Abstract Time-invariant photonic structures amplify or absorb light based on their intrinsic material gain or loss. The coherent interference of multiple beams in space, e.g., in a resonator, can be exploited to tailor the wave interaction with material gain or loss, respectively maximizing lasing or coherent perfect absorption. By contrast, a time-varying system is not bound to conserve energy, even in the absence of material gain or loss, and can support amplification or absorption of a probe wave through parametric phenomena. Here, we demonstrate theoretically and experimentally how a subwavelength film of indium tin oxide, whose bulk permittivity is homogeneously and periodically modulated via optical pumping, can be dynamically tuned to act both as a non-resonant amplifier and a perfect absorber, by manipulating the relative phase of two counterpropagating probe beams. This extends the concept of coherent perfect absorption to the temporal domain. We interpret this result as selective switching between the gain and loss modes present in the momentum bandgap of a periodically modulated medium. By tailoring the relative intensity of the two probes, high-contrast modulation can be achieved with up to 80% absorption and 400% amplification. Our results demonstrate control of gain and loss in time-varying media at optical frequencies and pave the way towards coherent manipulation of light in Floquet-engineered complex photonic systems.
Abstract Time-invariant photonic structures amplify or absorb light based on their intrinsic material gain or loss. The coherent interference of multiple beams in space, e.g., in a resonator, can be exploited to tailor the wave interaction with material gain or loss, respectively maximizing lasing or coherent perfect absorption. By contrast, a time-varying system is not bound to conserve energy, even in the absence of material gain or loss, and can support amplification or absorption of a probe wave through parametric phenomena. Here, we demonstrate theoretically and experimentally how a subwavelength film of indium tin oxide, whose bulk permittivity is homogeneously and periodically modulated via optical pumping, can be dynamically tuned to act both as a non-resonant amplifier and a perfect absorber, by manipulating the relative phase of two counterpropagating probe beams. This extends the concept of coherent perfect absorption to the temporal domain. We interpret this result as selective switching between the gain and loss modes present in the momentum bandgap of a periodically modulated medium. By tailoring the relative intensity of the two probes, high-contrast modulation can be achieved with up to 80% absorption and 400% amplification. Our results demonstrate control of gain and loss in time-varying media at optical frequencies and pave the way towards coherent manipulation of light in Floquet-engineered complex photonic systems.
In the time-reversed counterpart to laser emission, incident coherent optical fields are perfectly absorbed within a resonator that contains a loss medium instead of a gain medium. The incident fields and frequency must coincide with those of the corresponding laser with gain. We demonstrated this effect for two counterpropagating incident fields in a silicon cavity, showing that scattering [corrected] can be modulated [corrected] by two orders of magnitude, the maximum predicted by theory for our experimental setup. In addition, we showed that absorption can be reduced substantially by varying the relative phase of the incident fields. The device, termed a "coherent perfect absorber," functions as an absorptive interferometer, with potential practical applications in integrated optics.
The resonant absorption, emission, and scattering of light are the fundamental optical processes that have been used both to probe matter and to manipulate light itself. In the last decade there has been essential progress in coherent control of both linear and nonlinear optical responses based on resonant excitation of atomic coherence in multilevel quantum systems. Some interesting and useful phenomena, resulting from coherent control of absorption and the group index, such as electromagnetically induced transparency, lasing without inversion, and ultra-slow group velocity of light have been widely studied. This work is focused on coherent control of refractive index and resonant fluorescence in multilevel medium. \n \nWe suggest two promising schemes for resonant enhancement of the refractive index with eliminated absorption and propose their implementation in transition element doped crystals with excited state absorption and in a cell of Rb atoms at natural abundance. We show how to use one of these schemes for spatial variation of the refractive index via its periodic resonant increase/decrease, remarkably keeping at the same time zero absorption/gain. It opens the way to production of transparent photonic structures (such as distributed Bragg reflectors, holey fibers, or photonic crystals) in a homogeneous resonant atomic media such as dielectrics with homogeneously distributed impurities, atomic, or molecular gases. These optically produced photonic structures could easily be controlled (including switching on/off, changing amplitude and period of modulation) and would be highly selective in frequency, naturally limited by the width of the optical resonance. \n \nWe also derive the optical fluorescence spectra of a three-level medium driven by two coherent fields at the adjacent transitions in a general case when all three transitions are allowed. We show that coherent driving can efficiently control the distribution of intensities between the fluorescent channels. In particular, the total intensity of fluorescence at the transition which is not driven by the optical fields may essentially exceed the fluorescence intensity at the driven transitions under the condition of two-photon resonance. This counter-intuitive effect is due to depletion of the intermediate state via atomic interference.
Virtual gain refers to the simulation of real light amplification using radiation with exponentially decaying amplitude so that its complex frequency corresponds to the scattering pole. We study theoretically virtual gain in a two-level resonant medium for different regimes of light-matter interaction depending on the radiation intensity. We show that virtual gain at the pole can be most clearly observed for low intensities, when the medium is absorbing, in contrast to the saturated medium at high intensities. The efficiency of virtual gain can be tuned with the light intensity and controlled dynamically through the population inversion of the medium. Our results show that resonantly absorbing media paradoxically mimic a gainlike response, which admits a number of related phenomena and methods to mold both optical signals and material properties without relying on instability-prone gain media.
Achieving dynamic and broadband control of superradiance and subradiance at elevated temperatures is central to quantum photonic technologies. Herein, we theoretically investigate near-field photonics combined with adiabatic and non-adiabatic time-varying media—created via temporal modulation of material properties—to dynamically generate and coherently manipulate quantum emission states, including single photons and photon pairs. Distinctively, this cavity-free near-field method operates effectively at practical temperatures (tens of Kelvin), circumventing traditional operational constraints. We initiate this approach by exploiting plasmonically coupled silicon carbide color centers, which are used as quantum emitters (QEs), with relatively long coherence lifetimes, enabling precise quantum state control before temperature-induced dephasing sets in. In particular, a hybrid plasmonic waveguide is used as the light delivery method, where its subdiffracted near-field generates nanoscale heating that effectively tunes the energies of color centers, via phonon occupation, on resonance with the near-field. Furthermore, we employ transparent conducting oxides, such as indium tin oxide, that may achieve significant refractive index modulation on the femto–picosecond timescales. The resulting behavior is that of a photonic time crystal (PTC) or an epsilon-near-zero (ENZ) material response, dependent on modulation times, and characterized by the amplification or increased absorption of light, respectively, where both enhance field localization around the embedded QEs and extend periods of super- or subradiance compared to static conditions. Our methodology significantly simplifies scalable quantum photonic integration, while advancing quantum memories and entanglement capabilities under accessible conditions.
High-performance non-reciprocal photonic devices can improve the efficiency of optical quantum manipulation, information processing, and quantum simulation effectively. The enhanced optical signal can simultaneously amplify the weak signal output by the quantum system and isolate the sensitive quantum system from the back-scattered external noise, which is the core technology of high-performance photonic devices. In our previous work ( 2023 Opt. Express 31 38228 ), we have achieved dynamic control of unidirectional reflection amplification based on four-wave mixing gain and the use of coupling field intensity varying linearly with position. In this work, we design a simple three-level closed loop coherent gain atomic system, setting the intensity of coupling field to be varying with position step shape to break the spatial symmetry of probe susceptibility, and achieving perfect non-reciprocal reflection light amplification. In contrast, the stepped variation of coupling field intensity is easier to adjust in experiment, greatly reducing the difficulty in the experiment. Specifically, the system introduces phase modulation. By changing the phase, the frequency region of probe gain and absorption can be switched, which makes the modulation of reflection amplification more flexible.
Virtual perfect absorption (VPA) is an effect simulating real absorption of light by using excitation at a complex frequency corresponding to a scattering zero. We theoretically study VPA in resonantly absorbing and amplifying media irradiated by two counterpropagating waves with exponentially growing amplitudes. We show that VPA critically depends on the medium density (i.e., level of loss or gain) deteriorating in the high-density limit. In contrast, almost ideal VPA persists in the PT-symmetric loss-gain bilayer. For high enough gain, powerful quasilasing pulses are observed at later times symmetrically (single amplifying layer) or asymmetrically (PT-symmetric structure) generated in both propagation directions.