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arXiv:2502.00188

Dynamics of Magnetic Evaporative Beamline Cooling for Preparation of Cold Atomic Beams

A. Ashtari Esfahani, S. Bhagvati, S. Böser, Matthew J. Brandsema, R. Cabral, V. A. Chirayath, C. Claessens, N. Coward, L. de Viveiros, Peter J. Doe, Elliott, M. G., S. Enomoto, M. Fertl, Joseph A. Formaggio, B. T. Foust, J. K. Gaison, P. Harmston, Karsten M. Heeger, B. J. P. Jones, Karim, E., K. Kazkaz, P. T. Kolbeck, M. Li, A. Lindman, C.-Y. Liu, C. Matthé, R. Mohiuddin, B. Monreal, Brunilda Mucogllava, R. Mueller, Akshima Negi, J. A. Nikkel, Elise Novitski, Noah S. Oblath, Oueslati, M., J. I. Peña, W. Pettus, V. S. Ranatunga, R. Reimann, A. L. Reine, R. G. H. Robertson, L. Saldaña, P. L. Slocum, F. Spanier, Juliana Stachurska, K. Stogsdill, Yu-Hao Sun, Pranava Teja Surukuchi, Taylor, L., A. B. Telles, Florian Thomas, Larisa A. Thorne, Thümmler, T., W. Van De Pontseele, Brent A. VanDevender, T. E. Weiss, M. Wynne, A. Ziegler

Published Jan 31, 2025• 0 citations
arXivHTMLPDF

Abstract

The most sensitive direct neutrino mass searches today are based on measurement of the endpoint of the beta spectrum of tritium to infer limits on the mass of the unobserved neutrino. To avoid the smearing associated with the distribution of molecular final states in the T-He molecule, the next generation of these experiments will need to employ atomic (T) rather than molecular (T$_{2}$) tritium sources, at currents of at least 10$^{15}$ atoms per second. Following production, atomic T can be trapped in gravitational and/or magnetic bottles for beta spectrum experiments, if and only if it can first be cooled to millikelvin temperatures. Accomplishing this cooling presents substantial technological challenges. The Project 8 collaboration is developing a technique based on magnetic evaporative cooling along a beamline (MECB) for the purpose of cooling T to feed a magneto-gravitational trap that also serves as a cyclotron radiation emission spectroscope. Initial tests of the approach are planned in a pathfinder apparatus using atomic Li. This paper presents a method for analyzing the dynamics of the MECB technique, and applies these calculations to the design of systems for cooling and slowing of atomic Li and T. A scheme is outlined that could provide a current of T at the millikelvin temperatures required for the Project 8 neutrino mass search.

DOI
10.48550/arxiv.2502.00188

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The most sensitive direct neutrino mass searches today are based on measurement of the endpoint of the beta spectrum of tritium to infer limits on the mass of the unobserved neutrino. To avoid the smearing associated with the distribution of molecular final states in the T-He molecule, the next generation of these experiments will need to employ atomic (T) rather than molecular (T2_{2}2​) tritium sources, at currents of at least 1015^{15}15 atoms per second. Following production, atomic T can be trapped in gravitational and/or magnetic bottles for beta spectrum experiments, if and only if it can first be cooled to millikelvin temperatures. Accomplishing this cooling presents substantial technological challenges. The Project 8 collaboration is developing a technique based on magnetic evaporative cooling along a beamline (MECB) for the purpose of cooling T to feed a magneto-gravitational trap that also serves as a cyclotron radiation emission spectroscope. Initial tests of the approach are planned in a pathfinder apparatus using atomic Li. This paper presents a method for analyzing the dynamics of the MECB technique, and applies these calculations to the design of systems for cooling and slowing of atomic Li and T. A scheme is outlined that could provide a current of T at the millikelvin temperatures required for the Project 8 neutrino mass search.
The most sensitive direct neutrino mass searches today are based on measurement of the end point of the $\ensuremath{\beta}$ spectrum of tritium to infer limits on the mass of the unobserved neutrino. To avoid the smearing associated with the distribution of molecular final states in the T-He molecule, the next generation of these experiments will need to employ atomic (T) rather than molecular (T2)({\mathrm{T}}_{2})(T2​) tritium sources, at currents of at least 1015{10}^{15}1015 atoms per second. Following production, atomic T can be trapped in gravitational and/or magnetic bottles for $\ensuremath{\beta}$ spectrum experiments, if and only if it can first be cooled to millikelvin temperatures. Accomplishing this cooling presents substantial technological challenges. The Project 8 collaboration is developing a technique based on magnetic evaporative cooling along a beamline (MECB) for the purpose of cooling T to feed a magnetogravitational trap that also serves as a cyclotron radiation emission spectroscope. Initial tests of the approach are planned in a pathfinder apparatus using atomic Li. This paper presents a method for analyzing the dynamics of the MECB technique and applies these calculations to the design of systems for cooling and slowing of atomic Li and T. A scheme is outlined that could provide a current of T at the millikelvin temperatures required for the Project 8 neutrino mass search.
While cold molecule experiments are rapidly moving towards their promised benefits of precision spectroscopy, controllable chemistry, and novel condensed phases, heretofore the field has been greatly limited by a lack of methods to cool and compress chemically diverse species to temperatures below ten millikelvin. While in atomic physics these needs are fulfilled by laser cooling, magneto-optical trapping, and evaporative cooling, until now none of these techniques have been applicable to molecules. In this thesis, two major breakthroughs are reported. The first is the observation of evaporative cooling in magnetically trapped hydroxyl (OH) radicals, which potentially opens a path all the way to Bose-Einstein condensation of dipolar radicals, as well as allowing cold- and ultracold-chemistry studies of fundamental reaction mechanisms. Through the combination of an extremely high gradient magnetic quadrupole trap and the use of the OH Λ-doublet transition to enable highly selective forced evaporation, cooling by an order of magnitude in temperature was achieved and yielded a final temperature no higher than 5mK. The second breakthrough is the successful application of laser cooling and magneto-optical trapping to molecules. Motivated by a proposal in this thesis, laser cooling of molecules is now known to be technically feasible in a select but substantial pool of diatomic molecules. The demonstration of not only Doppler cooling but also two-dimensional magneto-optical trapping in yttrium (II) oxide, YO, is expected to enable rapid growth in the availability of ultracold molecules--just as the invention of the atomic magneto-optical trap stimulated atomic physics twenty-five years ago.
We propose a concept for a cryogenic source of atomic tritium at sub-Kelvin temperatures and energies suitable for magnetic trapping. The source is based on the dissociation of solid molecular T2 films below 1 K by electrons from a pulsed RF discharge, a technique recently demonstrated for atomic hydrogen, combined with buffer-gas cooling and magnetic confinement. We analyze the key processes limiting the source performance, adsorption, spin exchange and recombination, and show that atomic tritium fluxes exceeding 1e15 1/s at kinetic energies of 100 mK can be achieved at the entrance to the magnetic trap. Such a source would enable Doppler-free two-photon 1S-2S spectroscopy in atomic tritium for high-precision measurements of the triton charge radius, providing a crucial benchmark for bound-state QED and improving the comparison between electronic, muonic, and scattering determinations of nuclear sizes in light systems. Beyond spectroscopy, an atomic tritium source avoids molecular final state broadening in the beta decay and is therefore necessary for next generation neutrino mass measurements; combined with detector technologies such as sub-eV resolution quantum sensors or cyclotron radiation emission spectroscopy, it enables an order of magnitude improvement compared to the current best experimental limit. Additionally, the source can be used to generate a beam of low field seeking deuterium atoms for loading magnetic traps, an important benchmark before trapping tritium atoms, which is useful for precision spectroscopy.
Abstract Next generation tritium decay experiments to determine the absolute neutrino mass require high-precision measurements of β -decay electron energies close to the kinematic end point. To achieve this, the development of high phase-space density sources of atomic tritium is required, along with the implementation of methods to control the motion of these atoms to allow extended observation times. A promising approach to efficiently and accurately measure the kinetic energies of individual β -decay electrons generated in these dilute atomic gases, is to determine the frequency of the cyclotron radiation they emit in a precisely characterised magnetic field. This cyclotron radiation emission spectroscopy technique can benefit from recent developments in quantum technologies. Absolute static-field magnetometry and electrometry, which is essential for the precise determination of the electron kinetic energies from the frequency of their emitted cyclotron radiation, can be performed using atoms in superpositions of circular Rydberg states. Quantum-limited microwave amplifiers will allow precise cyclotron frequency measurements to be made with maximal signal-to-noise ratios and minimal observation times. Exploiting the opportunities offered by quantum technologies in these key areas, represents the core activity of the Quantum Technologies for Neutrino Mass project. Its goal is to develop a new experimental apparatus that can enable a determination of the absolute neutrino mass with a sensitivity on the order of 10 meV / c 2 .
The continuous injection and propagation of a cold atomic beam in a 1.7 m long high-gradient (up to 2.7 kG/cm) magnetic guide is demonstrated. Continuous injection is accomplished by side-loading a magnetic guide with atoms from a sequence of two modified magneto-optical traps. In the high-gradient portion of the guide, the guided atomic beam has a transverse temperature of 420 muK +/- 40 muK, a longitudinal temperature of 1 mK, and an average velocity of order 1 m/s. Essential for the characterization of this steady-state atomic beam, imaging methods compatible with the high field-gradients associated with this magnetic guide have been investigated and developed. By utilizing a probe laser tuned to an open transition, the fluorescence yield per atom is largely fixed throughout the trap volume, independent of the trapping field. This enables a reliable conversion of fluorescence images into atomic-density profiles. Using a fixed radio-frequency (nurf) current coupled directly onto the guide wires, continuous and selective removal of atoms with a transverse energy exceeding hnurf is demonstrated. This removal scheme is the essence of an rf filter, where the number of modes occupied by the atomic flow is reduced. Through sufficient rf-filtering, a near-single-mode guided atomic beam should be achievable, enabling basic atom-interferometric experiments. The extension of this fixed-frequency removal of atoms for continuous position-resolved evaporative cooling in a long magnetic guide is outlined. Employing an innovative gridless technique for performing Direct Simulation of rarefied gas dynamics via Monte Carlo (DSMC), the evaporative cooling process in a guided atomic beam has been simulated. Both fixed-frequency as well as variable-frequency evaporative cooling layouts have been explored and the results of these simulations are presented. The implementation of this gridless technique is presented and its benefits are briefly outlined. In parallel with the development of a continuous-wave atom laser, tools suited to manipulate cold atomic beams in atom guides have been explored. An atomic guide with a tunable aspect ratio, using rf-dressed state potentials, is presented.
Evaporative cooling has proven to be an invaluable technique in atomic physics, allowing for the study of effects such as Bose-Einstein condensation. One main topic of this thesis is the first application of evaporative cooling to cold non-neutral plasmas stored in an ion trap. We (the ALPHA collaboration) have achieved cooling of a cloud of antiprotons to a temperature as low as 9 K, two orders of magnitude lowerthan ever directly measured previously. The measurements are well-described by appropriate rate equations for the temperature and number of particles. The technique has direct application to the ongoing attempts to produce trapped samples of antihydrogen. In these experiments the maximum trap depths are ex tremely shallow (~0.6 K for ground state atoms), and careful control of the trapped antiprotons and positrons used to form the (anti)atoms is essential to succes. Since 2006 powerful tools to diagnose and manipulate the antiproton and positron plasmas in the ALPHA apparatus have been developed and used in attempts to trap antihydrogen. These efforts are the second main topic of this thesis.