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arXiv:1906.08565 · Nanophotonics

Coherent nonlinear optics of quantum emitters in nanophotonic waveguides

Pierre Türschmann, Hanna Le Jeannic, Signe F. Simonsen, Harald R. Haakh, Stephan Götzinger, Vahid Sandoghdar, Peter Lodahl, Nir Rotenberg

Published Jun 1, 2018• 71 citations
arXivHTMLPDF

Abstract

Abstract Coherent quantum optics, where the phase of a photon is not scrambled as it interacts with an emitter, lies at the heart of many quantum optical effects and emerging technologies. Solid‐state emitters coupled to nanophotonic waveguides are a promising platform for quantum devices, as this element can be integrated into complex photonic chips. Yet, preserving the full coherence properties of the coupled emitter‐waveguide system is challenging because of the complex and dynamic electromagnetic landscape found in the solid state. Here, we review progress toward coherent light‐matter interactions with solid‐state quantum emitters coupled to nanophotonic waveguides. We first lay down the theoretical foundation for coherent and nonlinear light‐matter interactions of a two‐level system in a quasi‐one‐dimensional system, and then benchmark experimental realizations. We discuss higher order nonlinearities that arise as a result of the addition of photons of different frequencies, more complex energy level schemes of the emitters, and the coupling of multiple emitters via a shared photonic mode. Throughout, we highlight protocols for applications and novel effects that are based on these coherent interactions, the steps taken toward their realization, and the challenges that remain to be overcome.

DOI
10.1515/nanoph-2019-0126

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Abstract Coherent quantum optics, where the phase of a photon is not scrambled as it interacts with an emitter, lies at the heart of many quantum optical effects and emerging technologies. Solid‐state emitters coupled to nanophotonic waveguides are a promising platform for quantum devices, as this element can be integrated into complex photonic chips. Yet, preserving the full coherence properties of the coupled emitter‐waveguide system is challenging because of the complex and dynamic electromagnetic landscape found in the solid state. Here, we review progress toward coherent light‐matter interactions with solid‐state quantum emitters coupled to nanophotonic waveguides. We first lay down the theoretical foundation for coherent and nonlinear light‐matter interactions of a two‐level system in a quasi‐one‐dimensional system, and then benchmark experimental realizations. We discuss higher order nonlinearities that arise as a result of the addition of photons of different frequencies, more complex energy level schemes of the emitters, and the coupling of multiple emitters via a shared photonic mode. Throughout, we highlight protocols for applications and novel effects that are based on these coherent interactions, the steps taken toward their realization, and the challenges that remain to be overcome.
Controlling light photon-by-photon is central to quantum optics. At a fundamental level, photon interactions are mediated by their coupling to atoms, and ultimate control requires deterministic light-matter interfacing of single photons to single atoms. Extending this paradigm to radiatively couple multiple individual atoms in a deterministic and scalable manner opens the arena of many-body quantum optics. Here, we realize such a setting by coherently coupling solid-state artificial atoms to a nanophotonic waveguide and demonstrate higher-order photon correlations that are controlled by the number of quantum emitters. We study the scaling of nonlinear photonic transport induced by emitter-photon scattering and demonstrate that adding a quantum emitter generates higher-order photon correlations. Specifically, we experimentally observe genuine three-photon correlations from a pair of collectively coupled emitters, while contributions from lower photon numbers are suppressed. In addition, we scale to three resonant quantum emitters coupled to the waveguide. These advancements demonstrate the onset of many-body quantum optics in waveguide quantum electrodynamics, enabling new photonic quantum simulators, the creation of many-body entangled states, and the exploration of novel quantum phase transitions.
Abstract Single photons constitute a main platform in quantum science and technology: they carry quantum information over extended distances in the future quantum internet1 and can be manipulated in advanced photonic circuits enabling scalable photonic quantum computing. The main challenge in quantum photonics is how to generate advanced entangled resource states and efficient light-matter interfaces offer a path way. Here we utilize the efficient and coherent coupling of a single quantum emitter to a nanophotonic waveguide for realizing quantum nonlinear interaction between single-photon wavepackets. This inherently multimode quantum system constitutes a new research frontier in quantum optics. We demonstrate control of a photon with another photon and experimentally unravel the dynamical response of two-photon interactions mediated by a quantum emitter, and show that the induced quantum correlations are controlled by the pulse duration. The work will open new avenues for tailoring complex photonic quantum resource states.
Coherent interactions between quantum emitters in tailored photonic structures is a fundamental building block for future quantum technologies, but remains challenging to observe in complex solid-state environments, where the role of decoherence must be considered. Here, we investigate the optical interaction between two quantum emitters mediated by one-dimensional waveguides in a realistic solid-state environment, focusing on the creation, population, and detection of a subradiant state, in the presence of dephasing. We show that as dephasing increases, the signatures of subradiance quickly vanish in intensity measurements, yet remain pronounced in photon correlation measurements, particularly when the two emitters are pumped separately so as to populate the subradiant state efficiently. The applied Green's tensor approach is used to model a photonic crystal waveguide, including the dependence on the spatial position of the integrated emitter. The work lays out a route to the experimental realization of subradiant states in nanophotonic waveguides containing solid-state emitters.
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Coherent photon-emitter interfaces offer a way to mediate efficient nonlinear photon-photon interactions, much needed for quantum information processing. Here we experimentally study the case of a two-level emitter, a quantum dot, coupled to a single optical mode in a nanophotonic waveguide. We carry out few-photon transport experiments and record the statistics of the light to reconstruct the scattering matrix elements of one- and two-photon components. This provides direct insight to the complex nonlinear photon interaction that contains rich many-body physics.