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arXiv:2609.07454

High-purity fluorescence photon bundle emission from two separate emitters

Zhicai Chen, Jun Xu, Deyi Kong, Xiangming Hu, Fei Wang

quant-phSubmitted Sep 7, 2026• Announced Sep 8, 2026• 0 citations
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Abstract

We propose a scheme for generating high-purity fluorescence two-photon bundles from two spatially separate two-level emitters, whose correlated excitation is mediated by a strongly driven auxiliary emitter. Unlike bosonic-mode-based approaches, the finite excitation space of the two target emitters intrinsically excludes higher-excitation manifolds, and thus eliminates impurity photons associated with undesired higher-excitation states. We further analytically characterize the residual population of off-resonant single-excitation states and show that suppressing the corresponding leakage improves photon bundle purity. Our scheme offers a feasible pathway for constructing high-purity quantum light sources with promising applications in quantum information processing.

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10 pages, 8 figures

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We propose a scheme for generating high-purity fluorescence two-photon bundles from two spatially separate two-level emitters, whose correlated excitation is mediated by a strongly driven auxiliary emitter. Unlike bosonic-mode-based approaches, the finite excitation space of the two target emitters intrinsically excludes higher-excitation manifolds, and thus eliminates impurity photons associated with undesired higher-excitation states. We further analytically characterize the residual population of off-resonant single-excitation states and show that suppressing the corresponding leakage improves photon bundle purity. Our scheme offers a feasible pathway for constructing high-purity quantum light sources with promising applications in quantum information processing.
We propose a component-selective scheme for improving two-photon sources in a cavity-coupled two-atom system, where a single cavity mode interacts with two two-level atoms driven by phase-controlled classical fields of the same frequency. By controlling the atomic detunings and driving phase, the system can be tailored toward optimized cavity-field two-photon blockade or strongly correlated fluorescence photon-pair emission. When the two-cavity-photon component is enhanced, the cavity field exhibits optimized two-photon blockade with simultaneous suppression of unwanted one- and three-photon components at a comparable two-photon population. In another parameter regime, strongly correlated fluorescence photon pairs can also be generated from the two atoms by selecting the double-atomic-excitation component in the same two-excitation manifold. This approach provides a route toward high-quality and versatile two-photon sources, with potential applications in few-photon quantum optics and quantum information processing.
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High-purity and bright single-photon sources are important for quantum information processing and precision measurement. We propose a collectively enhanced universal photon-blockade scheme in a multi-emitter two-photon Tavis--Cummings system. Independent coherent drives of the cavity and collective emitter enable destructive interference between two-photon excitation pathways, while collective coupling supplies level anharmonicity. Full-quantum master-equation simulations, the Holstein--Primakoff approximation, and a non-Hermitian probability-amplitude analysis yield the optimal conditions: cavity resonance together with phase and amplitude matching. Compared with a purely collective blockade, the proposed scheme lowers g(2)(0)g^{(2)}(0)g(2)(0), and essentially preserves the single-photon population. As the emitter number NNN increases, the optimal point remains at Δc=0Δ_c=0Δc​=0, while the minimum correlation follows gmin⁡(2)(0)∝N−2g_{\min}^{(2)}(0)\propto N^{-2}gmin(2)​(0)∝N−2. By contrast, unconventional photon blockade shifts away from resonance as NNN increases, limiting its purity improvement and brightness. In the weak-drive regime, universal blockade obeys g(2)(0)∝εa2g^{(2)}(0)\propto\varepsilon_a^2g(2)(0)∝εa2​, owing to a higher-order bypass through the three-excitation manifold. The drive strength therefore provides an additional purity--brightness control, although the interference mechanism makes the scheme more sensitive to dissipation-rate mismatch. Our results establish a scalable route to bright, high-purity, and tunable single-photon emission in multi-emitter cavity-QED systems.
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