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arXiv:2605.18289

Strong nanomechanical Duffing nonlinearity and interactions induced through cavity optomechanics

Jesse J. Slim, Ewold Verhagen

cond-mat.mes-hallphysics.opticsquant-phSubmitted May 18, 2026• Announced May 19, 2026
arXivHTMLPDF

Abstract

Nonlinearity is a key resource in both classical and quantum signal processing. Nonlinear nanomechanical elements have found applications ranging from sensing to computing, while networks of nonlinear resonators, as well as nonlinearly coupled networks of linear resonators, constitute promising platforms for simulating complex dynamics. Here, we experimentally demonstrate an approach to realizing strong mechanical nonlinearity in nanomechanical resonators, fully controlled through optical laser drives. The mechanism exploits the nonlinearity of the radiation-pressure interaction in a cavity optomechanical system, which gives rise to a nonlinear optical spring effect. The resulting Duffing nonlinearity is conveniently tunable in strength via pump laser power, while its sign is controlled by laser detuning. Moreover, we demonstrate that the nonlinear optical spring mediates effective interactions between mechanical modes coupled to a common cavity, inducing tunable nonlinear interactions between them that impact spectral response and dynamics. These results establish cavity optomechanics as a versatile and in-situ reconfigurable platform for engineering nonlinear dynamics in resonators and networks.

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Nonlinearity is a key resource in both classical and quantum signal processing. Nonlinear nanomechanical elements have found applications ranging from sensing to computing, while networks of nonlinear resonators, as well as nonlinearly coupled networks of linear resonators, constitute promising platforms for simulating complex dynamics. Here, we experimentally demonstrate an approach to realizing strong mechanical nonlinearity in nanomechanical resonators, fully controlled through optical laser drives. The mechanism exploits the nonlinearity of the radiation-pressure interaction in a cavity optomechanical system, which gives rise to a nonlinear optical spring effect. The resulting Duffing nonlinearity is conveniently tunable in strength via pump laser power, while its sign is controlled by laser detuning. Moreover, we demonstrate that the nonlinear optical spring mediates effective interactions between mechanical modes coupled to a common cavity, inducing tunable nonlinear interactions between them that impact spectral response and dynamics. These results establish cavity optomechanics as a versatile and in-situ reconfigurable platform for engineering nonlinear dynamics in resonators and networks.
The nonlinearity is essential for creation of non-classical states of the cavity or mechanical resonator such as squeezed or cat states. A microwave cavity can be made nonlinear by, for instance, adding Josephson junctions. The mechanical resonator is inherently nonlinear. The radiation pressure interaction between cavity and mechanical resonator is also inherently nonlinear but typically under strong drive of the cavity interaction can be linearized. However, if the optomechanical system is in the strong coupling regime nonlinear quantum effects become observable. These three cases provide the motivation for our studies. We start with backaction analysis of the classical regime of a dc SQUID (superconducting quantum interference device) with an embedded mechanical resonator. Then, we perform quantum analysis to understand how the asymmetry of two Josephson junctions influences the coupling strength of optomechanical interactions such as radiation pressure, cross-Kerr and single-photon beam splitter. Using variational method and self-consistent harmonic approximation we estimate the influence of the radiation pressure coupling and Kerr nonlinearity of the cavity on the effective frequency and dissipation of the cavity. The second part of this thesis focuses on the nonlinearity of the mechanical resonator coupled to the optical/microwave cavity. We study in details the nonlinear optomechanical response and draw the response map to summarize all results of the overcoupled and undercoupled cavity for the red and blue sidebands additionally to the weak and strong drive powers. In the end, w e confirm the developed theory by using it to numerically fit the experimental results.
The quantum nonlinear regime of optomechanics is reached when nonlinear effects of the radiation pressure interaction are observed at the single-photon level. This requires couplings larger than the mechanical frequency and cavity-damping rate, and is difficult to achieve experimentally. Here we show how to exponentially enhance the single-photon optomechanical coupling strength using only additional linear resources. Our method is based on using a large-amplitude, strongly detuned mechanical parametric drive to amplify mechanical zero-point fluctuations and hence enhance the radiation pressure interaction. It has the further benefit of allowing time-dependent control, enabling pulsed schemes. For a two-cavity optomechanical set-up, we show that our scheme generates photon blockade for experimentally accessible parameters, and even makes the production of photonic states with negative Wigner functions possible. We discuss how our method is an example of a more general strategy for enhancing boson-mediated two-particle interactions and nonlinearities.
In this dissertation, I theoretically investigate the open system dynamics of cavity optomechanical systems in the quantum limit, where a mechanical resonator couples to a cavity mode via radiation pressure force. Recent developments in nano-fabrication and cooling techniques make it possible to optically control and manipulate the motion of micro- and nano-mechanical resonator. Several experiments have demonstrated the possibility of preparing macroscopic mechanical resonators into their quantum ground state, which makes optomechanical systems an ideal candidate for studying the quantum behavior of macroscopic objects. One important direction in quantum optomechanics is the study of the decoherence of optomechanical system due to the interaction with their external environments. This dissertation explores the decoherence effects by considering the influence of the radiation pressure coupling on the interaction between optomechanical system and its environments. Because the effects of the nonlinear interaction vary with the optomechanical coupling strength, three different interaction regimes are fully studied here: the weak coupling, the intermediate coupling and the strong coupling.
Cavity optomechanics represents a flexible platform for the implementation of quantum technologies, useful in particular for the realization of quantum interfaces, quantum sensors and quantum information processing. However, the dispersive, radiation-pressure interaction between the mechanical and the electromagnetic modes is typically very weak, harnessing up to now the demonstration of interesting nonlinear dynamics and quantum control at the single photon level. It has already been shown both theoretically and experimentally that if the interaction is mediated by a Josephson circuit, one can have an effective dynamics corresponding to a huge enhancement of the single-photon optomechanical coupling. Here we analyze in detail this phenomenon in the general case when the cavity mode and the mechanical mode interact via an off-resonant qubit. Using a Schrieffer-Wolff approximation treatment, we determine the regime where this tripartite hybrid system behaves as an effective cavity optomechanical system in the strong coupling regime.
The nonlinear quantum regime is crucial for implementing interesting quantum effects, which have wide applications in modern quantum science. Here we propose an effective method to reach the nonlinear quantum regime in a modulated optomechanical system (OMS), which is originally in the weak-coupling regime. The mechanical spring constant and optomechanical interaction are modulated periodically. This leads to the result that the resonant optomechanical interaction can be effectively enhanced into the single-photon strong-coupling regime by the modulation-induced mechanical parametric amplification. Moreover, the amplified phonon noise can be suppressed completely by introducing a squeezed vacuum reservoir, which ultimately leads to the realization of photon blockade in a weakly coupled OMS. The reached nonlinear quantum regime also allows us to engineer the nonclassical states (e.g., Schr\"odinger cat states) of the cavity field, which are robust against the phonon noise. This work offers an alternative approach to enhance the quantum nonlinearity of an OMS, which should expand the applications of cavity optomechanics in the quantum realm.
Controlling the interaction between localized optical and mechanical excitations is now possible following advances in micro- and nano-fabrication techniques. To date, most experimental studies of optomechanics have focused on measurement and control of the mechanical subsystem through its interaction with optics, and have led to the experimental demonstration of dynamical back-action cooling and optical rigidity of the mechanical system. However, the optical response of these systems is also modified in the presence of mechanical interactions, leading to effects such as Electromagnetically Induced Transparency (EIT) and parametric normal-mode splitting, and thus a platform for strongly nonlinear optics. In this talk we propose and demonstrate the use of the optomechanical nonlinearity as a new way of controlling the velocity of light via engineered photon-phonon interactions. Our results demonstrate EIT and tunable optical delays on a nanoscale optomechanical crystal device, fabricated by simply etching holes into a thin film of Silicon. At low temperature (8.7 K), we show an optically-tunable delay of 50 ns with near-unity optical transparency, and superluminal light with a 1.4 μs signal advance. These results, while indicating significant progress towards an integrated quantum optomechanical memory, are also relevant to classical signal processing applications.