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Doklady of the National Academy of Sciences of Belarus

Interaction of different-shape optical pulses with resonant amplifying media

Denis V. Novitsky

Published Jan 5, 2026• 0 citations
Publisher

Abstract

Using the numerical solution of the Maxwell–Bloch equations, we study the interaction of short light pulses with resonant amplifying media. We consider pulses of various shapes – with Gaussian, rectangular, and exponential envelopes, the latter of which has recently attracted increased attention due to its potential for implementing new effects such as virtual absorption. We show that by choosing the shape and duration of the incident pulses, we can control the intensity and time of the amplified radiation generation, as well as the population dynamics of the medium levels.

DOI
10.29235/1561-8323-2025-69-6-462-467

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Summary form only given. We study the interaction between intense (50 MW peak power), shaped ultrafast laser pulses and optically dense samples of Rb vapor. In particular, we concentrate our attention on laser pulses with a the complex hyperbolic secant envelope, or equivalently, a sech electric field envelope with a tanh frequency sweep. In order to produce and characterize the shaped laser pulses used in our experiments, we exploited several new technologies: amplified, shaped laser pulses were generated using an acousto-optic modulator-based system combined with a chirped-pulse regenerative amplifier. The amplitude and phase of these pulses were then characterized by the STRUT (spectrally and temporally resolved upconversion technique). The STRUT was used to measure the laser pulses both before and after propagating through Rb vapor. Examples of such experimental STRUT images are presented. The complex sech pulse was selected because, in optically thin media, only it and rectangular pulses give complete analytical solutions to the Bloch equations. This shape has been found to generate complete population inversion over a well-defined and amplitude-insensitive bandwidth. In optically dense samples the excited state dynamics are not so straightforward. We have found, both in experiments and theoretically, that the extent and character of the population inversion is related to the frequency sweep of the laser pulses as does the amount of residual excited population after the pulse and any subsequent stimulated emission.
The dynamics of pulses with durations comparable to the inverse transition frequency that propagate in an optical medium is studied in terms of two integrable systems of Maxwell-Bloch equations. The first model describes the field interaction with a nondegenerate medium with a permanent dipole moment and permanent external pumping. A general formula is derived for the N -soliton solution. Particular solutions are used as examples to investigate the effect of permanent dipole moment and pumping on the soliton dynamics. The second model describes the interaction between two-component electric-field pulses and a two-level degenerate medium with permanent upper-level pumping. For different initial magnetic-sublevel populations, soliton solutions are used as examples to show that pumping causes a change in polarization dynamics. A two-soliton solution is used to analyze the interaction of solitons in a two-level medium with external pumping.
Amplification of electromagnetic field pulses approximately one cycle in duration in multilevel media with an effective permanent dipole moment is studied theoretically without application of the approximation of slowly varying envelopes for the case of unidirectional propagation of the radiation. For three-level and quasi-two-level media, it is shown that the set of Maxwell-Schrödinger equations can be reduced to an integrable set of equations for an effective two-level medium. The presence of an (effective) permanent dipole moment of the medium was found to lead to new specific features of the amplification and control of the dynamics of field pulses.
We theoretically investigate the propagation of few-cycle laser pulses in resonant two-level dense media with a subwavelength structure, which is described by the full Maxwell—Bloch equations without the frame of slowly varying envelope and rotating wave approximations. The input pulses can be shaped into shorter ones with a single or less than one optical cycle. The effect of the parameters of the subwavelength structure and laser pulses is studied. Our study shows that the media with a subwavelength structure can significantly shape the few-cycle pulses into a subcycle pulse, even for the case of chirp pulses as input fields. This suggests that such subwavelength structures have potential application in the shaping of few-cycle laser pulses.
Abstract The interest in unipolar pulses in optics is related to the possibility of their efficient action on quantum objects. In this work, we study the interaction of a short rectangular unipolar pulse with a two-level resonant medium under conditions that the pulse duration is shorter than the relaxation times of the medium. It is paradoxical that the polarization and the population difference of the medium oscillate not at the Rabi frequency, but, rather, at a frequency that is proportional to the sum of the squared frequency of the resonant transition of the medium and the squared Rabi frequency of the pulse. This phenomenon is similar to the Stark effect, which consists of a shift of the transition frequencies of a medium in a constant external electric field. The possibility of generating radiation at frequencies that exceed the resonant transition frequency of the medium upon its excitation by a rectangular unipolar pulse is discussed.