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arXiv:2301.05404 · Physical Review A

Tunable virtual gain in resonantly absorbing media

Denis V. Novitsky

Published Jan 20, 2023• 8 citations
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Abstract

Virtual gain refers to the simulation of real light amplification using radiation with exponentially decaying amplitude so that its complex frequency corresponds to the scattering pole. We study theoretically virtual gain in a two-level resonant medium for different regimes of light-matter interaction depending on the radiation intensity. We show that virtual gain at the pole can be most clearly observed for low intensities, when the medium is absorbing, in contrast to the saturated medium at high intensities. The efficiency of virtual gain can be tuned with the light intensity and controlled dynamically through the population inversion of the medium. Our results show that resonantly absorbing media paradoxically mimic a gainlike response, which admits a number of related phenomena and methods to mold both optical signals and material properties without relying on instability-prone gain media.

DOI
10.1103/physreva.107.013516

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Virtual gain refers to the simulation of real light amplification using radiation with exponentially decaying amplitude so that its complex frequency corresponds to the scattering pole. We study theoretically virtual gain in a two-level resonant medium for different regimes of light-matter interaction depending on the radiation intensity. We show that virtual gain at the pole can be most clearly observed for low intensities, when the medium is absorbing, in contrast to the saturated medium at high intensities. The efficiency of virtual gain can be tuned with the light intensity and controlled dynamically through the population inversion of the medium. Our results show that resonantly absorbing media paradoxically mimic a gainlike response, which admits a number of related phenomena and methods to mold both optical signals and material properties without relying on instability-prone gain media.
Virtual perfect absorption (VPA) is an effect simulating real absorption of light by using excitation at a complex frequency corresponding to a scattering zero. We theoretically study VPA in resonantly absorbing and amplifying media irradiated by two counterpropagating waves with exponentially growing amplitudes. We show that VPA critically depends on the medium density (i.e., level of loss or gain) deteriorating in the high-density limit. In contrast, almost ideal VPA persists in the PT\mathcal{P}TPT-symmetric loss-gain bilayer. For high enough gain, powerful quasilasing pulses are observed at later times symmetrically (single amplifying layer) or asymmetrically (PT\mathcal{P}TPT-symmetric structure) generated in both propagation directions.
Abstract Time-invariant photonic structures amplify or absorb light based on their intrinsic material gain or loss. The coherent interference of multiple beams in space, e.g., in a resonator, can be exploited to tailor the wave interaction with material gain or loss, respectively maximizing lasing or coherent perfect absorption. By contrast, a time-varying system is not bound to conserve energy, even in the absence of material gain or loss, and can support amplification or absorption of a probe wave through parametric phenomena. Here, we demonstrate theoretically and experimentally how a subwavelength film of indium tin oxide, whose bulk permittivity is homogeneously and periodically modulated via optical pumping, can be dynamically tuned to act both as a non-resonant amplifier and a perfect absorber, by manipulating the relative phase of two counterpropagating probe beams. This extends the concept of coherent perfect absorption to the temporal domain. We interpret this result as selective switching between the gain and loss modes present in the momentum bandgap of a periodically modulated medium. By tailoring the relative intensity of the two probes, high-contrast modulation can be achieved with up to 80% absorption and 400% amplification. Our results demonstrate control of gain and loss in time-varying media at optical frequencies and pave the way towards coherent manipulation of light in Floquet-engineered complex photonic systems.
Using the numerical solution of the Maxwell–Bloch equations, we study the interaction of short light pulses with resonant amplifying media. We consider pulses of various shapes – with Gaussian, rectangular, and exponential envelopes, the latter of which has recently attracted increased attention due to its potential for implementing new effects such as virtual absorption. We show that by choosing the shape and duration of the incident pulses, we can control the intensity and time of the amplified radiation generation, as well as the population dynamics of the medium levels.
Resonant nonlinear-optical interference processes in four-level Doppler-broadened media are studied. Specific features of amplification and optical switching of short-wavelength radiation in a strongly-absorbing resonant gas under coherent quantum control with two longer wavelength radiations, are investigated. The major outcomes are illustrated with virtual experiments aimed at inversionless short-wavelength amplification, which also address deficiencies in this regard in recent experiments. With numerical simulations related to the proposed experiment in optically-dense sodium dimer vapor, we show optimal condition for optical switching and the expected gain of the probe radiation, which is above the oscillation threshold.
Nonlinear optics normally involves the change in the susceptibility of a material due to the presence of optical radiation. In many cases, the light-matter interaction produces a change in the refractive index of the medium, as occurs in photorefractive media, as well as in Kerr-like media, Brillouin-active media and absorbing media with thermallyinduced refractive index changes. Such nonlinear refractive index variation corresponds to a change in the real part of the optical susceptibility %. In resonant materials, the optical radiation induces stimulated emission (or absorption) causing transfer of population between different energy states of the medium. This can lead to saturation of the amplification (or absorption) corresponding to changes in the imaginary part of the susceptibility x= i2odk where the amplitude gain coefficient a(I) is a saturable function of the intensity /, and k is the magnitude of the wavevector of the optical radiation. The interference of two (or more) coherent beams I(x) in the laser amplifier can cause a modulation of the population inversion N(x). This modulation of the inversion is commonly known as spatial hole burning in lasers and leads to formation of a gain-grating a(x) = 1/2GN(X) where G is the stimulated emission cross-section. The gain grating can act as a very efficient diffractive optical element exhibiting high diffraction efficiency that may be even greater than unity [16] and also very high phase conjugate reflectivity using four-wave mixing (FWM) geometries [5-7].
We theoretically study the propagation through a resonant absorbing medium of a time-dependent perturbation modulating the amplitude of a continuous wave (cw). Modeling the medium as a two-level system and linearizing the Maxwell-Bloch equations for the perturbation, we establish an exact analytical expression of the transfer function relating the Fourier transforms of the incident and transmitted perturbations. It directly gives the gain and the phase shift undergone in the medium by a harmonic modulation. For the case of a pulse modulation, it enables us to determine the transmission time of the pulse center of mass (group delay), evidencing the relative contributions of the coherent and incoherent (population) relaxations. We show that the group delay has a negative value (fast light) fixed by the coherent effects when the cw intensity is small compared to the saturation intensity and becomes positive (slow light) when this intensity increases, before attaining a maximum that cannot exceed the population relaxation time. The analytical results are completed by numerical determinations of the shape of the transmitted pulses in the different regimes.