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arXiv:2512.02207

Uncertainty Principle and Angular Momentum Generation in Microscopic Fission Models

G. Scamps, A. Guilleux, D. Regnier, A. Bernard

nucl-thnucl-exquant-phSubmitted Dec 1, 2025• Announced Dec 3, 2025• Revised Jul 27, 2026 (v2)
v1 · Dec 1, 2025v2 · Jul 27, 2026
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Abstract

The generation of angular momentum (intrinsic spin) in fission fragments has recently attracted renewed attention. While several microscopic approaches reproduce the spin distribution qualitatively using projection techniques, the physical origin of the fragments' angular momentum in density functional theory remains unclear. In this work, we investigate the mechanisms responsible for the spin distribution of fission fragments within a microscopic TDDFT framework. We compare spin distributions obtained from projection operators with those predicted by a simple expression derived from the uncertainty relation between angle and angular momentum, where angular fluctuations are estimated using a Monte Carlo sampling of nucleon positions. We find that a large portion of the spin distribution obtained from projection methods can be explained by the uncertainty principle. Our results thus show that, within microscopic approaches, the spin of fission fragments originates primarily from quantum uncertainty associated with their orientation angle with respect to the fission axis, mainly due to quadrupole deformation and, to a lesser extent, octupole deformation.

Comments
10 pages, 6 figures

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The generation of angular momentum (intrinsic spin) in fission fragments has recently attracted renewed attention. While several microscopic approaches reproduce the spin distribution qualitatively using projection techniques, the physical origin of the fragments' angular momentum in density functional theory remains unclear. In this work, we investigate the mechanisms responsible for the spin distribution of fission fragments within a microscopic TDDFT framework. We compare spin distributions obtained from projection operators with those predicted by a simple expression derived from the uncertainty relation between angle and angular momentum, where angular fluctuations are estimated using a Monte Carlo sampling of nucleon positions. We find that a large portion of the spin distribution obtained from projection methods can be explained by the uncertainty principle. Our results thus show that, within microscopic approaches, the spin of fission fragments originates primarily from quantum uncertainty associated with their orientation angle with respect to the fission axis, mainly due to quadrupole deformation and, to a lesser extent, octupole deformation.
Nuclear time-dependent density functional theory is used to investigate spin generation and entanglement of fission fragments in spontaneous fission of ^{252}Cf, incorporating both axial and nonaxial deformations. Axially symmetric fission trajectories enforce strict constraints: counterrotation (twisting mode) along the fission axis and equiprobable bending and wriggling modes perpendicular to it. Nonaxial modes broaden the distributions of fission fragment spin projection on the fission axis, and allow for axial (tilting) collective rotations, which are forbidden on axially symmetric trajectories. Mutual information analysis reveals that axial-symmetry breaking reduces spin-spin correlations along the fission axis of symmetric cases, while perpendicular correlations remain more resilient. The effect of triaxial degrees of freedom on the opening angle distribution between the spins of the fission fragments is analyzed.
Nuclear time-dependent density functional theory is used to investigate spin generation and entanglement of fission fragments in spontaneous fission of 252^{252}252Cf, incorporating both axial and non-axial deformations. Axially symmetric fission trajectories enforce strict constraints: counter rotation (twisting mode) along the fission axis and equiprobable bending/wriggling modes perpendicular to it. Non-axial modes broaden the distributions of fission fragment spin projection on the fission axis, and allow for axial (tilting) collective rotations, which are forbidden on axially symmetric trajectories. Mutual information analysis reveals that axial-symmetry breaking reduces spin-spin correlations along the fission axis of symmetric cases, while perpendicular correlations remain more resilient. The effect of triaxial degrees of freedom on the opening angle distribution between the spins of the fission fragments is analyzed.
The uncertainty principle places fundamental limits on the accuracy with which we are able to measure the values of different physical quantities (Heisenberg 1949 The Physical Principles of the Quantum Theory (New York: Dover); Robertson 1929 Phys. Rev. 34 127). This has profound effects not only on the microscopic but also on the macroscopic level of physical systems. The most familiar form of the uncertainty principle relates the uncertainties in position and linear momentum. Other manifestations include those relating uncertainty in energy to uncertainty in time duration, phase of an electromagnetic field to photon number and angular position to angular momentum (Vaccaro and Pegg 1990 J. Mod. Opt. 37 17; Barnett and Pegg 1990 Phys. Rev. A 41 3427). In this paper, we report the first observation of the last of these uncertainty relations and derive the associated states that satisfy the equality in the uncertainty relation. We confirm the form of these states by detailed measurement of the angular momentum of a light beam after passage through an appropriate angular aperture. The angular uncertainty principle applies to all physical systems and is particularly important for systems with cylindrical symmetry.
A comparative analysis of experiments devoted to studying, in the fission process, ( n,fn,fn,f ) angular correlations, on one hand, and ( n,nn,nn,n ) and ( n,nfn,nfn,nf ) angular correlations, on the other hand, is performed on the basis of the model proposed earlier for describing muon conversion in fragments originating from the prompt fission of 238{}^{238}238 U nuclei that is induced by negatively charged muons. It is shown that each of these experiments may provide information that does not depend on the results of the other experiments and which is complementary to them. Historically, the situation resembles the Einstein–Podolsky–Rosen (EPR) paradox. An experimental verification of the theoretical relation between the alignment and polarization of fragment spins in the CORA experiment is of crucial importance.
Nuclear fission presents a unique example of quantum entanglement in strongly interacting many-body systems. A heavy nucleus can split into hundreds of combinations of two complementary fragments in the fission process. The entanglement of fragment wave functions is persistent even after separation and impacts the partition of particles and energies between fragments. Based on microscopic dynamical calculations of the fission of 240 Pu, this work finds that dynamical quantum entanglement is indispensable in the appearance of sawtooth distributions of average excitation energies of fragments and thus neutron multiplicities, but not in average neutron excess of fragments. Both sawtooth slopes from particle-number projections are found to be steep – a feature which can be alleviated by random fluctuations. The persistent entanglement is mainly due to non-adiabatic dynamics since the final splitting is so fast that the non-localization of wave functions is kept during the separation. These findings may impact the understanding of quantum entanglement more broadly in mesoscopic systems.