In this PhD thesis, we will present the theoretical and experimental work that led to the realization of a radio-frequency circuit quantum electrodynamics system (RFcQED). In chapter 2, we provide a detailed derivation of the Hamiltonian of circuit QED formulated in the context of the Rabi model, and extract expressions for the cross-Kerr interaction. The resulting requirements for the coupling rate in RFcQED are discussed, one of them being the need to dramatically increase the coupling rate compared to typical circuit QED device. In chapter 3 we cover two experimental approaches to increasing the coupling in a circuit QED system, one making use of a high impedance resonator, the second utilizing a large coupling capacitor. In chapter 4, we combine these two approaches to implement RFcQED. Through strong dispersive coupling, we could measure individual photons in a megahertz resonator, demonstrate quantum control by cooling the resonator to the ground state or preparing Fock states, and finally observe with nanosecond resolution the re-thermalization of these states. In chapter 5 we present QuCAT or Quantum Circuit Analyzer Tool in Python, a software package that can be used for the design of circuit QED systems such as the one presented in this thesis. In chapter 6 we discuss how certain interplays between general relativity and quantum mechanics cannot be described using our current laws of physics. In particular, we show how radio-frequency mechanical oscillators are perfect candidates to perform experiments in this regime. In chapter 7 we present the prospects for coupling such mechanical oscillator to weakly anharmonic superconducting circuits such as the transmon qubit or RFcQED systems.
In this PhD thesis, we will present the theoretical and experimental work that led to the realization of a radio-frequency circuit quantum electrodynamics system (RFcQED). In chapter 2, we provide a detailed derivation of the Hamiltonian of circuit QED formulated in the context of the Rabi model, and extract expressions for the cross-Kerr interaction. The resulting requirements for the coupling rate in RFcQED are discussed, one of them being the need to dramatically increase the coupling rate compared to typical circuit QED device. In chapter 3 we cover two experimental approaches to increasing the coupling in a circuit QED system, one making use of a high impedance resonator, the second utilizing a large coupling capacitor. In chapter 4, we combine these two approaches to implement RFcQED. Through strong dispersive coupling, we could measure individual photons in a megahertz resonator, demonstrate quantum control by cooling the resonator to the ground state or preparing Fock states, and finally observe with nanosecond resolution the re-thermalization of these states. In chapter 5 we present QuCAT or Quantum Circuit Analyzer Tool in Python, a software package that can be used for the design of circuit QED systems such as the one presented in this thesis. In chapter 6 we discuss how certain interplays between general relativity and quantum mechanics cannot be described using our current laws of physics. In particular, we show how radio-frequency mechanical oscillators are perfect candidates to perform experiments in this regime. In chapter 7 we present the prospects for coupling such mechanical oscillator to weakly anharmonic superconducting circuits such as the transmon qubit or RFcQED systems.
PhD Thesis: Superconducting circuit quantum electrodynamics (QED) has developed into a powerful platform for studying the interaction between matter and different states of light. In this context, superconducting quantum bits (qubits) act as artificial atoms interacting with quantized modes of the electromagnetic field. The field can be trapped in superconducting microwave resonators or propagating in transmission lines. In this thesis, we particularly study circuit QED systems where microwave fields are coupled with superconducting flux and transmon qubits. We optimize the coherence properties of the resonators, by analyzing loss mechanisms at excitation powers of approximately one photon on average. We find that two-level fluctuators associated with oxide layers at substrate and metal surfaces and metal-metal interfaces represent the predominant loss channel. Furthermore, we show how broadband thermal photon fields influence the relaxation and dephasing properties of a superconducting transmon qubit. To this end, we study several second-order loss channels of the transmon qubit and find that the broadband fields introduce a larger decay rate than expected from the Purcell filter defined by the resonator. Additionally, we show that qubit dephasing at the flux-insensitive point as well as low-frequency parameter fluctuations can be enhanced by thermal fields. Finally, we study how artificial atoms react to changes in inherent properties of the light fields. We perform a detailed analysis of the photon statistics of thermal fields using their relation to the qubits coherence properties. We quantitatively recover the expected n2+n-law for the photon number variance and confirm this result by direct correlation measurements. We then show a novel technique for the in-situ conversion of the interaction parity in light-matter interaction. To this end, we couple spatially controlled microwave fields to a flux qubit with two degrees of freedom.
This thesis explores nonlinear couplings in superconducting circuits with the purpose of achieving quantum control over the elementary excitations of light and motion. It consists mainly of three research themes. The first theme concerns the experimental realisation of a tuneable coupling scheme, giving rise to different interactions with adjustable ratios, between two transmon qubits. The tuneable capabilities of the device together with its versatile geometry and high coherence make it an interesting building block for analog quantum simulators of certain classes of complex problems. The second theme concerns two theoretical proposals for controlling mechanical resonators using transmon qubits. In the first part we analyse an electromechanical circuit architecture giving rise to tuneable three-body interactions between two qubits and a mechanical beam. Several protocols are performed numerically demonstrating ground-state cooling and the creation of mechanical quantum states, such as single-phonon and multi-phonon superposition states as well as qubit-phonon entanglement. Additionally, schemes for generating arbitrary quantum states are explored. The second part relies on the same concept for coupling a mechanical resonator to a transmon qubit and explores the qubit-resonator system in the ultrastrong coupling regime, where the optomechanical coupling approaches or even exceeds the mechanical frequency. We find that for certain coupling strengths ground-state cooling is possible and devise a protocol for generating macroscopic quantum superposition states, known as “Shrödinger cats”, on the mechanical resonator. Finally, the third research theme presented in the thesis concerns an experiment where a cold superconducting qubit is employed to readout and control a thermally populated radio-frequency resonator coupled via a strong dispersive coupling. By means of reservoir engineering, ground-state cooling as well as stabilisation of Fock states in the resonator are demonstrated reaching a new operating regime for circuit quantum electrodynamics.
In this thesis, experimentally relevant aspects and open questions of quantum information processing and measurement in circuit quantum electrodynamics have been investigated theoretically. Circuit quantum electrodynamics is a relatively young field combining superconducting transmission line resonators on-chip with superconducting quantum bits which serve as artificial atoms. Remarkable experiments have underlined the prospects of circuit QED as a possible architecture for quantum information processing as well as a framework within which quantum optics experiments can be performed. In contrast to their optical counterparts, these experiments reach the ultra-strong coupling limit and allow e.g. the generation of Fock states, the study of decoherence and the observation of quantum jumps. We present the physics of superconducting circuits based on the Josephson junction as a non-linear circuit element. We discuss the various types of quantum bits (qubits) before turning to an introduction on cavity QED and conclude the introduction with a brief presentation of the most relevant experiments and a short introduction to the principles and prospects of quantum information processing. Building on the pioneering theoretical and experimental work in which up to three qubits have been integrated on a chip and successfully coupled via a cavity mode, we propose a scheme to overcome the natural limits concerning scalability in these systems. Usually, scalability is severely limited by the resonance width of the qubit transitions and the attainable frequency range for both qubit transition and cavity resonance frequencies. This limits the present setups to at most ten qubits. As a possible solution, we propose and investigate a cross-bar grid layout of cavities with qubits at the intersections. It turns out that this setup, allowing for up to about 1000 qubits, offers significant advantages over e.g. nearest-neighbor coupling schemes. In addition, it can serve as a building block for a truly scalable scheme for fault-tolerant quantum information processing with superconducting circuits by combining 7x7 arrays in a staircase manner. Furthermore, we discuss and simulate different possibilities to improve upon the suggested scheme by e.g. using resonant gates and optimal control theory. Another focus of the present thesis is measurement physics. In order to investigate e.g. the possibilities of using a circuit QED system to dispersively detect single microwave photons or to generate multi-qubit entangled states, we introduce in a pedagogical manner the basics of stochastic master equations which generate quantum trajectories before turning to concrete applications. Quantum trajectories have proven to be a state-of-the-art tool to analyze measurement situations in a very realistic manner by giving access to both the measurement record as well as the internal quantum dynamics conditioned on this record. Using the method of quantum trajectories as generated by stochastic master equations, we discuss a scheme to efficiently generate multi-qubit entangled states in a very flexible way. The method is based on a collective, dispersive qubit readout. By this measurement, a suitable product state of N qubits can be reliably converted into e.g. an N-qubit Greenberger-Horne-Zeilinger or W state. We propose and discuss the scheme and investigate the effects of decoherence and parameter spread as they would be encountered in experiment. Last but not least, we propose and fully analyze a scheme to dispersively detect single itinerant microwave photons. While experiments to generate single microwave photons have already been successfully performed, their single-shot quantum non-demolition detection has not been possible so far. The scheme presented in this thesis closes this gap in the circuit QED toolbox and reaches detection efficiencies of 30% only limited by fundamental quantum mechanics in this case the Quantum Zeno effect. This detection scheme could be used in quantum communication or quantum cryptography applications.
Circuit quantum electrodynamics (cQED), exemplified by a coupled system of a superconducting qubit and a microwave cavity, is a powerful framework for the quantum control and measurement of macroscopic quantum states in solid-state circuits. Quantum circuits based on superconducting qubits have emerged as one of the leading platforms in the pursuit of fault-tolerant quantum computing. Despite significant progress in extending qubit lifetimes, refining experimental protocols, and scaling up quantum processors, errors arising from the control and measurement of superconducting qubits continue to hinder the realization of a universal quantum computer. To investigate the error mechanisms for state-of-the-art qubits, we realize long-lived superconducting transmon qubits that exhibit fluctuating lifetimes, with an average of 0.2 ms and a maximum exceeding 0.4 ms. We then investigate their dominant error mechanism. By introducing novel time-resolved error measurements that are synchronized with the operation of the pulse tube cooler in a dilution refrigerator, we find that mechanical vibrations from the pulse tube induce nonequilibrium dynamics in highly coherent qubits, leading to their correlated bit-flip errors. Our findings not only deepen our understanding of qubit error mechanisms but also provide valuable insights into potential error-mitigation strategies for achieving fault tolerance by decoupling superconducting qubits from their mechanical environments. We also present a novel scheme for operating a cQED system in a regime where the cavity is largely displaced. We find that a qubit drive at the bare cavity frequency can effectively displace the cavity field while minimizing the cavity-drive-induced dephasing and the ac Stark shift. Furthermore, we demonstrate that standard cQED protocols, such as qubit control, readout, and cavity single-photon generation, remain compatible with largely displaced cavity fields, even beyond the critical photon number. These findings open new pathways for exploring cQED dynamics in large-photon-number regimes, including the study of nonlinear phenomena in microwave cavities, the saturation of two-level system baths for extending the coherence of microwave quantum states, and the acceleration of the dispersive readout. Finally, mechanical resonators have emerged as integral components in quantum computing for storing and transducing quantum information. Low-frequency mechanical resonators, with extremely low energy dissipation rates, are particularly interesting for extending the lifetimes of stored quantum information. However, integrating low-frequency mechanical resonators with qubits is challenging because their small energy gaps make coherent energy exchange and ground-state preparation difficult. In this thesis, we report the first steps towards the characterization of a hybrid quantum device, consisting of a Transmon qubit and a circuit optomechanical system, both coupled to a 3D microwave cavity.
As superconducting circuits emerge as a leading platform for scalable quantum information processing, building comprehensive bridges from the foundational principles of macroscopic quantum phenomena to the architecture of modern quantum devices is increasingly essential for introducing new researchers to the field. This tutorial provides a self-contained, pedagogical introduction to superconducting quantum circuits at the undergraduate level. Beginning with an overview of superconductivity and the Josephson effect, the tutorial systematically develops the quantization of microwave circuits into the framework of circuit quantum electrodynamics (cQED). The transmon qubit is then introduced as a state-of-the-art application, with a detailed derivation of its Hamiltonian and its interaction with control and readout circuitry. The theoretical formalism is consolidated through a numerical simulation of vacuum Rabi oscillations in a driven transmon-resonator system, a canonical experiment that demonstrates the coherent energy exchange characteristic of the strong coupling regime. This work serves as a foundational guide and first point of contact, equipping students and researchers with the conceptual and mathematical tools necessary to understand and engineer superconducting quantum hardware.
One of the key elements in circuit quantum electrodynamics (cQED) is the superconducting microwave resonator, which can enable strong coupling to and between nanoscale quantum systems, and as a result has emerged as an essential tool for both quantum information and quantum sensing. In this thesis, I will discuss new applications of superconducting resonators in both of these fields, which illustrates how quantum information and quantum sensing can be strongly tied together. As the field of quantum information continues to grow, various platforms for realizing a quantum computer have been proposed. One attractive platform is to control and manipulate the spin of an electron to form spin qubits, which have demonstrated a long coherence time, weak coupling to the environment, and high fidelity single- and two-qubit gates. However, scaling beyond two qubits has proven challenging, as has incorporating long-range coupling, although both are crucial for making spin qubits a scalable quantum computing platform. The confinement of electromagnetic fields in superconducting resonators enables strong coupling to small systems, such as the single electrons of a spin qubit. In the first part of this thesis, I will describe how a singlet-triplet spin qubit coupled to a high-impedance superconducting resonator constitutes a promising architecture for mediating long-ranged interactions based on a longitudinal coupling between the resonator and qubit. I will discuss the technical developments needed to successfully implement this novel type of interaction in a hybrid spin qubit-resonator device. This type of interaction has several advantages over the more commonly studied transverse coupling scheme: it does not require careful tuning of the qubit frequency to match that of the resonator, which facilitates scaling to a large number of qubits, and also avoids the loss of coherence, which is inevitable in resonant coupling. This type of interaction therefore opens promising paths for generating high-fidelity long-ranged two-qubit coupling by employing superconducting microwave resonators. By adapting techniques used in quantum information, we have also developed a new technique in quantum sensing, where we employ superconducting resonators as a probe of quantum materials such as mesoscopic systems, two-dimensional materials, and heterostructures, which are otherwise challenging to experimentally access with conventional techniques. In the second part of my thesis, I will discuss how implementing cQED techniques from quantum information allows us to probe the symmetry of the order parameter in unconventional superconductors. Unconventional superconductors are not readily available, and we therefore study an engineered system that comprises of interfacing a ferromagnet and superconductor, in which unconventional pairing can be induced into the ferromagnet. This platform allows us to simultaneously excite spin waves, a collective excitation of spins, in the ferromagnet, which opens new directions for studying interactions between coherently coupled magnons (quanta of spin waves) and unconventional superconducting states. Finally, by applying the same technique to a two-dimensional (2D) superconductor, tungsten ditelluride, we leverage this platform in an attempt to study the order parameter of its intrinsic superconducting phase. The nature of the order parameter in this material remains an open question, as both topological and superconducting phases can exist, possibly simultaneously. This work thus demonstrates a unique use of superconducting resonators beyond quantum information applications.