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Optical and Quantum Sensing and Precision Metrology II

A roadmap to matter-wave interferometry with complex things and applications in quantum sensing

Markus Arndt

Published Mar 9, 2022• 0 citations
Publisher

Abstract

The wave-particle duality is a key concept of quantum physics and extending quantum superpositions to bodies of increasing mass and complexity has become a key goal to numerous research groups. Such experiments are motivated by the desire to probe and better understand the quantum-classical interface in advanced tests of spontaneous or gravity-induced wave function collapse and in the search for non-linear modifications of quantum theory. High mass interferometry has been proposed to serve in the search for light dark matter via weak recoil decoherence as well as in tests of the weak equivalence principle by comparing a large variety of quantum systems with very distinct internal composition, excitation, mass, shape or angular momentum. Here we discuss the experimental state of the art in high-mass matter-wave interferometry, as well as new perspectives from cluster and nanoparticle physics to push quantum superpositions by 3 to 4 orders of magnitude in mass or up to 6 orders of magnitude in 'macroscopicity'. We discuss different near-field interferometer configurations that shall become useful in near-future demonstrations of quantum phenomena with objects as diverse as proteins, metal clusters and dielectric nanoparticles.

DOI
10.1117/12.2616793

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Abstract The quantum superposition principle is a fundamental concept of physics 1 and the basis of numerous quantum technologies 2,3 . Yet, it is still often regarded counterintuitive because we do not observe its key features on the macroscopic scales of our daily lives. It is, therefore, interesting to ask how quantum properties persist or change as we increase the size and complexity of objects 4 . A model test for this question can be realized by matter-wave interferometry, in which the motion of individual massive particles becomes delocalized and needs to be described by a wave function that spans regions far larger than the particle itself 5 . Over the years, this has been explored with a series of objects of increasing mass and complexity 6–9 and a growing community aims at pushing this to ever larger limits. Here we present an experimental platform that extends matter-wave interference to large metal clusters, a qualitatively new material class for quantum experiments. We specifically demonstrate quantum interference of sodium nanoparticles, which can each contain more than 7,000 atoms at masses greater than 170,000 Da. They propagate in a Schrödinger cat state with a macroscopicity 10 of μ = 15.5, surpassing previous experiments 5,9,11 by an order of magnitude.
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We discuss modern developments in quantum optics with organic molecules, clusters and nanoparticles -- in particular recent realizations of near-field matter-wave interferometry. A unified theoretical description in phase space allows us to describe quantum interferometry in position space and in the time domain on an equal footing. In order to establish matter-wave interferometers as a universal tool, which can accept and address a variety of nanoparticles, we elaborate on new quantum optical elements, such as diffraction gratings made of matter and light, as well as their absorptive and dispersive interaction with complex materials. We present Talbot-Lau interferometry (TLI), the Kapitza-Dirac-Talbot-Lau interferometer (KDTLI) and interferometry with pulsed optical gratings (OTIMA) as the most advanced devices to study the quantum wave nature of composite matter. These experiments define the current mass and complexity record in interferometric explorations of quantum macroscopicity and they open new avenues to quantum assisted metrology with applications in physical chemistry and biomolecular physics.
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Designing experiments which delocalize ever more complex and more massive particles requires a quantitative assessment of new interferometer configurations.Here, we introduce a figure of merit which quantifies the difference between a genuine quantum interference pattern and a classical shadow and use it to compare a number of near-field interferometer schemes.This allows us to identify the most promising setups for future tests of the quantum superposition principle, and to discuss the perspectives of interferometry with complex molecules and clusters.