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arXiv:2606.31775 · Nanoscale

Energy–time entanglement from a monolithically integrated quantum dot on silicon

Marcel Hohn, Imad Limame, Peter Ludewig, Chirag C. Palekar, Aris Koulas‐Simos, Kerstin Volz, Stephan Reitzenstein

Published Jan 1, 2026• 0 citations
arXivHTMLPDF

Abstract

Scalable quantum photonic technologies require deterministic sources of entangled photons that are compatible with established semiconductor manufacturing platforms. While self-assembled III-V semiconductor quantum dots are among the most promising sources of on-demand entanglement generation, their integration with silicon-based architectures remains a central challenge. Here, we demonstrate energy-time entanglement from a single InGaAs/GaAs quantum dot monolithically grown on a silicon substrate. Under resonant two-photon excitation, we achieve coherent control of the biexciton-exciton cascade, evidenced by the formation of dressed-states and Rabi oscillations. Using a four-channel Franson interferometer, we observe phase-dependent two-photon interference with visibilities up to (64.0 ± 7.0)% for a 80 ps integration window (and (49.4 ± 1.9)% for a 1600 ps window), approaching the threshold for Bell inequality violation at short timescales. Despite these constraints, the observation of Franson interference establishes monolithic III-V-on-silicon quantum dots as viable sources of energy-time entangled photons. These results represent a crucial step toward fully integrated, silicon-substrate-compatible quantum photonic circuits for large-scale quantum communication and information processing.

DOI
10.1039/d6nr02565j

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Energy-time (E-T) entanglement is widely employed in long-distance quantum entanglement distribution due to its strong robustness against transmission fluctuations. In this Letter, we report what we believe to be the first silicon monolithically integrated E-T entanglement system, which integrates the photon sources, wavelength demultiplexers, and Franson interferometers on a single chip. Also, by utilizing low-loss multimode waveguides in Franson interferometers, we measured an on-chip quantum interference visibility of 99.66% (±0.47%), to our knowledge one of the highest values for integrated E-T entanglement systems reported to date. The quantum interference after 1- and 5-km fiber propagation shows visibilities of 96.72% (±0.78%) and 97.46% (±1.23%), respectively. These results demonstrate the potential of using silicon monolithic integration for advance E-T entanglement-based quantum communication networks.
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Entanglement is a major resource in advanced quantum technology, where it can enable secure exchange of information over large distances. Energy-time entanglement is particularly attractive for its beneficial robustness in fiber-based quantum communication and can be demonstrated in the Franson interferometer. We report on Franson-type interference from a resonantly driven biexciton cascade under continuous wave excitation. Our measurements yield a maximum visibility of (73 ±\pm± 2)% surpassing the limit of violation of Bell's inequality (70.7%) by more than one standard deviation. Despite being unable to satisfy a loophole free violation, our work demonstrates promising results concerning future works on such a system. Furthermore, our systematical studies on the impact of driving strength indicate that dephasing mechanisms and deviations from the cascaded emission have major impact on the degree of the measured energy-time entanglement.
The strong confinement of semiconductor excitons in a quantum dot gives rise to atomlike behavior. The full benefit of such a structure is best observed in resonant excitation where the excited state can be deterministically populated and coherently manipulated. Because of the large refractive index and device geometry it remains challenging to observe resonantly excited emission that is free from laser scattering in III/V self-assembled quantum dots. Here we exploit the biexciton binding energy to create an extremely clean single photon source via two-photon resonant excitation of an InAs/GaAs quantum dot. We observe complete suppression of the excitation laser and multiphoton emissions. Additionally, we perform full coherent control of the ground-biexciton state qubit and observe an extended coherence time using an all-optical echo technique. The deterministic coherent photon pair creation makes this system suitable for the generation of time-bin entanglement and experiments on the interaction of photons from dissimilar sources.
An integrated source of time-energy entangled photons is demonstrated through resonantly enhanced spontaneous four-wave mixing in a silicon micro-ring resonator. A Franson type set-up is employed to show the quantum interference between photon pairs with a visibility exceeding 90% and a violation of the Bell's inequality by more than 10 standard deviations. The high spectral brightness and the extremely small footprint of our source make it suitable for the development of quantum information protocols integrated on chip.
The biexciton cascade process in self-assembled quantum dots (QDs) provides an ideal system for realizing deterministic entangled photon-pair sources, which are essential to quantum information science. The entangled photon pairs have recently been generated in experiments after eliminating the fine-structure splitting (FSS) of excitons using a number of different methods. Thus far, however, QD-based sources of entangled photons have not been scalable because the wavelengths of QDs differ from dot to dot. Here, we propose a wavelength-tunable entangled photon emitter mounted on a three-dimensional stressor, in which the FSS and exciton energy can be tuned independently, thereby enabling photon entanglement between dissimilar QDs. We confirm these results via atomistic pseudopotential calculations. This provides a first step towards future realization of scalable entangled photon generators for quantum information applications.