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AVS Quantum Science

A roadmap for universal high-mass matter-wave interferometry

Filip Kiałka, Yaakov Y. Fein, Sebastian Pedalino, Stefan Gerlich, Markus Arndt

Published Apr 27, 2022• 19 citations
Publisher

Abstract

Creating quantum superposition states of bodies with increasing mass and complexity is an exciting and important challenge. Demonstrating such superpositions is vital for understanding how classical observations arise from the underlying quantum physics. Here, we discuss how recent progress in macromolecule interferometry can be combined with the state of the art in cluster physics to push the mass record for matter-wave interference with wide state separation by 3 to 4 orders of magnitude. We show how near-field interferometers in different configurations can achieve this goal for a wide range of particle materials with strongly varying properties. This universality will become important in advanced tests of wave function collapse and of other modifications of quantum mechanics, as well as in the search for light dark matter and in tests of gravity with composite quantum systems.

DOI
10.1116/5.0080940

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Creating quantum superposition states of bodies with increasing mass and complexity is an exciting and important challenge. Demonstrating such superpositions is vital for understanding how classical observations arise from the underlying quantum physics. Here, we discuss how recent progress in macromolecule interferometry can be combined with the state of the art in cluster physics to push the mass record for matter-wave interference with wide state separation by 3 to 4 orders of magnitude. We show how near-field interferometers in different configurations can achieve this goal for a wide range of particle materials with strongly varying properties. This universality will become important in advanced tests of wave function collapse and of other modifications of quantum mechanics, as well as in the search for light dark matter and in tests of gravity with composite quantum systems.
The wave-particle duality is a key concept of quantum physics and extending quantum superpositions to bodies of increasing mass and complexity has become a key goal to numerous research groups. Such experiments are motivated by the desire to probe and better understand the quantum-classical interface in advanced tests of spontaneous or gravity-induced wave function collapse and in the search for non-linear modifications of quantum theory. High mass interferometry has been proposed to serve in the search for light dark matter via weak recoil decoherence as well as in tests of the weak equivalence principle by comparing a large variety of quantum systems with very distinct internal composition, excitation, mass, shape or angular momentum. Here we discuss the experimental state of the art in high-mass matter-wave interferometry, as well as new perspectives from cluster and nanoparticle physics to push quantum superpositions by 3 to 4 orders of magnitude in mass or up to 6 orders of magnitude in 'macroscopicity'. We discuss different near-field interferometer configurations that shall become useful in near-future demonstrations of quantum phenomena with objects as diverse as proteins, metal clusters and dielectric nanoparticles.
Abstract The quantum superposition principle is a fundamental concept of physics 1 and the basis of numerous quantum technologies 2,3 . Yet, it is still often regarded counterintuitive because we do not observe its key features on the macroscopic scales of our daily lives. It is, therefore, interesting to ask how quantum properties persist or change as we increase the size and complexity of objects 4 . A model test for this question can be realized by matter-wave interferometry, in which the motion of individual massive particles becomes delocalized and needs to be described by a wave function that spans regions far larger than the particle itself 5 . Over the years, this has been explored with a series of objects of increasing mass and complexity 6–9 and a growing community aims at pushing this to ever larger limits. Here we present an experimental platform that extends matter-wave interference to large metal clusters, a qualitatively new material class for quantum experiments. We specifically demonstrate quantum interference of sodium nanoparticles, which can each contain more than 7,000 atoms at masses greater than 170,000 Da. They propagate in a Schrödinger cat state with a macroscopicity 10 of μ = 15.5, surpassing previous experiments 5,9,11 by an order of magnitude.
Designing experiments which delocalize ever more complex and more massive particles requires a quantitative assessment of new interferometer configurations.Here, we introduce a figure of merit which quantifies the difference between a genuine quantum interference pattern and a classical shadow and use it to compare a number of near-field interferometer schemes.This allows us to identify the most promising setups for future tests of the quantum superposition principle, and to discuss the perspectives of interferometry with complex molecules and clusters.
Recent progress and future prospects of matter-wave interferometry with complex organic molecules and inorganic clusters are reviewed. Three variants of a near-field interference effect, based on diffraction by material nanostructures, at optical phase gratings, and at ionizing laser fields are considered. The theoretical concepts underlying these experiments and the experimental challenges are discussed. This includes optimizing interferometer designs as well as understanding the role of decoherence. The high sensitivity of matter-wave interference experiments to external perturbations is demonstrated to be useful for accurately measuring internal properties of delocalized nanoparticles. The prospects for probing the quantum superposition principle are investigated in the limit of high particle mass and complexity.
Summary. — This chapter reviews recent experiments on matter wave interferometry with large molecules. Starting from an elementary introduction to matter wave physics we discuss far-field diffraction and near-field interferometry with thermally excited many-body systems. We describe the constraints imposed by decoherence and dephasing effects, and present an outlook to the future challenges in macromolecule and cluster interferometry. PACS 03.75.-b – Matter waves. 1. – Historical introduction and overview The year 1923 is generally considered as the year of birth of matter wave physics. It is the year when Louis de Broglie proposed the idea that each material particle is accompanied by an oscillatory phenomenon [1]. De Broglie based his hypothesis on two discoveries: the energy-frequency equivalence for photons, E = ¯hω, and the energy-mass equivalence for matter, E = mc 2. While the first relation had already been central to Planck’s explanation of the black body spectrum [2] and to Einstein’s analysis of the photo effect [3], the latter was a consequence of Einstein’s theory of special relativity.
We discuss modern developments in quantum optics with organic molecules, clusters and nanoparticles -- in particular recent realizations of near-field matter-wave interferometry. A unified theoretical description in phase space allows us to describe quantum interferometry in position space and in the time domain on an equal footing. In order to establish matter-wave interferometers as a universal tool, which can accept and address a variety of nanoparticles, we elaborate on new quantum optical elements, such as diffraction gratings made of matter and light, as well as their absorptive and dispersive interaction with complex materials. We present Talbot-Lau interferometry (TLI), the Kapitza-Dirac-Talbot-Lau interferometer (KDTLI) and interferometry with pulsed optical gratings (OTIMA) as the most advanced devices to study the quantum wave nature of composite matter. These experiments define the current mass and complexity record in interferometric explorations of quantum macroscopicity and they open new avenues to quantum assisted metrology with applications in physical chemistry and biomolecular physics.