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CRC Press eBooks

Wave-mixing and Phase Conjugation in Laser Active Media

Kazuo Kuroda

Published Mar 14, 2002• 0 citations
Publisher

Abstract

Nonlinear optics normally involves the change in the susceptibility of a material due to the presence of optical radiation. In many cases, the light-matter interaction produces a change in the refractive index of the medium, as occurs in photorefractive media, as well as in Kerr-like media, Brillouin-active media and absorbing media with thermallyinduced refractive index changes. Such nonlinear refractive index variation corresponds to a change in the real part of the optical susceptibility %. In resonant materials, the optical radiation induces stimulated emission (or absorption) causing transfer of population between different energy states of the medium. This can lead to saturation of the amplification (or absorption) corresponding to changes in the imaginary part of the susceptibility x= i2odk where the amplitude gain coefficient a(I) is a saturable function of the intensity /, and k is the magnitude of the wavevector of the optical radiation. The interference of two (or more) coherent beams I(x) in the laser amplifier can cause a modulation of the population inversion N(x). This modulation of the inversion is commonly known as spatial hole burning in lasers and leads to formation of a gain-grating a(x) = 1/2GN(X) where G is the stimulated emission cross-section. The gain grating can act as a very efficient diffractive optical element exhibiting high diffraction efficiency that may be even greater than unity [16] and also very high phase conjugate reflectivity using four-wave mixing (FWM) geometries [5-7].

DOI
10.1201/9781482264951-13

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Nonlinear optics normally involves the change in the susceptibility of a material due to the presence of optical radiation. In many cases, the light-matter interaction produces a change in the refractive index of the medium, as occurs in photorefractive media, as well as in Kerr-like media, Brillouin-active media and absorbing media with thermallyinduced refractive index changes. Such nonlinear refractive index variation corresponds to a change in the real part of the optical susceptibility %. In resonant materials, the optical radiation induces stimulated emission (or absorption) causing transfer of population between different energy states of the medium. This can lead to saturation of the amplification (or absorption) corresponding to changes in the imaginary part of the susceptibility x= i2odk where the amplitude gain coefficient a(I) is a saturable function of the intensity /, and k is the magnitude of the wavevector of the optical radiation. The interference of two (or more) coherent beams I(x) in the laser amplifier can cause a modulation of the population inversion N(x). This modulation of the inversion is commonly known as spatial hole burning in lasers and leads to formation of a gain-grating a(x) = 1/2GN(X) where G is the stimulated emission cross-section. The gain grating can act as a very efficient diffractive optical element exhibiting high diffraction efficiency that may be even greater than unity [16] and also very high phase conjugate reflectivity using four-wave mixing (FWM) geometries [5-7].
Phase conjugal ion by degenerate four-wave mixing (DTVVM) in saturable gain media is a nonlinear process of major interest for applications to dynamic holography and phase-distortion correction of an optical wave propagating in laser media [1,2,3]. The use of laser amplifiers for such operations presents very attractive features including the automatic matching of the nonlinearity with the laser wavelength, a fast response time and a high efficiency of the nonlinear process due to the laser amplification of all interacting beams. This process is based on the possibility of writing dynamic gain gratings when interfering beams are propagating in a laser medium by gain saturation.
A calculation procedure and various large-signal and numerical solutions are presented for degenerate four-wave mixing in optical Kerr media, and for phase conjugate resonators using degenerate four-wave mixing. The solutions presented take full account of nonlinear refractive index changes, pump depletion, signal saturation, distributed losses, and possible external mirrors with laser gain. We find that including the nonlinear index change generally causes little change in the reflectivity or power output of degenerate four-wave mixing devices, at least with symmetric pumping. The optimum power output from a phase conjugate resonator with and without a laser gain medium is calculated. The results provide some theoretical guidance for designing phase conjugate resonators. PACS Code 42. 65. Bp; 42. 60. Da
A theory of degenerate four-wave mixing in absorbing media is developed in terms of a general nonlinear susceptibility. The predictions of the theory are examined in both high and low reflectivity regimes and the specific nonlinearity-inducing mechanisms of thermally induced refractive index changes, the Kerr effect, and saturable absorption are considered. Such a theory is of particular relevance to degenerate four-wave mixing experiments in the ultraviolet and the predictions of the theory are compared with results obtained from such experiments.
Phase distortion correction of an optical wave propagating in laser media is a crucial problem to be taken into account in most of laser systems. For this purpose, phase conjugation through stimulated Brillouin scattering using the master oscillator-power amplification configuration has shown a very good potential to obtain high beam quality in solid-state lasers that operate at variable repetition rates. Another attractive alternative to generate the phase-conjugate wavefronts is to use a four-wave mixing (DFWM) process in the laser amplifier. In this medium, the interference between the interacting beams leads to a spatial modulation of the complex susceptibility of the medium by gain saturation (amplitude gain grating). This all-solid-state solution presents the advantage of suppressing the external nonlinear medium and would realize the required functions in the laser medium itself. Moreover, due to the amplification experienced by all the interacting beams, associated to the resonant nonlinearity of the gain saturation, high reflectivities already have been achieved in Nd:YAG amplifiers using a multipass geometry.1,2
We have shown previously that two strong laser beams (with the same frequency) counterpropagating in a Kerr nonlinear medium with linear dispersion become un stable when their intensities exceed a certain threshold.1 We demonstrate here that the system exhibits large (theoretically unlimited) amplification of a probe beam when the two pumping beams have their intensities slightly below the threshold. This is in contrast to the conventional phase conjugation due to four-wave mixing in a nondispersive Kerr nonlinear medium. The mechanism of amplification in our system can be explained in terms of positive distributed feedback from the Kerr nonlinear index grating formed by two strong pumping laser beams in the presence of dispersion giving rise to a light-induced distributed-feedback resonator. This feedback is attributed to the fact that the weak beams with both signal frequency, ω + δ, and conjugate frequency, ω − δ, propagate with phase speed different (due to dispersion) from that of a pumping wave with frequency ω, which triggers the exponentially increasing energy exchange between weak and strong beams at the nonlinear index grating (this energy exchange is prohibited in nondispersive media). When the probe frequency approaches a frequency of one of the longitudinal modes of the light-induced distributed resonator, and the pumping intensity approaches the threshold of instability, the resonant amplification increases infinitely; for presently available laser intensity stabilities, amplification as large as 104 is feasible.
Optical phase conjugation is concerned with the use of nonlinear optical effects to precisely reverse the direction of propagation of each plane wave in an arbitrary beam of light. This causes the return beam to exactly retrace the path of the incident beam, leading to many applications of automatic pointing and tracking (even in the presence of an inhomogeneous medium). The main goals of this course are familiarization with how each of the many nonlinear optical effects gives rise to a phase conjugate signal, and understanding and appreciation of the many potential applications for optical phase conjugation. Conjugation techniques involving Kerr-like degenerate four-wave mixing, resonant degenerate four-wave mixing, stimulated Brillouin scattering, photorefractive effects, surface phenomena, and others will be carefully reviewed. Applications of particular importance to this course will include distortion correction, pointing, tracking, laser-resonator design, optical information processing, etc. Throughout the course, key references will be identified for those wishing to pursue any topic more vigorously.