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arXiv:2408.07375 · Physics Letters B

Quantum entanglement in nuclear fission

Qiang Yu, Junchen Pei, Kyle Godbey

Published Jan 14, 2025• 15 citations
arXivHTMLPDF

Abstract

Nuclear fission presents a unique example of quantum entanglement in strongly interacting many-body systems. A heavy nucleus can split into hundreds of combinations of two complementary fragments in the fission process. The entanglement of fragment wave functions is persistent even after separation and impacts the partition of particles and energies between fragments. Based on microscopic dynamical calculations of the fission of 240 Pu, this work finds that dynamical quantum entanglement is indispensable in the appearance of sawtooth distributions of average excitation energies of fragments and thus neutron multiplicities, but not in average neutron excess of fragments. Both sawtooth slopes from particle-number projections are found to be steep – a feature which can be alleviated by random fluctuations. The persistent entanglement is mainly due to non-adiabatic dynamics since the final splitting is so fast that the non-localization of wave functions is kept during the separation. These findings may impact the understanding of quantum entanglement more broadly in mesoscopic systems.

DOI
10.1016/j.physletb.2025.139248

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Nuclear fission presents a unique example of quantum entanglement in strongly interacting many-body systems. A heavy nucleus can split into hundreds of combinations of two complementary fragments in the fission process. The entanglement of fragment wave functions is persistent even after separation and impacts the partition of particles and energies between fragments. Based on microscopic dynamical calculations of the fission of 240 Pu, this work finds that dynamical quantum entanglement is indispensable in the appearance of sawtooth distributions of average excitation energies of fragments and thus neutron multiplicities, but not in average neutron excess of fragments. Both sawtooth slopes from particle-number projections are found to be steep – a feature which can be alleviated by random fluctuations. The persistent entanglement is mainly due to non-adiabatic dynamics since the final splitting is so fast that the non-localization of wave functions is kept during the separation. These findings may impact the understanding of quantum entanglement more broadly in mesoscopic systems.
Quantum computers promise advantages for simulating strongly correlated quantum many-body systems, like atomic nuclei, that are beyond the reach of classical computers. Realizing this potential requires understanding the quantum complexity structure of the target problem. We investigate the time-evolution of two key indicators of quantum complexity, bipartite entanglement entropy and non-local magic (non-stabilizerness), in nuclear reaction dynamics. We analyze two representative dynamical processes: scattering in a one-dimensional model of strongly interacting fermions governed by the Negele potential, and a realistic simulation of 240^{240}240Pu fission within time-dependent Hartree-Fock-Bogoliubov (TDHFB) theory. In the former case, we find that interactions dynamically generate both entanglement and non-local magic, leaving persistent signatures of quantum complexity in the outgoing states. In the latter, we observe that substantial quantum complexity survives in the spatial bipartition of daughter fragments well beyond scission. The presence of significant non-local magic and entanglement in both cases strongly indicate that quantum computers would provide substantial advantages for accurately simulating nuclear reaction dynamics.
Nuclear fission provides a unique manifestation of spatially nonlocal many-body entanglement. We compute the bipartite spatial entanglement entropy exactly along dynamical fission trajectories, by leveraging the fermionic Gaussian state formulation. Across seven representative fissioning channels, the final entanglement entropy correlates strongly with the intrinsic particle number variance of the fragment, yet exhibits no simple dependence on scission geometries. Most notably the entanglement is significantly suppressed when fragments are magic nuclei, revealing a shell anti-entanglement effect. This work establishes entanglement entropy as a novel lens that extends the conventional conception of nuclear fission.
Nuclear reactions present an interesting case for studies of the time evolution of entanglement between complex quantum systems. In this work, the time-dependent nuclear density-functional theory is employed to explore entanglement in multinucleon transfer reactions. As an illustrative example, for the reaction 40Ca+208Pb^{40}\mathrm{Ca}+^{208}\mathrm{Pb}40Ca+208Pb at Elab=249MeV{E}_{\mathrm{lab}}=249\phantom{\rule{4pt}{0ex}}\mathrm{MeV}Elab​=249MeV, in the interval of impact parameters 4.65−−7.40fm4.65--7.40\phantom{\rule{4pt}{0ex}}\mathrm{fm}4.65−−7.40fm, and the relativistic density-functional PC-PK1, we compute the von Neumann entropies, entanglement between fragments, nucleon-number fluctuations, and Shannon entropy for the nucleon-number observable. A simple linear correlation is established between the entanglement and nucleon-number fluctuation of the final fragments. The entanglement between the fragments can be related to the corresponding excitation energies and angular momenta. The relationship between the von Neumann entropy and the Shannon entropy for the nucleon-number observable is analyzed, as well as the time evolution of the entanglement (nucleon-number fluctuation). The entanglement is also calculated for a range of incident energies and it is shown how, depending on the impact parameter, the entanglement increases with the collision energy.
Nuclear time-dependent density functional theory is used to investigate spin generation and entanglement of fission fragments in spontaneous fission of 252^{252}252Cf, incorporating both axial and non-axial deformations. Axially symmetric fission trajectories enforce strict constraints: counter rotation (twisting mode) along the fission axis and equiprobable bending/wriggling modes perpendicular to it. Non-axial modes broaden the distributions of fission fragment spin projection on the fission axis, and allow for axial (tilting) collective rotations, which are forbidden on axially symmetric trajectories. Mutual information analysis reveals that axial-symmetry breaking reduces spin-spin correlations along the fission axis of symmetric cases, while perpendicular correlations remain more resilient. The effect of triaxial degrees of freedom on the opening angle distribution between the spins of the fission fragments is analyzed.
Nuclear time-dependent density functional theory is used to investigate spin generation and entanglement of fission fragments in spontaneous fission of ^{252}Cf, incorporating both axial and nonaxial deformations. Axially symmetric fission trajectories enforce strict constraints: counterrotation (twisting mode) along the fission axis and equiprobable bending and wriggling modes perpendicular to it. Nonaxial modes broaden the distributions of fission fragment spin projection on the fission axis, and allow for axial (tilting) collective rotations, which are forbidden on axially symmetric trajectories. Mutual information analysis reveals that axial-symmetry breaking reduces spin-spin correlations along the fission axis of symmetric cases, while perpendicular correlations remain more resilient. The effect of triaxial degrees of freedom on the opening angle distribution between the spins of the fission fragments is analyzed.
Abstract We compute the proton-neutron entanglement entropy in the interacting nuclear shell model for a variety of nuclides and interactions. Some results make intuitive sense, for example, that the shell structure, as governed by single-particle and monopole energies, strongly affects the energetically available space and thus the entanglement entropy. We also find a surprising result: that the entanglement entropy at low excitation energy tends to decrease for nuclides when N ≠ Z. While we provide evidence this arises from the physical nuclear force by contrasting with random two-body interactions which shows no such decrease, the exact mechanism is unclear. Nonetheless, the low entanglement suggests that in models of neutron-rich nuclides, the coupling between protons and neutrons may be less computationally demanding than one might otherwise expect.