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arXiv:2112.00122

In situ control of integrated Kerr nonlinearity

Chaohan Cui, Liang Zhang, Linran Fan

Published Nov 30, 2021• 0 citations
arXivHTMLPDF

Abstract

Kerr nonlinearity in nanophotonic cavities provides a versatile platform to explore fundamental physical sciences and develop novel photonic technologies. This is driven by the precise dispersion control and significant field enhancement with nanoscale structures. Beyond dispersion and pump engineering, the direct control of Kerr nonlinearity can release the ultimate performance and functionality of photonic systems. Here, we report the in situ control of integrated Kerr nonlinearity through its interplay with the cascaded Pockels nonlinear process. Kerr nonlinearity is tuned over 10~dB dynamic range without modifying photonic structures. Fano resonance is observed with nonlinear spectrum, in contrast to standard linear transmission. This confirms the quantum interference between competing optical nonlinear pathways. Besides nonlinearity enhancement, we also demonstrate the novel capability to suppress the material intrinsic nonlinearity. Finally, we use the tunable nonlinearity to control the spectral brightness and coincidence-to-accidental ratio of single-photon generation. This work paves the way towards the complete nanoscale control of optical nonlinear processes at quantum level.

DOI
10.48550/arxiv.2112.00122

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Kerr nonlinearity in nanophotonic cavities provides a versatile platform to explore fundamental physical sciences and develop novel photonic technologies. This is driven by the precise dispersion control and significant field enhancement with nanoscale structures. Beyond dispersion and pump engineering, the direct control of Kerr nonlinearity can release the ultimate performance and functionality of photonic systems. Here, we report the in situ control of integrated Kerr nonlinearity through its interplay with the cascaded Pockels nonlinear process. Kerr nonlinearity is tuned over 10~dB dynamic range without modifying photonic structures. Fano resonance is observed with nonlinear spectrum, in contrast to standard linear transmission. This confirms the quantum interference between competing optical nonlinear pathways. Besides nonlinearity enhancement, we also demonstrate the novel capability to suppress the material intrinsic nonlinearity. Finally, we use the tunable nonlinearity to control the spectral brightness and coincidence-to-accidental ratio of single-photon generation. This work paves the way towards the complete nanoscale control of optical nonlinear processes at quantum level.
The enhancement of the optical nonlinear effects at nanoscale is important in the on-chip optical information processing. We theoretically propose the mechanism of the great Kerr nonlinearity enhancement by using anisotropic Purcell factors in a double-Λ type four-level system, i.e., if the bisector of the two vertical dipole moments lies in the small/large Purcell factor axis in the space, the Kerr nonlinearity will be enhanced/decreased due to the spontaneously generated coherence accordingly. Besides, when the two dipole moments are parallel, the extremely large Kerr nonlinearity increase appears, which comes from the double population trapping. Using the custom-designed resonant plasmonic nanostructure which gives an anisotropic Purcell factor environment, we demonstrate the effective nanoscale control of the Kerr nonlinearity. Such controllable Kerr nonlinearity may be realized by the state-of-the-art nanotechnics and it may have potential applications in on-chip photonic nonlinear devices.
We present a study on manipulation and enhancement of multiphoton bundles emission under a moderate atom-cavity coupling, by constructing a two-photon Jaynes-Cummings model integrated with Kerr nonlinearity in a single atom-cavity system. We show that the vacuum-Rabi splittings for the n th dressed states can be significantly enhanced by Kerr interaction. This remarkable enhancement in energy-spectrum anharmonicity with the well-resolved multiphoton resonance facilitates the generation of special nonclassical states beyond the strong-coupling limit in the experiment. In particular, both two- and three-photon blockades are observed with adjusting the amplitude of the cavity-driving or atom-pump fields. Moreover, we discover that transitions between two- and three-photon bundles can be achieved through tuning the atom-cavity detuning or Kerr nonlinearity. It further showcases the three-photon blockade is substantially strengthened when both the cavity and atomic fields are jointly driven. Our proposal unveils a pathway for realizing highly controllable nonclassical states and quantum devices with combining two-photon Jaynes-Cummings interactions and Kerr nonlinearity, which may pave the way for versatile applications in quantum information science, e.g., all-optical switches and transistors. Published by the American Physical Society 2024
The enhancement of the optical nonlinear effects at nanoscale is important in the on-chip optical information processing. We theoretically propose the mechanism of the great Kerr nonlinearity enhancement by using anisotropic Purcell factors in a double-Λ type four-level system, i.e., if the bisector of the two vertical dipole moments lies in the small/large Purcell factor axis in the space, the Kerr nonlinearity will be enhanced/decreased due to the spontaneously generated coherence accordingly. Besides, when the two dipole moments are parallel, the extremely large Kerr nonlinearity increase appears, which comes from the double population trapping. Using the custom-designed resonant plasmonic nanostructure which gives an anisotropic Purcell factor environment, we demonstrate the effective nanoscale control of the Kerr nonlinearity. Such controllable Kerr nonlinearity may be realized by the state-of-the-art nanotechnics and it may have potential applications in on-chip photonic nonlinear devices.
Nonlinearity is a key resource in both classical and quantum signal processing. Nonlinear nanomechanical elements have found applications ranging from sensing to computing, while networks of nonlinear resonators, as well as nonlinearly coupled networks of linear resonators, constitute promising platforms for simulating complex dynamics. Here, we experimentally demonstrate an approach to realizing strong mechanical nonlinearity in nanomechanical resonators, fully controlled through optical laser drives. The mechanism exploits the nonlinearity of the radiation-pressure interaction in a cavity optomechanical system, which gives rise to a nonlinear optical spring effect. The resulting Duffing nonlinearity is conveniently tunable in strength via pump laser power, while its sign is controlled by laser detuning. Moreover, we demonstrate that the nonlinear optical spring mediates effective interactions between mechanical modes coupled to a common cavity, inducing tunable nonlinear interactions between them that impact spectral response and dynamics. These results establish cavity optomechanics as a versatile and in-situ reconfigurable platform for engineering nonlinear dynamics in resonators and networks.
Quantum nanophotonics merges the precision of nanoscale light manipulation with the capabilities of quantum technologies, offering a pathway for enhanced light-matter interaction and compact realization of quantum devices. Here, we show how a recently-demonstrated nonlinear nanophotonic process can be employed to selectively create photonic high-dimensional quantum states (qudits). We utilize the nonlinearity on the surface of the nanophotonic device to dress, through the polarization of the pump field, the near-field modes carrying angular momentum and their superpositions. This idea is an important step towards experimental realizations of quantum state generation and manipulation through nonlinearity within nanophotonic platforms, and enables new capabilities for on-chip quantum devices.