Exploring van der Waals Cuprate Superconductors Using a Hybrid Microwave Circuit
Haolin Jin, Giuseppe Serpico, Yejin Lee, Tommaso Confalone, Christian N. Saggau, Flavia Lo Sardo, Genda D. Gu, Berit Hansen Goodge, Edouard Lesne, Domenico Montemurro, Kornelius Nielsch, Nicola Poccia, Uri Vool
High Resolution Image Download MS PowerPoint Slide The advent of two-dimensional van der Waals materials is a frontier of condensed matter physics and quantum devices. However, characterizing such materials remains challenging due to the limitations of bulk material techniques, necessitating the development of specialized methods. Here, we investigate the superconducting properties of Bi 2 Sr 2 CaCu 2 O 8+ x flakes by integrating them with a hybrid superconducting microwave resonator. The hybrid resonator is significantly modified by the interaction with the flake while maintaining a high quality factor (3 × 10 4 ). We also observe a significant upshift of the resonator frequency with increasing temperature, as well as a positive nonlinearity. These effects originate from a presently unknown microscopic mechanism within the flake, and can be modeled as a two-level system bath interacting with the resonant mode. Our findings open a path for high quality hybrid circuits with van der Waals flakes for exploring novel materials and developing new devices for quantum technology.
High Resolution Image Download MS PowerPoint Slide The advent of two-dimensional van der Waals materials is a frontier of condensed matter physics and quantum devices. However, characterizing such materials remains challenging due to the limitations of bulk material techniques, necessitating the development of specialized methods. Here, we investigate the superconducting properties of Bi 2 Sr 2 CaCu 2 O 8+ x flakes by integrating them with a hybrid superconducting microwave resonator. The hybrid resonator is significantly modified by the interaction with the flake while maintaining a high quality factor (3 × 10 4 ). We also observe a significant upshift of the resonator frequency with increasing temperature, as well as a positive nonlinearity. These effects originate from a presently unknown microscopic mechanism within the flake, and can be modeled as a two-level system bath interacting with the resonant mode. Our findings open a path for high quality hybrid circuits with van der Waals flakes for exploring novel materials and developing new devices for quantum technology.
Abstract Ultra low-loss microwave materials are crucial for enhancing quantum coherence and scalability of superconducting qubits. Van der Waals (vdW) heterostructure is an attractive platform for quantum devices due to the single-crystal structure of the constituent two-dimensional (2D) layered materials and the lack of dangling bonds at their atomically sharp interfaces. However, new fabrication and characterization techniques are required to determine whether these structures can achieve low loss in the microwave regime. Here we report the fabrication of superconducting microwave resonators using NbSe2 that achieve a quality factor Q > 105. This value sets an upper bound that corresponds to a resistance of ⩽ 192 μ Ω when considering the additional loss introduced by integrating NbSe2 into a standard transmon circuit. This work demonstrates the compatibility of 2D layered materials with high-quality microwave quantum devices.
The high critical magnetic field and relatively high critical temperature of niobium nitride (NbN) make it a promising material for applications in superconducting quantum technology. However, NbN-based superconducting circuits are sensitive to decoherence sources such as two-level system (TLS) defects. Here, we numerically and experimentally investigate NbN superconducting microwave coplanar waveguide resonator arrays with a 100 nm thickness, capacitively coupled to a common coplanar waveguide on a silicon chip. We observe that the resonators' internal quality factor (Qi) decreases fromQi∼1.07×106in a high power regime toQi∼1.36×105in the single photon regime. Data from this study is consistent with the TLS theory, which describes the TLS interactions in resonator substrates and interfaces. Moreover, we study the temperature (T) dependence ofQiand resonance frequencyfrof coplanar waveguide resonators to characterize the quasiparticle density. We observe that the increase in kinetic inductance at higher temperatures is the main reason for the frequency shift. Finally, we measurefrandQiin response to in-plane magnetic fields (B∣∣). We verify thatQistays well above104up toB∣∣= 240 mT in the photon number<nph>= 1.8 atT= 100 mK. Our results could enable the development of robust microwave superconducting circuits for circuit quantum electrodynamics at high magnetic fields required for hybrid superconducting-semiconducting quantum circuits.
Flux-tunable transmon incorporating a van der Waals superconductor via an Al/AlOx/4Hb-TaS2 Josephson junction
Incorporating van der Waals (vdW) superconductors into Josephson elements extends circuit-QED beyond conventional Al/AlOx/Al tunnel junctions and enables microwave probes of unconventional condensates and subgap excitations. In this work, we realize a flux-tunable transmon whose nonlinear inductive element is an Al/AlOx/4Hb-TaS2 Josephson junction. The tunnel barrier is formed by sequential deposition and full in-situ oxidation of ultrathin Al layers on an exfoliated 4Hb-TaS2 flake, followed by deposition of a top Al electrode, yielding a robust, repeatable hybrid junction process compatible with standard transmon fabrication. Embedding the device in a three-dimensional copper cavity, we observe a SQUID-like flux-dependent spectrum that is quantitatively reproduced by a standard dressed transmon--cavity Hamiltonian, from which we extract parameters in the transmon regime. Across measured devices we obtain sub-microsecond energy relaxation (T1 from 0.08 to 0.69μs), while Ramsey measurements indicate dephasing faster than our 16 ns time resolution. We also find a pronounced discrepancy between the Josephson energy inferred from spectroscopy and that expected from the Ambegaokar--Baratoff relation using room-temperature junction resistances, pointing to nontrivial junction physics in the hybrid Al/AlOx/4Hb-TaS2 system. Although we do not resolve material-specific subgap modes in the present geometry, this work establishes a practical route to integrating 4Hb-TaS2 into coherent quantum circuits and provides a baseline for future edge-sensitive designs aimed at enhancing coupling to boundary and subgap degrees of freedom in vdW superconductors.
Hybrid quantum systems with high-Tc superconducting resonators
Superconducting microwave resonators are crucial elements of microwave circuits, offering a wide range of potential applications in modern science and technology. While conventional low-T[Formula: see text] superconductors are mainly employed, high-T[Formula: see text] cuprates could offer enhanced temperature and magnetic field operating ranges. Here, we report the realization of [Formula: see text] superconducting coplanar waveguide resonators, and demonstrate a continuous evolution from a lossy undercoupled regime, to a lossless overcoupled regime by adjusting the device geometry, in good agreement with circuit model theory. A high-quality factor resonator was then used to perform electron spin resonance measurements on a molecular spin ensemble across a temperature range spanning two decades. We observe spin-cavity hybridization indicating coherent coupling between the microwave field and the spins in a highly cooperative regime. The temperature dependence of the Rabi splitting and the spin relaxation time point toward an antiferromagnetic coupling of the spins below 2 K. Our findings indicate that high-Tc superconducting resonators hold great promise for the development of functional circuits. Additionally, they suggest novel approaches for achieving hybrid quantum systems based on high-T[Formula: see text] superconductors and for conducting electron spin resonance measurements over a wide range of magnetic fields and temperatures.
Abstract We fabricated Josephson junctions with two-dimensional (2D) non-superconducting Bi 2 Sr 2 CaCu 2 O 8+δ (Bi-2212) crystal flakes between Nb film. We provide a solution to get clean non-superconducting Bi-2212 flakes from optimal doping, and develop a fabrication process to make such Nb/Bi-2212 flakes/Nb Josephson heterostructures. A good Fraunhofer-like critical current modulation under magnetic fields could be observed where the shape of the junction area has been taken into account, indicating a relatively homogeneous supercurrent profile through junction. Fractional Shapiro steps could be observed, suggesting some unconventional properties in such a structure. Hopefully, the potential value for novel electronic devices like the Josephson transistor will be seen in this kind of junctions. Our work has led to the development of a novel quantum device based on the two-dimensional material BSCCO, paving the way for next-generation superconducting integrated circuits utilizing 2D materials.
Hybrid quantum systems play an essential role in efforts towards the advancements of quantum information technology and quantum sensing by bridging distinct technological platforms. In particular, hybrid systems comprising superconducting microwave circuits are being pursued intensely in light of existing achievements in superconducting qubits and precise quantum control in microwave circuits. Their realization relies on the design of superconducting resonators capable of coupling to an oscillatory mode of a second quantum system, facilitating the probing and manipulation of one via the other. In order to accommodate the coupled system, its particular constraints and requirements must be respected, which may be quite extreme from the perspective of established superconducting circuit design and operation. Overcoming this challenge has proved to be a substantial obstacle for the attainment of strongly coupled hybrid systems, despite spectacular advances in superconducting microwave circuits individually. In this work, we examine two approaches tackling this issue for different hybrid quantum systems, focusing on the optimization and characterization of the superconducting circuits. The first device aims at a superconductor-atom hybrid system through the coupling to Rydberg-Rydberg transitions in ultra-cold Rb-87 atoms trapped near the superconducting chip. Using simulations in conjunction with theoretical considerations, we demonstrate a comprehensive geometry parameter optimization procedure for maximum coupling rate. Presenting an experimental implementation of the resulting circuit, we validate its suitability for use under the intended operation conditions, including the option of tuning the electronic transition frequencies using a dc voltage. Secondly, we investigate a device designed for applications in large magnetic in-plane fields used to mediate coupling to integrated micromechanical oscillators; more specifically it is a flux-tunable SQUID resonator comprising Josephson nano-constrictions as nonlinear inductive components. Performing a thorough characterization of its frequency and Kerr anharmonicity tuning behavior at fields up to several hundred mT, we discover a pronounced asymmetry in its flux response at large fields. We show this asymmetry to be caused by the nano-constrictions turning into Josephson diodes, develop an intuitive macroscopic model for its field-induced emergence and reconstruct the diode current-phase relation from the flux tuning data. Several figures of merit informing the suitability of the SQUID resonators for optomechanical systems as well as other applications are improved by the diode effect, highlighting the potential of Josephson diodes in superconducting microwave circuits. Our results provide a promising stepping stone for the advancement of hybrid systems involving superconducting microwave circuits, putting new and exciting operation and coupling regimes within reach.