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arXiv:2412.13981

Cold source of atomic hydrogen for loading large magnetic traps

Aleksei Semakin, Janne Ahokas, Otto Hanski, V. Dvornichenko, Tom Kiilerich, F. Nez, P. Yzombard, Валерий Викторович Несвижевский, E. Widmann, P. Crivelli, Sergey Vasiliev

Published Dec 18, 2024• 0 citations
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Abstract

We present a design and performance tests of an intense source of cold hydrogen atoms for loading large magnetic traps. Our source is based on a cryogenic dissociator of molecular hydrogen at 0.6 K followed by a series of thermal accommodators at 0.5, 0.2 and 0.13 K with inner surfaces covered by a superfluid helium film. All components are thermally anchored to corresponding stages of a dilution refrigerator. The source provides a continuous flux of 7$\cdot$$10^{13}$ H atoms/s in a temperature range of 130-200 mK. We have successfully used the source for loading a large Ioffe-Pritchard magnetic trap recently built in our laboratory [arXiv:2108.09123 or Rev. Sci. Instr. 93 (2), 023201 (2022)]. Calorimetric measurements of the atomic recombination heat allow reliable determination of the atomic flux and H gas density in the trap. We have tested the performance of the source and loading of H atoms into the trap at various configurations of the trapping field, reducing the magnetic barrier height to 75% and 50% of the nominal value of 0.8 T (0.54 K) as well as at the open configuration of the trap at its lower end, when the atoms are in contact with the trapping cell walls covered by a superfluid helium film. In the latter case, raising the trapping cell temperature to 200-250 mK, the low-field seeking atoms at densities exceeding 10$^{11}$ cm$^{-3}$ can be stored for the time over 1000 s, sufficiently long for experiments on precision spectroscopy of cold H gas.

DOI
10.48550/arxiv.2412.13981

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We present a design and performance tests of an intense source of cold hydrogen atoms for loading large magnetic traps. Our source is based on a cryogenic dissociator of molecular hydrogen at 0.6 K followed by a series of thermal accommodators at 0.5, 0.2 and 0.13 K with inner surfaces covered by a superfluid helium film. All components are thermally anchored to corresponding stages of a dilution refrigerator. The source provides a continuous flux of 7\cdot$$10^{13} H atoms/s in a temperature range of 130-200 mK. We have successfully used the source for loading a large Ioffe-Pritchard magnetic trap recently built in our laboratory [arXiv:2108.09123 or Rev. Sci. Instr. 93 (2), 023201 (2022)]. Calorimetric measurements of the atomic recombination heat allow reliable determination of the atomic flux and H gas density in the trap. We have tested the performance of the source and loading of H atoms into the trap at various configurations of the trapping field, reducing the magnetic barrier height to 75% and 50% of the nominal value of 0.8 T (0.54 K) as well as at the open configuration of the trap at its lower end, when the atoms are in contact with the trapping cell walls covered by a superfluid helium film. In the latter case, raising the trapping cell temperature to 200-250 mK, the low-field seeking atoms at densities exceeding 1011^{11}11 cm−3^{-3}−3 can be stored for the time over 1000 s, sufficiently long for experiments on precision spectroscopy of cold H gas.
Abstract We present a design and performance tests of an intense source of cold hydrogen atoms for loading large magnetic traps. Our source is based on a cryogenic dissociator of molecular hydrogen at 0.6 K followed by a series of thermal accommodators at 0.5, 0.2 and 0.13 K with inner surfaces covered by a superfluid helium film. All components are thermally anchored to corresponding stages of a dilution refrigerator. The source provides a continuous flux of 7×10137\times 10^{13}7×1013 7 × 10 13 H atoms/s in a temperature range of 130–200 mK. We have successfully used the source for loading a large Ioffe–Pritchard magnetic trap recently built in our laboratory (Ahokas et al. in Rev Sci Instrum 93(2):023201, 2022). Calorimetric measurements of the atomic recombination heat allow reliable determination of the atomic flux and H gas density in the trap. We have tested the performance of the source and loading of H atoms into the trap at various configurations of the trapping field, reducing the magnetic barrier height to 75 %\%% % and 50 %\%% % of the nominal value of 0.8 T (0.54 K) as well as at the open configuration of the trap at its lower end, when the atoms are in contact with the trapping cell walls covered by a superfluid helium film. In the latter case, raising the trapping cell temperature to 200–250 mK, the low-field seeking atoms at densities exceeding 10 11^{11}11 11 cm−3\hbox {cm}^{-3}cm−3 cm - 3 can be stored for the time over 10 3^33 3 s, sufficiently long for experiments on precision spectroscopy of cold H gas. Graphic abstract
We describe the design and performance of a large magnetic trap for storage and cooling of atomic hydrogen (H). The trap operates in the vacuum space of a dilution refrigerator at a temperature of 1.5 K. Aiming at a large volume of the trap, we implemented the octupole configuration of linear currents (Ioffe bars) for the radial confinement, combined with two axial pinch coils and a 3 T solenoid for the cryogenic H dissociator. The octupole magnet consists of eight race-track segments, which are compressed toward each other with magnetic forces. This provides a mechanically stable and robust construction with a possibility of replacement or repair of each segment. A maximum trap depth of 0.54 K (0.8 T) was reached, corresponding to an effective volume of 0.5 l for hydrogen gas at 50 mK. This is an order of magnitude larger than ever used for trapping atoms.
We propose a concept for a cryogenic source of atomic tritium at sub-Kelvin temperatures and energies suitable for magnetic trapping. The source is based on the dissociation of solid molecular T2 films below 1 K by electrons from a pulsed RF discharge, a technique recently demonstrated for atomic hydrogen, combined with buffer-gas cooling and magnetic confinement. We analyze the key processes limiting the source performance, adsorption, spin exchange and recombination, and show that atomic tritium fluxes exceeding 1e15 1/s at kinetic energies of 100 mK can be achieved at the entrance to the magnetic trap. Such a source would enable Doppler-free two-photon 1S-2S spectroscopy in atomic tritium for high-precision measurements of the triton charge radius, providing a crucial benchmark for bound-state QED and improving the comparison between electronic, muonic, and scattering determinations of nuclear sizes in light systems. Beyond spectroscopy, an atomic tritium source avoids molecular final state broadening in the beta decay and is therefore necessary for next generation neutrino mass measurements; combined with detector technologies such as sub-eV resolution quantum sensors or cyclotron radiation emission spectroscopy, it enables an order of magnitude improvement compared to the current best experimental limit. Additionally, the source can be used to generate a beam of low field seeking deuterium atoms for loading magnetic traps, an important benchmark before trapping tritium atoms, which is useful for precision spectroscopy.
Atomic hydrogen has been loaded into a 1-K deep magnetic trap through the use of a dilution refrigerator. Evaporative cooling has been used to cool the trapped hydrogen into the submillikelvin temperature regime. These techniques have produced a sample with density of 8 × 1013 cm-3 at a temperature of 100 μK. At this density a transition to a Bose-Einstein condensate is predicted to occur at a temperature of 30 μK. These results have been obtained with a magnetic trap that has been constructed to accommodate upcoming experiments based on laser spectroscopy of the 1S-2S two photon transition in the trapped hydrogen. A frequency doubled narrow linewidth cw dye laser system has been constructed to excite the 1S-2S transition. The excitation will be detected by the observation of electric field-induced Lyman-alpha fluorescence. The optical detection system should yield improved sample density and temperature diagnostic capabilities that will facilitate a closer approach to the quantum degenerate regime. Additionally the cold, confined hydrogen gas offers the possibility of improving the level of resolution of Doppler-free hydrogen 1S-2S laser spectroscopy by several orders of magnitude.
We describe the loading of a minimum-BBB-field trap with neutral atomic hydrogen cooled through thermal exchange with liquid-helium surfaces. We monitor the gas during filling and decay by observing the atoms which are ejected from the trap as a result of spin exchange and magnetic dipolar relaxation. The stability of the gas is unaffected if we change the wall coverage from pure 4He^{4}\mathrm{He}4He to dilute 3He^{3}\mathrm{He}3He and 4He^{4}\mathrm{He}4He mixtures. The maximum trapped density is 3 \ifmmode\times\else\texttimes\fi{} 1014{10}^{14}1014 ${\mathrm{cm}}^{\ensuremath{-}3}$ at about 100 mK. The limiting decay rate is attributed to dipolar relaxation and found to agree with theory for both magnitude and field dependence.
We have confined over 5\ifmmode\times\else\texttimes\fi{}1012{10}^{12}1012 atoms of hydrogen in a static magnetic trap. The atoms are loaded into the trap by precooling with a dilution refrigerator. At operating densities near 1\ifmmode\times\else\texttimes\fi{}1013{10}^{13}1013 ${\mathrm{cm}}^{\mathrm{\ensuremath{-}}3}$ the gas is observed to be electron and nuclear polarized in the uppermost hyperfine state. The long lifetime of the trapped gas (over 20 min) suggests that it is thermally decoupled from the wall and has evaporatively cooled to a temperature of about 40 mK. The residual decay of the gas density is consistent with spin relaxation induced by dipolar interactions between atoms.