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arXiv:2106.10208 · Optics Letters

Fiber-based biphoton source with ultrabroad frequency tunability

Santiago Lopez-Huidobro, Markus Lippl, Nicolas Y. Joly, Maria V. Chekhova

Published Jul 19, 2021• 10 citations
arXivHTMLPDF

Abstract

Tunable biphotons are highly important for a wide range of quantum applications. For some applications, especially interesting are cases where two photons of a pair are far apart in frequency. Here, we report a tunable biphoton source based on a xenon-filled hollow-core photonic crystal fiber. Tunability is achieved by adjusting the pressure of the gas inside the fiber. This allows us to tailor the dispersion landscape of the fiber, overcoming the principal limitations of solid-core fiber-based biphoton sources. We report a maximum tunability of 120 THz for a pressure range of 4 bar with a continuous shift of 30 THz/bar. At 21 bar, the photons of a pair are separated by more than one octave. Despite the large separation, both photons have large bandwidths. At 17 bar, they form a very broad (110 THz) band around the frequency of the pump.

DOI
10.1364/ol.434434

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Tunable biphotons are highly important for a wide range of quantum applications. For some applications, especially interesting are cases where two photons of a pair are far apart in frequency. Here, we report a tunable biphoton source based on a xenon-filled hollow-core photonic crystal fiber. Tunability is achieved by adjusting the pressure of the gas inside the fiber. This allows us to tailor the dispersion landscape of the fiber, overcoming the principal limitations of solid-core fiber-based biphoton sources. We report a maximum tunability of 120 THz for a pressure range of 4 bar with a continuous shift of 30 THz/bar. At 21 bar, the photons of a pair are separated by more than one octave. Despite the large separation, both photons have large bandwidths. At 17 bar, they form a very broad (110 THz) band around the frequency of the pump.
Nowadays fiber biphoton sources are nearly as popular as crystal-based ones. They offer a single spatial mode and easy integrability into optical networks. However, fiber sources lack the broad tunability of crystals, which do not require a tunable pump. Here, we report a broadly tunable biphoton source based on a suspended core fiber. This is achieved by introducing pressurized gas into the fibers hollow channels, changing the step index. The mechanism circumvents the need for a tunable pump laser, making this a broadly tunable fiber biphoton source with a convenient tuning mechanism, comparable to crystals. We report a continuous shift of 0.30 THz/bar of the sidebands, using up to 25 bar of argon.
Pairs of entangled photons-biphotons-are indispensable in quantum applications. However, some important spectral ranges, like the ultraviolet, have been inaccessible to them so far. Here, we use four-wave mixing in a xenon-filled single-ring photonic crystal fiber to generate biphotons with one of the photons in the ultraviolet and its entangled partner in the infrared spectral range. We tune the biphotons in frequency by varying the gas pressure inside the fiber and thus tailoring the fiber dispersion landscape. The ultraviolet photons are tunable from 271 nm to 231 nm and their entangled partners, from 764 nm to 1500 nm, respectively. Tunability up to 192 THz is achieved by adjusting the gas pressure by only 0.68 bar. At 1.43 bar, the photons of a pair are separated by more than 2 octaves. The access to ultraviolet wavelengths opens the possibility for spectroscopy and sensing with undetected photons in this spectral range.
Photon pairs (biphotons) are ubiquitous in quantum technologies. In particular, in quantum imaging and spectroscopy they enable measurements in hard-to-access spectral ranges [1] and increased sensitivity [2] . Among different sources of biphotons, four-wave mixing (FWM) in optical fibers is most efficient due to the large nonlinear interaction lengths and easy integrability into optical networks. However, fiber sources are usually not tuneable except by tuning the pump wavelength. Hollow-core photonic crystals fibers (PCF) filled by noble gas solve this problem: their dispersion landscape can be tailored by simply changing the gas pressure [3] , [4] . Additionally, they are free from Raman scattering and have a higher damage threshold than solid-core fibers [4] .
Raman-scattering noise in silica has been the key obstacle toward the realisation of high quality fiber-based photon-pair sources. Here, we experimentally demonstrate how to get past this limitation by dispersion tailoring a xenon-filled hollow-core photonic crystal fiber. The source operates at room temperature, and is designed to generate Raman-free photon-pairs at useful wavelength ranges, with idler in the telecom, and signal in the visible range. We achieve a coincidence-to-accidentals ratio as high as 2740 combined with an ultra low heralded second order coherence [Formula: see text], indicating a very high signal to noise ratio and a negligible multi-photon emission probability. Moreover, by gas-pressure tuning, we demonstrate the control of photon frequencies over a range as large as 13 THz, covering S-C and L telecom band for the idler photon. This work demonstrates that hollow-core photonic crystal fiber is an excellent platform to design high quality photon-pair sources, and could play a driving role in the emerging quantum technology.
In this Letter, we report a first, to the best of our knoqledge, experimental realization of a bright ultra-broadband (180 THz) fiber-based biphoton source with widely spectrally separated signal and idler photons. Such a two-photon source is realized due to the joint use of a broadband two-loop phase-matching of interacting light waves and high optical nonlinearity of a silica-core photonic crystal fiber. The high performance of the developed fiber source identifies it as an important and useful tool for a wide range of optical quantum applications.