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arXiv:2503.04508 · Light Science & Applications

Nonlinear nanophotonics for high-dimensional quantum states

Liat Nemirovsky-Levy, Amit Kam, Meir Lederman, Meir Orenstein, Uzi Pereg, Guy Bartal, Mordechai Segev

Published Jan 29, 2026• 9 citations
arXivHTMLPDF

Abstract

Quantum nanophotonics merges the precision of nanoscale light manipulation with the capabilities of quantum technologies, offering a pathway for enhanced light-matter interaction and compact realization of quantum devices. Here, we show how a recently-demonstrated nonlinear nanophotonic process can be employed to selectively create photonic high-dimensional quantum states (qudits). We utilize the nonlinearity on the surface of the nanophotonic device to dress, through the polarization of the pump field, the near-field modes carrying angular momentum and their superpositions. This idea is an important step towards experimental realizations of quantum state generation and manipulation through nonlinearity within nanophotonic platforms, and enables new capabilities for on-chip quantum devices.

DOI
10.1038/s41377-025-02179-0

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Abstract Quantum nanophotonics offers essential tools and technologies for controlling quantum states, while maintaining a miniature form factor and high scalability. Nanophotonic platforms can transfer information from the traditional degrees of freedom (DoFs) of photons, such as spin angular momentum (SAM) and orbital angular momentum (OAM), to the DoFs of the nanophotonic platform—and back, opening new directions for quantum information processing. Recent experiments have utilized, for entanglement the total angular momentum (TAM) of a photon—as a unique DoF of nanophotonic platforms—for demonstrating entanglement in TAM. Here, we unravel the morphing of quantum states of heralded single photons as they couple into and out of the near-field of a nanophotonic system. Through quantum state tomography, we discover that the TAM state of the near-field transforms to a free-space entangled state within a larger Hilbert space of SAM and OAM. Furthermore, we show that this entangled single photon state is in fact a quantum optical Stokes skyrmion with a topological invariant of ±2\pm 2±2 ± 2 . The concepts described here bring new ideas and methodologies in developing high-dimensional quantum circuitry on a chip.
Abstract High-dimensional quantum entanglement is an important resource for emerging quantum technologies such as quantum communication and quantum computation. The scalability of metres-long experimental setups limits high-dimensional entanglement in bulk optics. Advancements in quantum technology hinge on reproducible, and reconfigurable quantum devices—including photon sources, which are challenging to achieve in a scalable manner using bulk optics. Advances in nanotechnology and CMOS-compatible integration techniques have enabled the generation of entangled photons on millimeter-scale chips, significantly enhancing scalability, stability, replicability, and miniaturization for real-world quantum applications. In recent years we have seen several chip-scale demonstrations with different discrete degrees of freedom including path, frequency-bin, time-bin, and transverse modes, on many material platforms. A complete quantum photonic integrated circuit requires the generation, manipulation, and detection of quantum states, involving various active and passive quantum photonic components which further increase the degree of complexity. Here, we focus on the high-dimensional versions of qubits—qudits—and review the nonlinear optical processes that facilitate on-chip high-dimensional entangled photon sources, and the currently used material platforms. We discuss a range of current implementations of on-chip high-dimensional entangled photon sources and demonstrated applications. We comment on the current challenges due to the limitations of individual material platforms and present future opportunities in hybrid and heterogeneous integration strategies for the next generation of integrated quantum photonic chips.
At the quantum limit of nonlinear optics, where single photons interact with individual emitters, new phenomena are found. One-dimensional, subwavelength waveguides have recently emerged as a promising quantum optical platform capable of both guiding and confining photons, leading to efficient light-matter interactions and enhancing quantum optical nonlinearities. We explore this regime using both single organic molecules and epitaxially grown quantum dots coupled to nanoscale waveguides. In the first case, two-color experiments allow us to observe distinctly quantum nonlinearities such as Stark shifts of the molecular resonances or amplification without population inversion, although we are limited by relatively weak molecule-waveguide coupling. In contrast, quantum dots can be nearly perfectly coupled to waveguides, allowing us to demonstrate optical nonlinearities at the true single photon level. These, as we discuss, can be used as a basis for novel on-chip quantum technologies.