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arXiv:2005.13185 · Entropy

Quantum Photovoltaic Cells Driven by Photon Pulses

Sangchul Oh, Jung Jun Park, Hyunchul Nha

Published Jun 20, 2020• 2 citations
arXivHTMLPDF

Abstract

We investigate the quantum thermodynamics of two quantum systems, a two-level system and a four-level quantum photocell, each driven by photon pulses as a quantum heat engine. We set these systems to be in thermal contact only with a cold reservoir while the heat (energy) source, conventionally given from a hot thermal reservoir, is supplied by a sequence of photon pulses. The dynamics of each system is governed by a coherent interaction due to photon pulses in terms of the Jaynes-Cummings Hamiltonian together with the system-bath interaction described by the Lindblad master equation. We calculate the thermodynamic quantities for the two-level system and the quantum photocell including the change in system energy, the power delivered by photon pulses, the power output to an external load, the heat dissipated to a cold bath, and the entropy production. We thereby demonstrate how a quantum photocell in the cold bath can operate as a continuum quantum heat engine with a sequence of photon pulses continuously applied. We specifically introduce the power efficiency of the quantum photocell in terms of the ratio of output power delivered to an external load with current and voltage to the input power delivered by the photon pulse. Our study indicates a possibility that a quantum system driven by external fields can act as an efficient quantum heat engine under non-equilibrium thermodynamics.

DOI
10.3390/e22060693

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We investigate the quantum thermodynamics of two quantum systems, a two-level system and a four-level quantum photocell, each driven by photon pulses as a quantum heat engine. We set these systems to be in thermal contact only with a cold reservoir while the heat (energy) source, conventionally given from a hot thermal reservoir, is supplied by a sequence of photon pulses. The dynamics of each system is governed by a coherent interaction due to photon pulses in terms of the Jaynes-Cummings Hamiltonian together with the system-bath interaction described by the Lindblad master equation. We calculate the thermodynamic quantities for the two-level system and the quantum photocell including the change in system energy, the power delivered by photon pulses, the power output to an external load, the heat dissipated to a cold bath, and the entropy production. We thereby demonstrate how a quantum photocell in the cold bath can operate as a continuum quantum heat engine with a sequence of photon pulses continuously applied. We specifically introduce the power efficiency of the quantum photocell in terms of the ratio of output power delivered to an external load with current and voltage to the input power delivered by the photon pulse. Our study indicates a possibility that a quantum system driven by external fields can act as an efficient quantum heat engine under non-equilibrium thermodynamics.
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Recently, the thermodynamics of open quantum systems driven by light fields has been investigated in the framework of quantum heat engines, whose output work can be measured as a spectroscopic signal. In this work, we investigate a four-level quantum heat engine that generates cascaded entangled photon pairs, treating the hot bath as an incoherent thermal pump and focusing on the correlation statistics of the output work and photon indistinguishability. We show that the dissipative nonequilibrium dynamics of this thermodynamic open quantum system can be reconstructed by correlation measurements under carefully mediated optical control. Comparing our findings with the traditional coherently pumped model, we find that the thermal pumping has the potential to generate nonclassical correlations resulting in photon indistinguishability, displaying an advantage in probing the nonequilibrium effects induced by the baths at different temperatures. Our work also demonstrates that incoherent pumping can optimize such correlations in output work beyond the classical limit. Lastly, we show that nonclassical correlations and resonant power at steady state cannot be simultaneously maximized in the weak coupling regime. Published by the American Physical Society 2024
Conventional continuous quantum heat engines with incoherent heat transfer perform poorly as they exploit two-body interactions between the system and hot or cold baths, thus having limited capability to outperform their classical counterparts. We introduce distinct continuous quantum heat engines that utilize coherent heat transfer with baths, yielding genuine quantum enhancement in performance. These coherent engines consist of one qutrit system and two photonic baths and enable coherent heat transfer via two-photon transitions involving three-body interactions between the system and hot and cold baths. We demonstrate that coherent engines deliver significantly higher power output with much greater reliability, i.e., lower signal-to-noise ratio of the power, by hundreds of folds over their incoherent counterparts. Importantly, coherent engines can operate close to or at the maximal achievable reliability allowed by the quantum thermodynamic uncertainty relation. Moreover, coherent engines manifest more nonclassical features than incoherent engines because they violate the classical thermodynamic uncertainty relation by a greater amount and for a wider range of parameters. These genuine enhancements in the performance of coherent engines are directly attributed to their capacity to harness higher energetic coherence for the resonant driving case. The experimental feasibility of coherent engines and the improved understanding of how quantum properties can enhance performance may find applications in quantum enabled technologies.
Abstract We work on a comprehensive theoretical investigation of a three-level quantum heat engine operating with engineered squeezed thermal reservoirs. Unlike conventional quantum heat engines that use thermal reservoirs, we demonstrate that squeezed reservoirs can significantly enhance the engine's performance by increasing both efficiency and output power. Using a rigorous open-quantum-system approach, we derive the full Lindblad master equation for a three-level system interacting with hot and cold squeezed thermal baths. Through a detailed analysis of the steady-state thermodynamics, we obtain explicit expressions for heat currents, work output, and efficiency. Our results reveal that moderate squeezing parameters (r≈0.5r \approx 0.5r≈0.5) combined with optimal squeezing phase (ϕ=π/2\phi = \pi/2ϕ=π/2) enhance the engine efficiency by up to 40\% compared to the classical Carnot limit for the same temperature ratio. The power output shows a non-monotonic behavior with squeezing, exhibiting an optimal squeezing parameter that maximizes performance. We identify three distinct operational regimes: (i) heat engine regime, (ii) refrigerator regime, and (iii) heat pump regime, which can be tuned by adjusting the squeezing phase. The efficiency at maximum power follows a universal scaling ηMP≈ηCarnot/2+Δη(r)\eta_{MP} \approx \eta_{Carnot}/2 + \Delta\eta(r)ηMP​≈ηCarnot​/2+Δη(r), where Δη(r)\Delta\eta(r)Δη(r) represents the squeezing-induced enhancement. Our findings provide fundamental insights into the role of non-thermal reservoirs in quantum thermodynamics and offer practical guidelines for designing high-performance quantum heat engines using squeezed light and engineered baths.
Quantum coherence can affect the thermodynamics of small quantum systems. Coherences have been shown to affect the power generated by a quantum heat engine (QHE) which is coupled to two thermal photon reservoirs and to an additional cavity mode. We show that the fluctuations of the heat exchanged between the QHE and the reservoirs strongly depend on quantum coherence, especially when the engine operates as a refrigerator, i.e., heat current flows from the cold bath to the hot bath. Intriguingly, we find that the ratio of positive and negative (with respect to the thermodynamic force) fluctuations in the heat current satisfies a universal coherence-independent fluctuation theorem.
The single-atom version of the quantum heat engine based on electromagnetically induced transparency is theoretically investigated in this paper. In contact with a hot and a cold bath, the atom trapped in an optical cavity is coherently coupled by a coherent field, thus generating photons as output through a process that mimics a heat engine. Using semiclassical theory, we obtain the conditions for the classical gain parameter being positive. Then by taking a full quantum approach, we discuss the statistical property of the generated photons depicted by the photon number distribution and Wigner function, and show that it can be effectively tuned by the coupling field. Investigations on the energy and entropy balances of the heat engine process lead to an interesting result that the power of the engine is simply the energy per time provided by the hot reservoir. The coupling field plays a critical role in supporting the heat-engine process. However, the energy that it provides is all dumped into the cold reservoir. The total energy exchange conforms to the first law of thermodynamics. The efficiency of the engine depends on the temperatures of the two reservoirs and the strength of the coupling field. The entropy change of the heat-engine process suggests that when working far above the threshold of lasing, the efficiency approaches that of its atomic-ensemble-based partner.