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arXiv:2511.08313 · Physical Review Research

Cryogenic source of atomic tritium for precision spectroscopy and neutrino-mass measurements

Aleksei Semakin, Janne Ahokas, Tom Kiilerich, Sergey Vasiliev, Francois Nez, Pauline Yzombard, Valery Nesvizhevsky, Eberhard Widmann, Paolo Crivelli, Caroline Rodenbeck, Marco Röllig, Magnus Schlösser

physics.atom-phnucl-exphysics.ins-detquant-phSubmitted Nov 11, 2025• Announced Nov 12, 2025• 0 citations
v1 · Nov 11, 2025v2 · Feb 27, 2026v3 · Jul 2, 2026
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Abstract

We propose a concept for a cryogenic source of atomic tritium at sub-kelvin temperatures and energies suitable for magnetic trapping. The source is based on the dissociation of solid molecular tritium films below 1 K by electrons from a pulsed RF discharge, a technique recently demonstrated for atomic hydrogen, combined with buffer-gas cooling and magnetic confinement. We analyze the key processes limiting the source performance, adsorption, spin exchange and recombination, and show that atomic tritium fluxes exceeding 1e15 per second at kinetic energies of 100 mK can be achieved at the entrance of a magnetic trap. Such a source would enable Doppler-free two-photon 1S-2S spectroscopy in atomic tritium for high-precision measurements of the triton charge radius, providing a crucial benchmark for bound-state QED and improving the comparison between electronic, muonic, and scattering determinations of nuclear sizes in light systems. Beyond spectroscopy, an atomic tritium source avoids molecular final-state broadening in beta-decay and is therefore necessary for next-generation neutrino-mass measurements; combined with detector technologies such as sub-eV resolution quantum sensors or cyclotron radiation emission spectroscopy, it enables order-of-magnitude improvement compared to the current KATRIN sensitivity, reaching sensitivities below the inverted ordering regime. Additionally, the source can be used to generate a beam of low-field-seeking deuterium atoms for loading magnetic traps, an important benchmark before trapping tritium atoms and useful for precision spectroscopy.

Comments
10 pages, 2 figures

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We propose a concept for a cryogenic source of atomic tritium at sub-kelvin temperatures and energies suitable for magnetic trapping. The source is based on the dissociation of solid molecular tritium films below 1 K by electrons from a pulsed RF discharge, a technique recently demonstrated for atomic hydrogen, combined with buffer-gas cooling and magnetic confinement. We analyze the key processes limiting the source performance, adsorption, spin exchange and recombination, and show that atomic tritium fluxes exceeding 1e15 per second at kinetic energies of 100 mK can be achieved at the entrance of a magnetic trap. Such a source would enable Doppler-free two-photon 1S-2S spectroscopy in atomic tritium for high-precision measurements of the triton charge radius, providing a crucial benchmark for bound-state QED and improving the comparison between electronic, muonic, and scattering determinations of nuclear sizes in light systems. Beyond spectroscopy, an atomic tritium source avoids molecular final-state broadening in beta-decay and is therefore necessary for next-generation neutrino-mass measurements; combined with detector technologies such as sub-eV resolution quantum sensors or cyclotron radiation emission spectroscopy, it enables order-of-magnitude improvement compared to the current KATRIN sensitivity, reaching sensitivities below the inverted ordering regime. Additionally, the source can be used to generate a beam of low-field-seeking deuterium atoms for loading magnetic traps, an important benchmark before trapping tritium atoms and useful for precision spectroscopy.
Abstract Next generation tritium decay experiments to determine the absolute neutrino mass require high-precision measurements of β -decay electron energies close to the kinematic end point. To achieve this, the development of high phase-space density sources of atomic tritium is required, along with the implementation of methods to control the motion of these atoms to allow extended observation times. A promising approach to efficiently and accurately measure the kinetic energies of individual β -decay electrons generated in these dilute atomic gases, is to determine the frequency of the cyclotron radiation they emit in a precisely characterised magnetic field. This cyclotron radiation emission spectroscopy technique can benefit from recent developments in quantum technologies. Absolute static-field magnetometry and electrometry, which is essential for the precise determination of the electron kinetic energies from the frequency of their emitted cyclotron radiation, can be performed using atoms in superpositions of circular Rydberg states. Quantum-limited microwave amplifiers will allow precise cyclotron frequency measurements to be made with maximal signal-to-noise ratios and minimal observation times. Exploiting the opportunities offered by quantum technologies in these key areas, represents the core activity of the Quantum Technologies for Neutrino Mass project. Its goal is to develop a new experimental apparatus that can enable a determination of the absolute neutrino mass with a sensitivity on the order of 10 meV / c 2 .
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Abstract We present a design and performance tests of an intense source of cold hydrogen atoms for loading large magnetic traps. Our source is based on a cryogenic dissociator of molecular hydrogen at 0.6 K followed by a series of thermal accommodators at 0.5, 0.2 and 0.13 K with inner surfaces covered by a superfluid helium film. All components are thermally anchored to corresponding stages of a dilution refrigerator. The source provides a continuous flux of 7×10137\times 10^{13}7×1013 7 × 10 13 H atoms/s in a temperature range of 130–200 mK. We have successfully used the source for loading a large Ioffe–Pritchard magnetic trap recently built in our laboratory (Ahokas et al. in Rev Sci Instrum 93(2):023201, 2022). Calorimetric measurements of the atomic recombination heat allow reliable determination of the atomic flux and H gas density in the trap. We have tested the performance of the source and loading of H atoms into the trap at various configurations of the trapping field, reducing the magnetic barrier height to 75 %\%% % and 50 %\%% % of the nominal value of 0.8 T (0.54 K) as well as at the open configuration of the trap at its lower end, when the atoms are in contact with the trapping cell walls covered by a superfluid helium film. In the latter case, raising the trapping cell temperature to 200–250 mK, the low-field seeking atoms at densities exceeding 10 11^{11}11 11 cm−3\hbox {cm}^{-3}cm−3 cm - 3 can be stored for the time over 10 3^33 3 s, sufficiently long for experiments on precision spectroscopy of cold H gas. Graphic abstract
The most sensitive direct neutrino mass searches today are based on measurement of the end point of the $\ensuremath{\beta}$ spectrum of tritium to infer limits on the mass of the unobserved neutrino. To avoid the smearing associated with the distribution of molecular final states in the T-He molecule, the next generation of these experiments will need to employ atomic (T) rather than molecular (T2)({\mathrm{T}}_{2})(T2​) tritium sources, at currents of at least 1015{10}^{15}1015 atoms per second. Following production, atomic T can be trapped in gravitational and/or magnetic bottles for $\ensuremath{\beta}$ spectrum experiments, if and only if it can first be cooled to millikelvin temperatures. Accomplishing this cooling presents substantial technological challenges. The Project 8 collaboration is developing a technique based on magnetic evaporative cooling along a beamline (MECB) for the purpose of cooling T to feed a magnetogravitational trap that also serves as a cyclotron radiation emission spectroscope. Initial tests of the approach are planned in a pathfinder apparatus using atomic Li. This paper presents a method for analyzing the dynamics of the MECB technique and applies these calculations to the design of systems for cooling and slowing of atomic Li and T. A scheme is outlined that could provide a current of T at the millikelvin temperatures required for the Project 8 neutrino mass search.
The rates of elastic and inelastic scattering processes of spin-polarized atomic tritium are vital inputs for the design and operation of experiments using cold, magnetically trapped tritium atoms. Elastic scattering dominates the total cross section and dictates the thermophysical properties of the vapor, determining the efficiency of magnetic evaporative cooling and the fluid dynamical properties of the trapped atom cloud. Spin-changing cross sections in both exchange and dipolar channels determine the trap lifetime of the various hyperfine states, imposing constraints on the required atomic tritium supply rate to maintain a given trap density. Motivated by the needs of next-generation spectrometers that will study the tritium beta end point to infer the mass of the neutrino, we present new calculations of the elastic, spin-exchange, and dipolar cross sections for spin-polarized atomic tritium. Cross sections and rate constants are reported for magnetic field strengths of 0--10 T and temperatures from 0 to 100 K in all relevant Zeeman-hyperfine channels for both tritium and hydrogen. Results are benchmarked against past calculations for atomic hydrogen and the limited available results for tritium, and extend far into the regimes where past calculations have not been available.
The most sensitive direct neutrino mass searches today are based on measurement of the endpoint of the beta spectrum of tritium to infer limits on the mass of the unobserved neutrino. To avoid the smearing associated with the distribution of molecular final states in the T-He molecule, the next generation of these experiments will need to employ atomic (T) rather than molecular (T2_{2}2​) tritium sources, at currents of at least 1015^{15}15 atoms per second. Following production, atomic T can be trapped in gravitational and/or magnetic bottles for beta spectrum experiments, if and only if it can first be cooled to millikelvin temperatures. Accomplishing this cooling presents substantial technological challenges. The Project 8 collaboration is developing a technique based on magnetic evaporative cooling along a beamline (MECB) for the purpose of cooling T to feed a magneto-gravitational trap that also serves as a cyclotron radiation emission spectroscope. Initial tests of the approach are planned in a pathfinder apparatus using atomic Li. This paper presents a method for analyzing the dynamics of the MECB technique, and applies these calculations to the design of systems for cooling and slowing of atomic Li and T. A scheme is outlined that could provide a current of T at the millikelvin temperatures required for the Project 8 neutrino mass search.