The desire to understand the interaction between light and matter has stimulated centuries of research, leading to technological achievements that have shaped our world. One contemporary frontier of research into light-matter interaction considers regimes where quantum effects dominate. By understanding and manipulating these quantum effects, a vast array of new quantum-enhanced technologies become accessible. In this thesis, I explore and analyze fundamental components and processes for quantum optical devices with a focus on solid-state quantum systems. This includes indistinguishable single-photon sources, deterministic sources of entangled photonic states, photon-heralded entanglement generation between remote quantum systems, and deterministic optically-mediated entangling gates between local quantum systems. For this analysis, I make heavy use of an analytic quantum trajectories approach applied to a general Markovian master equation of an optically-active quantum system, which I introduce as a photon-number decomposition. This approach allows for many realistic system imperfections, such as emitter pure dephasing, spin decoherence, and measurement imperfections, to be taken into account in a straightforward and comprehensive way.
The desire to understand the interaction between light and matter has stimulated centuries of research, leading to technological achievements that have shaped our world. One contemporary frontier of research into light-matter interaction considers regimes where quantum effects dominate. By understanding and manipulating these quantum effects, a vast array of new quantum-enhanced technologies become accessible. In this thesis, I explore and analyze fundamental components and processes for quantum optical devices with a focus on solid-state quantum systems. This includes indistinguishable single-photon sources, deterministic sources of entangled photonic states, photon-heralded entanglement generation between remote quantum systems, and deterministic optically-mediated entangling gates between local quantum systems. For this analysis, I make heavy use of an analytic quantum trajectories approach applied to a general Markovian master equation of an optically-active quantum system, which I introduce as a photon-number decomposition. This approach allows for many realistic system imperfections, such as emitter pure dephasing, spin decoherence, and measurement imperfections, to be taken into account in a straightforward and comprehensive way.
In this paper, exciting progress of quantum optics in solid state is reviewed. The focus is on semiconductor microcavities with self-assembled quantum dots embedded in the active layer. Due to enormous progress in semiconductor nanotechnology, such photonic structures have become a model system for the study of quantum optics on a scalable and integrable technology platform with high potential for future applications in quantum information technology. Quantum optical phenomena have become accessible due to 3-D confinement of light and matter on the length scale of their wavelength in state-of-the-art semiconductor micro- and nanostructures. This confinement leads to a quantization of the associated photonic and electronic energy levels and requires a quantum mechanical description of the system in the framework of cavity quantum electrodynamics (cQED). This approach considers the dipole interaction between two-level quantum emitters and discrete photonic states of a microcavity. Within the well-known Jaynes-Cummings model, the dipole interaction is described in terms of a coherent exchange of energy between the emitter and the resonator mode. This coherent interaction in the so-called strong coupling regime of cQED is reflected in a normal mode splitting, the vacuum Rabi splitting, of the involved modes and represents a central feature of quantum optics in solid state. Another important example of quantum optics in semiconductor nanostructures is the generation of nonclassical light in specific quantum devices. Of particular interest is the realization of Fock states which represent states containing a well-defined number of photons. Single-photon sources, for instance, allow for the generation of single photons on demand, which is highly desirable for quantum communication systems. In this context, this review paper will present recent experimental studies of quantum optics in solid state. This paper is meant for readers who would like to become familiar with this topic and for experts being interested in the progress in this field. It will cover a broad range of studies ranging from examples of fundamental light-matter interaction in the quantum limit to devices capable of emitting single photons and entangled photon pairs on demand.
Quantum computing and quantum information processing are fast developing fields. As more and more qubits are integrated into the quantum computing systems, a deeper understanding and more careful modeling of the dynamics of these quantum systems in presence of driving and/or loss are necessary, not only for optimizing existing quantum devices, but also for designing and achieving novel method for more precise manipulation of these quantum systems. Our work investigating these quantum systems is inspired by quantum optics, a field focused on the quantum description of light and light-matter interactions. In this thesis, we use the theoretical toolboxes provided by quantum optics as well as condensed matter theory to investigate and model realistic quantum systems. Specifically, we focus on the Nitrogen-vacancy centers in diamond crystal, a Josephson parametric amplifier (that uses Josephson junctions as its non-linear elements), and plasmonic nanowire system. With the knowledge of the dynamics of these systems, we proposed single-photon heralded two-NV center quantum gates; designed and optimized the superconducting circuit for a Josephson parametric amplifier to improve the amplifier's saturation power; and designed new methods for robust light manipulation using topologically protected plasmonic modes. All the devices that we study are either ready to be implemented in experiments or have already been built. Further, as discussed in this thesis, our theoretical analysis of NV-centers can be extended to similar device types like solid-state defect centers, while our analysis of Josephson parametric amplifiers can be extended to other types of superconducting circuit systems.
In this thesis we have focused on the study of various systems which are presently widely studied in different areas of quantum optics and quantum information sciences. These, for example, include the coupled system of photonic waveguides which are known to be highly efficient in manipulating the flow of light. The Hamiltonian describing the evolution of field mode in coupled waveguides is effectively identical to the well-known tight binding Hamiltonian used in solid state physics. The advantage of waveguide system is the possibility to control various interactions by design and their low decoherence rate. The excellent stability offered by coupled waveguides has led to the observation of many key coherent effects such as quantum walk, Bloch oscillation, and discrete Talbot effect. For example, Bloch oscillations have been investigated in coupled waveguides using coherent beam of light. We wanted to inquire whether coherent phenomena such as Bloch oscillations can be possible with incoherent single photon sources. We discovered that Bloch oscillations are indeed possible with single photons provided we prepare single photons in a W state. Moreover, coupled waveguides also find applications in the field of quantum information processing. Since entanglement plays a prominent role in all these applications, it is important to understand the entanglement dynamics in these structures. We considered the case of squeezed input in one of the waveguide and showed that one can generate entanglement between the waveguide modes. We further continued our work on the entanglement generation in coupled waveguides by incorporating the effect of loss in the waveguide structure for the squeezed and photon number input states. We considered relevant experimental parameters and showed that waveguide structures are reasonably robust against the effect of loss. Another system which has attracted a great deal of interest is the optomechanical system. We consider an optomechanical system where an optical cavity mode is coupled to the square of the position of a mechanical oscillator. The optomechanical system can then be regarded as a quantum optical spring, i.e., a spring whose spring constant depends on the quantum state of another system. In particular, we consider the situation where the field inside the cavity is in a coherent state and the oscillator is prepared in its ground state. The quantized nature of the field produces new features in the optomechanical system.
Nonlinear photonics studies situations in which light passing through a material can be used to create, reshape, or convert other light in ways that are not possible in ordinary optical systems. In recent years, this has become especially important for quantum photonics, where carefully prepared states of light are used as resources for emerging technologies such as secure communication, ultra-precise measurement, and new forms of information processing. A major challenge, however, is that these effects are delicate, difficult to control, and highly sensitive to the imperfections that arise when trying to build practical devices on a chip. This thesis examines how such nonlinear quantum-optical processes can be both engineered more deliberately and modelled more realistically, with the broader goal of helping move quantum photonic technology from proof-of-principle laboratory demonstrations toward robust and scalable implementation. To do this, the thesis first places nonlinear quantum photonics in a broader technological context and explains the main physical ideas needed to understand how quantum states of light are generated, transformed, and measured. It then develops this picture through a set of concrete examples. These include a method for generating quantum light on a chip while avoiding one of the field’s standard fabrication steps, a proposed chip-scale device that could help connect otherwise incompatible quantum systems by changing the colour and spectral width of light, and a modelling framework that links quantum theory directly to realistic fabricated waveguides, including common imperfections such as loss, non-uniformity, and writing errors. The thesis also reviews a wider class of design methods in which the nonlinear properties of a material are deliberately patterned in order to tailor the light produced. Taken together, the central message is that progress in quantum photonics will depend not only on discovering new effects, but on learning how to design, fabricate, and model these devices in ways that make them practical outside idealized laboratory conditions.
Quantum optics, the study of light at the level of its building blocks, \nhas been one of the frontiers of science. The arena of quantum optics \nhas been fruitful for investigations of a wide range of interesting questions, \nfrom those on the fundamental structures in driven dissipative \nsystems to those on applications of quantum information processing \nand quantum communication. \nThe first part of this thesis is concerned with one of the holy grails \nof quantum optics: an efficient transfer of energy (coupling) between \nsingle photons and matter degrees of freedom. From a certain point \nof view, the problem of efficient coupling is purely geometrical. The \nefficiency of coupling between an atom and light is difficult because \nit is difficult to shape the wavefunction of a single photon such \nthat it overlaps perfectly with the matter degree of freedom (emitter). \nThe first contribution of this thesis is addressing this issue by considering \nan emitter which perfectly matches the single photon plane-wave. \nMoreover, luckily, such an emitter is already realized in nature in the \nform of a two-dimensional crystal. We show that a new generation \nof two-dimensional semiconductors, transition metal dichalcogenide \n(TMD) monolayers, have especially favorable characteristics for allowing \nhighly efficient coupling between photons and matter degrees \nof freedom. \nOne of the most important goals in realizing an efficient coupling \nbetween photons and matter degrees of freedom is that unlike photons, \nmatter excitations interact with each other. Hence, if we would \nlike to have photons which act as if they interact, one possible way \nis to first convert them into matter excitations, and then transfer the \ncorrelations due matter interactions back to photons. As the second \ncontribution of this thesis, we demonstrate that TMD monolayers placed \nwithin a cavity can help us create photons which avoid each other \nas if they interact. The effect can be simply understood as the TMD \nmonolayer acting as a filter for photons, such that it only allows the \npassage of one photon at a time. \nBesides being the fundamental building block of light, photons also \nserve as mediators of interactions between charged particles. In a \nsense, two positive charges repel each other because there is always \na photon which lets them know that they are close to one another. \nOn the other hand, systems of many interacting particles behave in \na completely different way then when they are alone. It may even be \nargued that all physical phenomena at some level emerge from the \nbehavior of many interacting constituents. Given this point of view, \nit is crucial to find ways to control photons in order to control the \ninteractions that they mediate between matter degrees of freedom. \nAs the third contribution of this thesis, we analyze an experimental \nscheme where the control of photonic degrees of freedom can allow \nan experimentalist to modify the strength and range of interactions \nbetween matter. In particular, we propose squeezed photon states as \na resource to control such interactions. \nThe second part of this thesis is concerned with the emergent phenomena \narising in a system of many interacting particles. In particular, \nthe fourth contribution of this thesis considers the combination \nof two fascinating phenomena which emerges such condensed matter \nsystems: superconductivity and geometric effects in lattice band \nstructures. Separately, both superconductivity and the non-trivial geometrical \neffects in lattice systems are well-established subfields of condensed \nmatter physics. Yet only more recently, the combination of \nthese two phenomena were investigated in the context of topological \nsuperconductors, as well as other superconducting states which emerge \non top of band structures with non-trivial geometry. In our study, \nwe attempt at clarifying one of the ways that the non-trivial geometry \nassociated with the lattice band structure may affect the dynamics of \nan emergent superconducting state. Surprisingly, our analysis shows \nthat one of the most robust characteristics of the superconductor, vortices \nenclosing a quantum of magnetic flux, can be modified due to \ngeometrical effects.
This thesis is concerned with finding technologically useful quantum phenomena that are robust against real world imperfections. We examine three different areas covering techniques for spin measurement, photon preparation and error correction. The first research chapter presents a robust spin-measurement procedure, using an amplification approach: the state of the spin is propagated over a two-dimensional array to a point where it can be measured using standard macroscopic state mea- surement techniques. Even in the presence of decoherence, our two-dimensional scheme allows a linear growth in the total spin polarisation - an important increase over the √t obtainable in one-dimension. The work is an example of how simple propagation rules can lead to predictable macroscopic behaviour and the techniques should be applicable in other state propagation schemes. The next chapter is concerned with strategies for obtaining a robust and reliable single photon source. Using a microscopic model of electron-phonon interactions and a quantum master equation, we examine phonon-induced decoherence and assess its impact on the rate of production, and indistinguishability, of single photons emitted from an optically driven quantum dot system. We find that, above a certain threshold of desired indistinguishability, it is possible to mitigate the deleterious effects of phonons by exploiting a three-level Raman process for photon production. We introduce a master equation technique for quantum jump situations that should have wide application in other situations. The final chapter focusses on toric error correcting codes. Toric codes form part of the class of surface codes that have attracted a lot of attention due to their ability to tolerate a high level of errors, using only local operations. We investigate the power of small scale toric codes and determine the minimum size of code necessary for a first experimental demonstration of toric coding power.