Quantum optics, the study of light at the level of its building blocks, \nhas been one of the frontiers of science. The arena of quantum optics \nhas been fruitful for investigations of a wide range of interesting questions, \nfrom those on the fundamental structures in driven dissipative \nsystems to those on applications of quantum information processing \nand quantum communication. \nThe first part of this thesis is concerned with one of the holy grails \nof quantum optics: an efficient transfer of energy (coupling) between \nsingle photons and matter degrees of freedom. From a certain point \nof view, the problem of efficient coupling is purely geometrical. The \nefficiency of coupling between an atom and light is difficult because \nit is difficult to shape the wavefunction of a single photon such \nthat it overlaps perfectly with the matter degree of freedom (emitter). \nThe first contribution of this thesis is addressing this issue by considering \nan emitter which perfectly matches the single photon plane-wave. \nMoreover, luckily, such an emitter is already realized in nature in the \nform of a two-dimensional crystal. We show that a new generation \nof two-dimensional semiconductors, transition metal dichalcogenide \n(TMD) monolayers, have especially favorable characteristics for allowing \nhighly efficient coupling between photons and matter degrees \nof freedom. \nOne of the most important goals in realizing an efficient coupling \nbetween photons and matter degrees of freedom is that unlike photons, \nmatter excitations interact with each other. Hence, if we would \nlike to have photons which act as if they interact, one possible way \nis to first convert them into matter excitations, and then transfer the \ncorrelations due matter interactions back to photons. As the second \ncontribution of this thesis, we demonstrate that TMD monolayers placed \nwithin a cavity can help us create photons which avoid each other \nas if they interact. The effect can be simply understood as the TMD \nmonolayer acting as a filter for photons, such that it only allows the \npassage of one photon at a time. \nBesides being the fundamental building block of light, photons also \nserve as mediators of interactions between charged particles. In a \nsense, two positive charges repel each other because there is always \na photon which lets them know that they are close to one another. \nOn the other hand, systems of many interacting particles behave in \na completely different way then when they are alone. It may even be \nargued that all physical phenomena at some level emerge from the \nbehavior of many interacting constituents. Given this point of view, \nit is crucial to find ways to control photons in order to control the \ninteractions that they mediate between matter degrees of freedom. \nAs the third contribution of this thesis, we analyze an experimental \nscheme where the control of photonic degrees of freedom can allow \nan experimentalist to modify the strength and range of interactions \nbetween matter. In particular, we propose squeezed photon states as \na resource to control such interactions. \nThe second part of this thesis is concerned with the emergent phenomena \narising in a system of many interacting particles. In particular, \nthe fourth contribution of this thesis considers the combination \nof two fascinating phenomena which emerges such condensed matter \nsystems: superconductivity and geometric effects in lattice band \nstructures. Separately, both superconductivity and the non-trivial geometrical \neffects in lattice systems are well-established subfields of condensed \nmatter physics. Yet only more recently, the combination of \nthese two phenomena were investigated in the context of topological \nsuperconductors, as well as other superconducting states which emerge \non top of band structures with non-trivial geometry. In our study, \nwe attempt at clarifying one of the ways that the non-trivial geometry \nassociated with the lattice band structure may affect the dynamics of \nan emergent superconducting state. Surprisingly, our analysis shows \nthat one of the most robust characteristics of the superconductor, vortices \nenclosing a quantum of magnetic flux, can be modified due to \ngeometrical effects.
Quantum optics, the study of light at the level of its building blocks, \nhas been one of the frontiers of science. The arena of quantum optics \nhas been fruitful for investigations of a wide range of interesting questions, \nfrom those on the fundamental structures in driven dissipative \nsystems to those on applications of quantum information processing \nand quantum communication. \nThe first part of this thesis is concerned with one of the holy grails \nof quantum optics: an efficient transfer of energy (coupling) between \nsingle photons and matter degrees of freedom. From a certain point \nof view, the problem of efficient coupling is purely geometrical. The \nefficiency of coupling between an atom and light is difficult because \nit is difficult to shape the wavefunction of a single photon such \nthat it overlaps perfectly with the matter degree of freedom (emitter). \nThe first contribution of this thesis is addressing this issue by considering \nan emitter which perfectly matches the single photon plane-wave. \nMoreover, luckily, such an emitter is already realized in nature in the \nform of a two-dimensional crystal. We show that a new generation \nof two-dimensional semiconductors, transition metal dichalcogenide \n(TMD) monolayers, have especially favorable characteristics for allowing \nhighly efficient coupling between photons and matter degrees \nof freedom. \nOne of the most important goals in realizing an efficient coupling \nbetween photons and matter degrees of freedom is that unlike photons, \nmatter excitations interact with each other. Hence, if we would \nlike to have photons which act as if they interact, one possible way \nis to first convert them into matter excitations, and then transfer the \ncorrelations due matter interactions back to photons. As the second \ncontribution of this thesis, we demonstrate that TMD monolayers placed \nwithin a cavity can help us create photons which avoid each other \nas if they interact. The effect can be simply understood as the TMD \nmonolayer acting as a filter for photons, such that it only allows the \npassage of one photon at a time. \nBesides being the fundamental building block of light, photons also \nserve as mediators of interactions between charged particles. In a \nsense, two positive charges repel each other because there is always \na photon which lets them know that they are close to one another. \nOn the other hand, systems of many interacting particles behave in \na completely different way then when they are alone. It may even be \nargued that all physical phenomena at some level emerge from the \nbehavior of many interacting constituents. Given this point of view, \nit is crucial to find ways to control photons in order to control the \ninteractions that they mediate between matter degrees of freedom. \nAs the third contribution of this thesis, we analyze an experimental \nscheme where the control of photonic degrees of freedom can allow \nan experimentalist to modify the strength and range of interactions \nbetween matter. In particular, we propose squeezed photon states as \na resource to control such interactions. \nThe second part of this thesis is concerned with the emergent phenomena \narising in a system of many interacting particles. In particular, \nthe fourth contribution of this thesis considers the combination \nof two fascinating phenomena which emerges such condensed matter \nsystems: superconductivity and geometric effects in lattice band \nstructures. Separately, both superconductivity and the non-trivial geometrical \neffects in lattice systems are well-established subfields of condensed \nmatter physics. Yet only more recently, the combination of \nthese two phenomena were investigated in the context of topological \nsuperconductors, as well as other superconducting states which emerge \non top of band structures with non-trivial geometry. In our study, \nwe attempt at clarifying one of the ways that the non-trivial geometry \nassociated with the lattice band structure may affect the dynamics of \nan emergent superconducting state. Surprisingly, our analysis shows \nthat one of the most robust characteristics of the superconductor, vortices \nenclosing a quantum of magnetic flux, can be modified due to \ngeometrical effects.
This established textbook provides an accessible but comprehensive introduction to the quantum nature of light and its interaction with matter. The field of quantum optics is covered with clarity and depth, from the underlying theoretical framework of field quantization, atom–field interactions, and quantum coherence theory, to important and modern applications at the forefront of current research such as quantum interferometry, squeezed light, quantum entanglement, cavity quantum electrodynamics, laser-cooled trapped ions, and quantum information processing. The text is suitable for advanced undergraduate and graduate students and would be an ideal main text for a course on quantum optics. This long-awaited second edition builds upon the success of the first edition, including many new developments in the field, particularly in the area of quantum state engineering. Additional homework problems have been added, and content from the first edition has been updated and clarified throughout.
Superconducting circuits are a powerful platform for studying and controlling the interaction between light and matter at the quantum level. In these systems, superconducting qubits act as artificial atoms (with matter-like degrees of freedom), whereas microwave resonators play the role of oscillators hosting photons (with photonic-like degrees of freedom). A major advantage of this platform is the ability to tailor the electromagnetic environment to which the qubits are coupled. This degree of control makes it possible to realize well-known quantum optics models, like the Jaynes-Cummings model, as well as more complex systems, like quantum electrodynamics close to a bandgap. In this thesis, we engineer structured electromagnetic environments and couple superconducting qubits to them to experimentally study their interaction. By coupling multiple microwave resonators together, we create a metamaterial. When an atom interacts with the metamaterial, an atom-photon bound state emerges. We observe the dynamics of the creation and dissolution of the atom-photon bound state, as well as the spectral content of its photonic component, for the first time to our knowledge.Our metamaterial is intrinsically nonlinear because each resonator is formed by an array of Josephson junctions to serve as an inductor. When the system is pumped, its phase diagram exhibits multimode dissipative phase transitions with timescales on the order of hundred seconds. There is ongoing theoretical debate about whether such phase transitions can occur in one-dimensional systems, a question we address and resolve in this work.Furthermore, we engineer qubit decay using two different approaches. In the first one, we engineer the decay of two coupled atoms to two waveguides by using a symmetric–antisymmetric coupling configuration. This approach enables selective coupling to bright and dark states of the system. In the second one, we suppress the Purcell decay of a qubit using a compact lumped-element Purcell filter. In addition, we characterize the Purcell decay by employing an auxiliary superconducting qubit as a sensitive power detector directly coupled to the feedline waveguide used for the qubit readout.In summary, this thesis presents three different methods for controlling light–matter interactions in structured quantum systems, including decay suppression with both Purcell filters and symmetry-selective couplings. The thesis also introduces new experimental techniques for probing atom-photon bound states and provides direct evidence of collective phenomena in driven-dissipative quantum metamaterials.
Quantum optics is the field of physics describing the interaction of individual photons with matter, but in recent years it has expanded beyond pure physics to become an important driving force for technological innovation. This book starts with an elementary description of the underlying physics and then builds up a more advanced treatment. The theory begins with the quantum description of the simple harmonic oscillator, and is subsequently extended to provide the tools required to discuss coherent states, the interaction of light with atoms, entangled states, quantum noise and dissipation, linear optical amplifiers, and the fundamental issues associated with Bell's theorem. There is an equally strong emphasis on experimental methods. A quantum description of lenses, mirrors, beam splitters, Y-junctions, circulators, and stops is applied to a collection of important experiments in linear optics. A description of the most important methods of primary photon detection is followed by an explanation of heterodyne and homodyne techniques. Spontaneous down conversion and quantum tomography are discussed, together with important experimental applications. These experimental and theoretical considerations come together in a chapter briefly discussing quantum noise and its suppression in telecommunications; the limitations and possibilities for quantum cloning; the principles and techniques of quantum cryptography; and the physical basis for quantum computing.
Quantum many-body systems coupling photonic and matter degrees of freedom are ideal for the realization of driven open quantum dynamics at the intersection of quantum optics and condensed matter. They offer the possibility to address unresolved issues regarding a variety of non-equilibrium phenomena. In such open systems, the substructure of the reservoir then introduces further timescales that may enter into competition with rapid system processes, raising long-standing questions about the influence of non-Markovian effects on dynamics and equilibration out of equilibrium. \n \nThe central result of this thesis is a general pseudo-particle technique that can be applied to a large class of models of interacting light and matter and allows for realistic and efficient simulations of the full non-equilibrium dynamics of these systems. Since organic molecules, as used in experiments with photon condensates, which provide the main area of application for this thesis, possess an electronic transition coupled to vibrational phonon modes, we construct a representation where an auxiliary boson is assigned to each vibrational state of the molecule. An operator constraint then enforces single occupation across all of these states. We emphasize that we implement the operator constraint exactly and that we are the first to apply a faithful auxiliary-boson representation to open quantum systems. \n \nAs a contribution to bridging the gap between well-understood equilibrium and less explored non-equilibrium phenomena, we investigate photon condensates as they are driven away from equilibrium. The earliest signs of the non-equilibrium character of the driven-dissipative photon gas do not manifest in the spectrally resolved intensity distribution but in the time dependence of the intensity fluctuations. The energy flow through the system renders it {non-Hermitian} and induces a novel driven-dissipative transition in the second-order correlations characterized by the appearance of exceptional points. If only the static intensity spectrum is monitored, this transition remains unnoticed, as does the fact that the system is not truly in equilibrium. Non-Markovian effects due to the non-separability of system and reservoir timescales are shown to become important far away from equilibrium. Furthermore, we derive a novel photon-condensate Gross-Pitaevskii equation, which is capable of describing photo-molecular coherence. Such effects cannot be captured by existing theories and hence serve as a validation of our auxiliary-boson method. These results provide a building block to understanding the properties of the photon condensates in stationary operation where they act as fluctuating light sources. In the future, lattice systems of coupled photon condensates may lead to the appearance of novel driven-dissipative phases of light.
A note to the reader Quantum optics has grown from a sub-discipline in atomic, molecular, and optical physics to a broad research area that bridges several branches of physics and that captures the imagination of the public. Quantum information science has put quantum optics into the spotlight of modern physics, as has the physics of ultracold quantum gases with its many spectacular connections to condensed-matter physics. Yet through all these exciting developments quantum optics has maintained a characteristic core of ideas that I try to explain in this slim volume. Quantum optics focuses on the simplest quantum objects, usually light and few-level atoms, where quantum mechanics appears in its purest form without the complications of more complex systems, often demonstrating in the laboratory the thought experiments that the founders of quantum mechanics dreamed of. Quantum optics has been, and will be for the foreseeable future, quintessential quantum mechanics, the quantum mechanics of simple systems, based on a core of simple yet subtle ideas and experiments. One of the strengths of quantum optics is the close connection between theory and experiment. Although this book necessarily is theoretical, many of the theoretical ideas I describe are guided by experiments or, in turn, have inspired experiments themselves. Another strength of quantum optics is that it is done by individuals or small teams. One single person or a small group can build and perform an entire experiment.
In recent years, topology has become increasingly prevalent in condensed matter physics. It has allowed us to understand, and even predict, a variety of striking and remarkable physical phenomena. The study of strongly interacting systems has similarly lavished us with a diverse range of exotic phases and unconventional transitions, many of which are still poorly understood. In this thesis we will explore the interplay between topology and interactions in an effort to uncover new and novel phases. First we study how interactions impact the quantum phase transition between a topologically non-trivial phase and a trivial phase. The combination of interactions and the low-energy degrees of freedom associated with the transition leads to the emergence of a dome of lattice-symmetry breaking nematic order. Such behaviour is reminiscent of a number of strongly correlated electronic systems. We move on to study the strongly interacting limit of one of the earliest and best-known non-interacting topological phases, Haldane's model of a Chern insulator. Recently realized with ultracold atoms in a shaken optical lattice, the model has a non-trivial topological invariant associated with its band structure. In the strongly interacting limit the spin degrees of freedom are all that survive and we find a rich phase diagram of magnetically ordered phases, using a combination of both classical and quantum techniques. Supplementing the model with an additional term we can `quantum-melt' one of these ordered states to produce a disordered, liquid state that we positively identify as a chiral spin liquid, a highly entangled state of matter with fractionalised excitations. We generalise this mechanism to other two dimensional lattices, uncovering a possible unifying framework with which to understand the emergence of chiral spin liquids in lattice spin models. Finally, motivated by groundbreaking experiments in the ultracold atoms community, we investigate a model of two-component bosons with an artificial spin-orbit coupling. The interplay between the lattice, interactions and spin-orbit coupling produces a variety of unusual superfluid phases. Using a novel Monte Carlo technique we reveal the finite temperature phase diagram that appears close to the Mott transition.