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arXiv:2408.12700 · Physical Review A

Spatiospectral control of spontaneous emission

Seyyed Hossein Asadpour, Muqaddar Abbas, Hamid Reza Hamedi, Julius Ruseckas, Emmanuel Paspalakis, Reza Asgari

Published Sep 9, 2024• 18 citations
arXivHTMLPDF

Abstract

We propose a scheme aimed at achieving spatiospectral control over spontaneous emission within a four-level atom-light coupling system interacting with optical vortices carrying orbital angular momentum (OAM). The atom comprises a ground level and two excited states coupled with two laser fields, forming a V subsystem where the upper states exclusively decay to a common fourth state via two channels. By investigating various initial states of the atom and considering the presence or absence of quantum interference in spontaneous emission channels, we analyze how the characteristics of the OAM-carrying vortex beam imprint onto the emission spectrum. The interplay between the optical vortex and the quantum system, including its environment modes, induces a wide variety of spatiospectral behavior, including two-dimensional spectral-peak narrowing, spectral-peak enhancement, spectral-peak suppression, and spontaneous emission reduction or quenching in the spatial azimuthal plane. Our findings shed light on the dynamics of atom--vortex-beam light interactions and offer insights into the manipulation of emission properties at the quantum level.

DOI
10.1103/physreva.110.033706

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We propose a scheme aimed at achieving spatiospectral control over spontaneous emission within a four-level atom-light coupling system interacting with optical vortices carrying orbital angular momentum (OAM). The atom comprises a ground level and two excited states coupled with two laser fields, forming a V subsystem where the upper states exclusively decay to a common fourth state via two channels. By investigating various initial states of the atom and considering the presence or absence of quantum interference in spontaneous emission channels, we analyze how the characteristics of the OAM-carrying vortex beam imprint onto the emission spectrum. The interplay between the optical vortex and the quantum system, including its environment modes, induces a wide variety of spatiospectral behavior, including two-dimensional spectral-peak narrowing, spectral-peak enhancement, spectral-peak suppression, and spontaneous emission reduction or quenching in the spatial azimuthal plane. Our findings shed light on the dynamics of atom--vortex-beam light interactions and offer insights into the manipulation of emission properties at the quantum level.
We propose a scheme for achieving spatially dependent spontaneous emission by using vortex light beams (OAM) in a five level atomic configuration. It consists of an upper excited level and four lower metastable levels. The excited level is simultaneously coupled to two ground levels by a coherent probe field and a vortex field, respectively. In addition, a microwave field couples two of the ground levels. The excited state is assumed to be coupled by the vacuum modes in the free space and eventually decays to a fifth metastable level. It is found that by manipulating key parameters such as the strength of the Laguerre–Gauss beams, the Rabi frequency and detuning of an external microwave field, and the initial state of the atoms, we can achieve highly tunable spontaneous emission spectra . A wide variety of spatiospectral behavior, including two-dimensional spectral-peak narrowing, spectral-peak enhancement and spontaneous emission quenching is obtained.
We propose a scheme to analyze the generation and detection of optical vortices via spontaneous emission spectra. We consider a five-level M-type atomic system that interacts with two structured coherent light sources and the vacuum radiation field. The photon emitted via spontaneous decay carries information about the orbital angular momentum (OAM) of the newly generated structured light. It is found that by varying the OAM of the driving fields, one can obtain various unique structured light fields via the interference of the two spontaneous decay channels. This research provides deep insights into how the manipulation of OAM of the driving fields coupled with multilevel atomic systems can enable control over the azimuthal aspects of the spontaneous emission. Considering the rich applications of structured light ranging from optical storage to optical communication, our proposal might be useful in quantum information processing techniques.
We propose an efficient scheme to manipulate spontaneous emission spectra using optical vortices carrying orbital angular momentum (OAM) in a coherently driven cold five-level atomic system assisted by a radio frequency (RF) or microwave field. Using experimentally achievable parameters, we find that the spontaneous emission is strongly influenced by quantum destructive interference. And we show that the structured light profile of the probe field can be transferred to the spontaneous emission spectrum via spontaneously generated coherence (SGC). With the aid of SGC, the intensities and detunings of the control and RF fields can be used to tailor the vortex-induced spontaneous emission spectra. When the control and RF fields are configured as vortex beams, it is demonstrated that the spontaneous emission can be coherently controlled through quantum interference by adjusting their topological charges (TCs). Furthermore, we explore intriguing optical properties of the vortex-induced spontaneous emission by varying the TCs of the probe and control fields. This coherently driven atomic system features three closely spaced levels, giving rise to multiple vortex-induced SGC pathways. Our scheme opens avenues for applications in structured light, ranging from optical storage to optical communication.
The atom-photon entanglement using the Laguerre-Gaussian (LG) beams is studied in the closed-loop three-level V-type quantum systems. We consider two schemes with near-degenerate and non-degenerate upper levels: in the first, the effect of the quantum interference due to the spontaneous emission is taken into account and in the second, a microwave plane wave is applied to the upper levels transition. It is shown that the atom-photon entanglement in both schemes depends on the intensity profile as well as the orbital angular momentum (OAM) of the applied fields so that the various spatially dependent entanglement patterns can be generated by Laguerre-Gaussian beams with different OAMs. However, due to the zero intensity,no entanglement appears in the center of the optical vortex beams. As a result, the entanglement between dressed atom and its spontaneous emissions in different points of the atomic vapor cell can be controlled by the OAM of the applied fields. Moreover, our numerical results show that the number of the local maximum degree of entanglement (DEM) peaks depends on the OAM of the applied fields. The degrees of freedom for OAM play a crucial role in spatially dependent atom-photon entanglement in such a way that it may possess broad applications in high-dimensional quantum information processing and data storage.
The noise-induced coherence created via the quantum interference of incoherent radiation in atomic three-level systems of V and \ensuremath{\Lambda} types driven by a pair of weak laser pulses is shown to result in exchange of optical vortices. In the three- level V-type atom-light coupling the system is populated in its ground level, while in the \ensuremath{\Lambda} model the system is initially prepared in an electromagnetically induced transparency state. By solving the quantum optical Maxwell-Bloch equations and with quantum interference of incoherent radiation present, we show that the orbital angular momentum (OAM) of the vortex probe beam can be transferred to a generated signal field. While the exchange efficiency in the V configuration is higher, the losses are less in the \ensuremath{\Lambda} scheme when we consider such a noise-induced coherence. We further discuss the effects of phase mismatching and inhomogeneous broadening on the energy conversion between light beams carrying OAM.
We study the propagation of probe pulses carrying orbital angular momentum (OAM) in a crystal of molecular magnets characterized by a double-$\mathrm{\ensuremath{\Lambda}}$ light-matter coupling scheme. The model is based on the four-wave mixing (FWM) of applied fields interacting with the magnetic dipole moment of the molecular magnets. We consider the light-matter interaction under the situation where a weak probe field carries an optical vortex and investigate the exchange of optical vortices between different frequencies via the FWM in the microwave region. The propagation of OAM beams with nonzero radial indices is then explored. It is found that the conservation of both azimuthal and radial indices is satisfied over the swapping of OAM states of light. Superimposing two initially weak OAM modes with different topological charges creates specific vortex beams with a very characteristic form. The resulting beam contains a central vortex as well as several singly charged peripheral vortices distributed at the same radial distance from the center of the light beam. This complex pattern of vortices arises because the intensity radius of two interfering OAM modes is different. It is shown that the boundary region of intensity dominance of two OAM modes can be controlled by the molecular magnets parameters and strong cw electromagnetic fields. Our proposed scheme may provide a route to study the solid systems suitable for quantum technologies as well as for OAM exchange devices for quantum information processing.