualitatively new material class for quantum experiments. We specifically demonstrate quantum interference of sodium nanoparticles, which can each contain more than 7,000 atoms at masses greater than 170,000 Da. They propagate in a Schrödinger cat state with a macroscopicity 10 of μ = 15.5, surpassing previous experiments 5,9,11 by an order of magnitude.
Matter-wave interferometry with nanoparticles will enable the development of quantum sensors capable of probing ultraweak fields with unprecedented applications for fundamental physics. The high sensitivity of such devices, however. makes them susceptible to several noise and decoherence sources and, as such, can operate only when sufficient isolation from the environment is achieved. It is thus imperative to model and characterize the interaction of nanoparticles with the environment and to estimate its deleterious effects. This paper will aim to study the decoherence of the matter-wave interferometer due to dipole-dipole interactions, which is one of the unavoidable channels for decoherence, even for a neutral micro-crystal. We will use the scattering model for decoherence, characterized by the differential cross section, in order to obtain simple expressions for the decoherence rate due to dipole-dipole interactions in the short- and long-wavelength limits that can be readily applied to estimate the available coherence time. We will conclude by applying the formulas we obtained to estimate the dipole-dipole decoherence rate for the quantum gravity-induced entanglement of masses protocol and discuss if the effects should be mitigated.
Recent progress and future prospects of matter-wave interferometry with complex organic molecules and inorganic clusters are reviewed. Three variants of a near-field interference effect, based on diffraction by material nanostructures, at optical phase gratings, and at ionizing laser fields are considered. The theoretical concepts underlying these experiments and the experimental challenges are discussed. This includes optimizing interferometer designs as well as understanding the role of decoherence. The high sensitivity of matter-wave interference experiments to external perturbations is demonstrated to be useful for accurately measuring internal properties of delocalized nanoparticles. The prospects for probing the quantum superposition principle are investigated in the limit of high particle mass and complexity.