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arXiv:2107.09147 · Journal of Physics Condensed Matter

Making high-quality quantum microwave devices with van der Waals superconductors

Abhinandan Antony, M. Gustafsson, Anjaly Rajendran, Avishai Benyamini, Guilhem J. Ribeill, Thomas Ohki, James Hone, Kin Chung Fong

Published Nov 30, 2021• 6 citations
arXivHTMLPDF

Abstract

Abstract Ultra low-loss microwave materials are crucial for enhancing quantum coherence and scalability of superconducting qubits. Van der Waals (vdW) heterostructure is an attractive platform for quantum devices due to the single-crystal structure of the constituent two-dimensional (2D) layered materials and the lack of dangling bonds at their atomically sharp interfaces. However, new fabrication and characterization techniques are required to determine whether these structures can achieve low loss in the microwave regime. Here we report the fabrication of superconducting microwave resonators using NbSe2 that achieve a quality factor Q > 105. This value sets an upper bound that corresponds to a resistance of ⩽ 192 μ Ω when considering the additional loss introduced by integrating NbSe2 into a standard transmon circuit. This work demonstrates the compatibility of 2D layered materials with high-quality microwave quantum devices.

DOI
10.1088/1361-648x/ac3e9d

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Abstract Ultra low-loss microwave materials are crucial for enhancing quantum coherence and scalability of superconducting qubits. Van der Waals (vdW) heterostructure is an attractive platform for quantum devices due to the single-crystal structure of the constituent two-dimensional (2D) layered materials and the lack of dangling bonds at their atomically sharp interfaces. However, new fabrication and characterization techniques are required to determine whether these structures can achieve low loss in the microwave regime. Here we report the fabrication of superconducting microwave resonators using NbSe2 that achieve a quality factor Q > 105. This value sets an upper bound that corresponds to a resistance of ⩽ 192 μ Ω when considering the additional loss introduced by integrating NbSe2 into a standard transmon circuit. This work demonstrates the compatibility of 2D layered materials with high-quality microwave quantum devices.
High-quality, single-crystal van der Waals (vdW) materials provide a promising platform for constructing Josephson junctions, but systematic studies have been limited by fabrication and measurement challenges. Here researchers characterize 24 vertical vdW superconductor-semiconductor junctions, including microwave spectroscopy of an all-vdW transmon qubit. Transport measurements reveal a crossover from proximity- to tunneling-type behavior with increasing semiconductor thickness. The results demonstrate how band alignment and materials engineering can be used to tailor qubit properties, establishing vdW heterostructures as an emerging platform for next-generation superconducting qubits.
State-of-the-art superconducting qubits rely on a limited set of thin-film materials. Expanding their materials palette can improve performance, extend operating regimes, and introduce new functionalities, but conventional thin-film fabrication hinders systematic exploration of new material combinations. Van der Waals (vdW) materials offer a highly modular crystalline platform that facilitates such exploration while enabling gate-tunability, higher-temperature operation, and compact qubit geometries. Yet it remains unknown whether a fully vdW superconducting qubit can support quantum coherence and what mechanisms dominate loss at both low and elevated temperatures in such a device. Here we demonstrate quantum-coherent merged-element transmons made entirely from vdW Josephson junctions. These first-generation, fully crystalline qubits achieve microsecond lifetimes in an ultra-compact footprint without external shunt capacitors. Energy relaxation measurements, together with microwave characterization of vdW capacitors, point to dielectric loss as the dominant relaxation channel up to hundreds of millikelvin. These results establish vdW materials as a viable platform for compact superconducting quantum devices.
Advances in solid-state physics, materials science, and device engineering have accelerated the development of superconducting qubits. Among emerging platforms, van der Waals (vdW) materials and their heterostructures are potentially attractive building blocks for quantum devices, yet their realization in qubit architectures remains largely underexplored. Here we report an all-vdW superconducting qubit based on a NbSe2_22​-hBN-NbSe2_22​ junction, in which a thin hBN layer simultaneously provides Josephson coupling and capacitive shunting between two NbSe2_22​ islands, forming a "merged-element" transmon. Temporal characterization using circuit quantum electrodynamics (cQED) techniques yields an average energy-relaxation time T1,avg=55 μsT_{1,\mathrm{avg}} = 55 ~μsT1,avg​=55 μs, Hahn-echo coherence time T2E,avg=21 μsT_{2\mathrm{E},\mathrm{avg}} = 21 ~μsT2E,avg​=21 μs, and Ramsey coherence time T2R,avg=1.9 μsT_{2\mathrm{R},\mathrm{avg}} = 1.9~μsT2R,avg​=1.9 μs. The relatively low Ramsey time is primarily attributable to an enhanced sensitivity to charge noise consistent with the realized device parameters and not a fundamental limitation. These results show that lumped-element superconducting qubits based on vdW heterostructures can achieve coherence times comparable to those of conventional Al-AlOx_\mathrm{x}x​-Al qubits, while offering a reduced device footprint and suppressed stray capacitive coupling.
High Resolution Image Download MS PowerPoint Slide The advent of two-dimensional van der Waals materials is a frontier of condensed matter physics and quantum devices. However, characterizing such materials remains challenging due to the limitations of bulk material techniques, necessitating the development of specialized methods. Here, we investigate the superconducting properties of Bi 2 Sr 2 CaCu 2 O 8+ x flakes by integrating them with a hybrid superconducting microwave resonator. The hybrid resonator is significantly modified by the interaction with the flake while maintaining a high quality factor (3 × 10 4 ). We also observe a significant upshift of the resonator frequency with increasing temperature, as well as a positive nonlinearity. These effects originate from a presently unknown microscopic mechanism within the flake, and can be modeled as a two-level system bath interacting with the resonant mode. Our findings open a path for high quality hybrid circuits with van der Waals flakes for exploring novel materials and developing new devices for quantum technology.
Abstract Quantum computers can potentially achieve an exponential speedup versus classical computers on certain computational tasks, recently demonstrated in superconducting qubit processors. However, the capacitor electrodes that comprise these qubits must be large in order to avoid lossy dielectrics. This tactic hinders scaling by increasing parasitic coupling among circuit components, degrading individual qubit addressability, and limiting the spatial density of qubits. Here, we take advantage of the unique properties of van der Waals (vdW) materials to reduce the qubit area by >1000 times while preserving the capacitance while maintaining quantum coherence. Our qubits combine conventional aluminum-based Josephson junctions with parallel-plate capacitors composed of crystalline layers of superconducting niobium diselenide and insulating hexagonal boron nitride. We measure a vdW transmon T1 relaxation time of 1.06 μs, demonstrating a path to achieve high-qubit-density quantum processors with long coherence times, and the broad utility of layered heterostructures in low-loss, high-coherence quantum devices.
Silicon-germanium (SiGe) is a material that possesses a multitude of applications ranging from transistors to electro-optical modulators and quantum dots. The diverse properties of SiGe also make it attractive to implementations involving superconducting quantum computing. Here, we demonstrate the fabrication of transmon quantum bits on SiGe layers and investigate the microwave loss properties of SiGe at cryogenic temperatures and single photon microwave powers. We find relaxation times of up to 100 μs, corresponding to a quality factor Q above 4 M for large pad transmons. The high Q values obtained indicate that the SiGe/Si heterostructure is compatible with state-of-the-art performance of superconducting quantum circuits.