This thesis explores nonlinear couplings in superconducting circuits with the purpose of achieving quantum control over the elementary excitations of light and motion. It consists mainly of three research themes. The first theme concerns the experimental realisation of a tuneable coupling scheme, giving rise to different interactions with adjustable ratios, between two transmon qubits. The tuneable capabilities of the device together with its versatile geometry and high coherence make it an interesting building block for analog quantum simulators of certain classes of complex problems. The second theme concerns two theoretical proposals for controlling mechanical resonators using transmon qubits. In the first part we analyse an electromechanical circuit architecture giving rise to tuneable three-body interactions between two qubits and a mechanical beam. Several protocols are performed numerically demonstrating ground-state cooling and the creation of mechanical quantum states, such as single-phonon and multi-phonon superposition states as well as qubit-phonon entanglement. Additionally, schemes for generating arbitrary quantum states are explored. The second part relies on the same concept for coupling a mechanical resonator to a transmon qubit and explores the qubit-resonator system in the ultrastrong coupling regime, where the optomechanical coupling approaches or even exceeds the mechanical frequency. We find that for certain coupling strengths ground-state cooling is possible and devise a protocol for generating macroscopic quantum superposition states, known as “Shrödinger cats”, on the mechanical resonator. Finally, the third research theme presented in the thesis concerns an experiment where a cold superconducting qubit is employed to readout and control a thermally populated radio-frequency resonator coupled via a strong dispersive coupling. By means of reservoir engineering, ground-state cooling as well as stabilisation of Fock states in the resonator are demonstrated reaching a new operating regime for circuit quantum electrodynamics.
This thesis explores nonlinear couplings in superconducting circuits with the purpose of achieving quantum control over the elementary excitations of light and motion. It consists mainly of three research themes. The first theme concerns the experimental realisation of a tuneable coupling scheme, giving rise to different interactions with adjustable ratios, between two transmon qubits. The tuneable capabilities of the device together with its versatile geometry and high coherence make it an interesting building block for analog quantum simulators of certain classes of complex problems. The second theme concerns two theoretical proposals for controlling mechanical resonators using transmon qubits. In the first part we analyse an electromechanical circuit architecture giving rise to tuneable three-body interactions between two qubits and a mechanical beam. Several protocols are performed numerically demonstrating ground-state cooling and the creation of mechanical quantum states, such as single-phonon and multi-phonon superposition states as well as qubit-phonon entanglement. Additionally, schemes for generating arbitrary quantum states are explored. The second part relies on the same concept for coupling a mechanical resonator to a transmon qubit and explores the qubit-resonator system in the ultrastrong coupling regime, where the optomechanical coupling approaches or even exceeds the mechanical frequency. We find that for certain coupling strengths ground-state cooling is possible and devise a protocol for generating macroscopic quantum superposition states, known as “Shrödinger cats”, on the mechanical resonator. Finally, the third research theme presented in the thesis concerns an experiment where a cold superconducting qubit is employed to readout and control a thermally populated radio-frequency resonator coupled via a strong dispersive coupling. By means of reservoir engineering, ground-state cooling as well as stabilisation of Fock states in the resonator are demonstrated reaching a new operating regime for circuit quantum electrodynamics.
In this thesis, we study two different physical systems, namely superconducting circuits and optomechanical cavities. \nIn the first part of the thesis, we study superconducting qubits and resonators and their potential to implement quantum information processing tasks. We propose a circuit quantum electrodynamics realization of a protocol to generate a Greenberger-Horne-Zeilinger (GHZ) state for transmon qubits homogeneously coupled to a microwave cavity in the dispersive limit. We derive an effective Hamiltonian with pairwise qubit exchange interactions of the XY type that can be globally controlled. Starting from a separable initial state, these interactions allow to generate a multi-qubit GHZ state within a time that does not depend on the number of qubits. We discuss how to probe the non-local nature and the genuine multipartite entanglement of the generated state. Finally, we investigate the stability of the proposed scheme to inhomogeneities in the physical parameters and the weak anharmonicity of transmon qubits. \nIn the second part of the thesis, we study optomechanical systems in which the position of a mechanical resonator modulates the resonance frequency of an optical cavity. The resulting radiation-pressure interaction is intrinsically nonlinear and can be used to implement strong Kerr nonlinearities and an effective interaction between photons. We investigate the optical bistability of such a system. The steady-state mean-field equation of the optical mode is identical to the one for a Kerr medium, and thus we expect it to have the same characteristic behavior with a lower, a middle, and an upper branch. However, the presence of position fluctuations of the mechanical resonator leads to a new feature: the upper branch will become unstable at sufficiently strong driving in certain parameter regimes. We identify the appropriate parameter regime for the upper branch to be stable, and we confirm, by numerical investigation of the quantum steady state, that the mechanical mode indeed acts as a Kerr nonlinearity for the optical mode in the low-temperature limit. This equivalence of the optomechanical system and the Kerr medium will be important for future applications of cavity optomechanics in quantum nonlinear optics and quantum information science. \n
In the late 1960s and early 1970s, the development of mechanical resonators was pushed forward in efforts to record gravitational waves. In order to push down the limit of the smallest detectable force, the radiation circulating in a Fabry-Perot cavity was demonstrated to modify the damping of the cavity end-mirror suspended to act as a mechanical resonator. A few years later, motivated by the study of the internal properties of atoms and ions, the radiation pressure of light was realized as a means to cool atomic motion. In the following years, the ground-state cooling of ion motion was achieved in landmark studies. For mechanical resonators parametrically coupled to Fabry-Perot cavities, it took much longer to reach quantum ground-state cooling, both in the microwave domain, where the original experiments took place, and in the optical domain. Ground-state cooling in both regimes was reached by three groups during the preparation of this thesis and was largely due to advancements in the fabrication methods. \n \nGround-state cooling allows, in principle, the quantum nature of mechanical resonators to be probed and harnessed. Microwave domain devices, which are focused on in this thesis, have the advantage that nonlinear elements (superconducting quantum bits, qubits) are readily available. These elements enable nonclassical state preparation of the qubit and the subsequent transfer to the microwave cavity. The goal is to transfer these quantum states to mechanical resonators. This would allow mechanics to be used as a quantum mechanical memory in quantum information processing thanks to their long lifetimes. \n \nIn this thesis, various aspects of microwave domain circuit optomechanics are studied. The main goal of this thesis is to study how to enhance the coupling between a quantum regime microwave device and a mechanical resonator by using Josephson junction –based qubits. Coherent interaction between a superconducting qubit and a classical driven mechanical field is demonstrated. The analysis presented in this thesis predicts that ground-state cooling and coherent state transfer is possible in the single-phonon regime with transmon-regime qubits. Also, traditional linear optomechanical systems are considered in which the mechanical resonator is coupled to an electrical resonator. Such systems exhibit a rich spectrum of phenomena from which the quantum-limited amplification and multimode effects are considered in this thesis. It is shown that the system operates near quantum-limited amplification, which could be reached if the mechanical resonator was in the ground state.
Superconducting circuits provide an architecture upon which cavity quantum electrodynamics (QED) can be implemented at microwave frequencies in a highly tunable environment. Known as circuit QED, these systems can achieve larger nonlinearities, stronger coupling and greater controllability than can be achieved in cavity QED, all in a customisable, solid state device, making this technology an exciting test bed for both quantum optics and quantum information processing. These new parameter regimes open up new avenues for quantum technology, while also allowing older quantum optics results to finally be tested. In particular is is now possible to experimentally produce nonclassical states, such as squeezed and Schr\\"odinger cat states, relatively simply in these devices. Using open quantum systems methods, in this thesis we investigate four problems which involve the use of nonclassical states in circuit QED. First we investigate the effects of a Kerr nonlinearity on the ability to preserve transported squeezed states in a superconducting cavity, and whether this setup permits us to generate, and perform tomography, of a highly squeezed field using a qubit, with possible applications in the characterisation of sources of squeezed microwaves. Second, we present a novel scheme for the amplification of cat states using a coupled qubit and external microwave drives, inspired by the stimulated Raman adiabatic passage. This scheme differs from similar techniques in circuit QED in that it is deterministic and therefore compatible with a protocol for stabilising cat states without the need for complex dissipation engineering. Next we use solutions of Fokker-Planck equations to study the exact steady-state response of two nonlinear systems: a transmon qubit coupled to a readout resonator, where we find good agreement with experiments and see simultaneous bistability of the cavity and transmon; and a parametrically driven nonlinear resonator, where we compare the classical and quantum phases of the system and discuss applications in the generation of squeezed states and stabilisation of cat states. Finally, we investigate the use of two different types of superconducting qubits in a single experiment, seeing that this enables engineering of the self- and cross-Kerr effects in a line of cavities. This could provide a valuable means of entangling cavity states, in addition to a resource for quantum simulation.
Circuit quantum electrodynamics (cQED), exemplified by a coupled system of a superconducting qubit and a microwave cavity, is a powerful framework for the quantum control and measurement of macroscopic quantum states in solid-state circuits. Quantum circuits based on superconducting qubits have emerged as one of the leading platforms in the pursuit of fault-tolerant quantum computing. Despite significant progress in extending qubit lifetimes, refining experimental protocols, and scaling up quantum processors, errors arising from the control and measurement of superconducting qubits continue to hinder the realization of a universal quantum computer. To investigate the error mechanisms for state-of-the-art qubits, we realize long-lived superconducting transmon qubits that exhibit fluctuating lifetimes, with an average of 0.2 ms and a maximum exceeding 0.4 ms. We then investigate their dominant error mechanism. By introducing novel time-resolved error measurements that are synchronized with the operation of the pulse tube cooler in a dilution refrigerator, we find that mechanical vibrations from the pulse tube induce nonequilibrium dynamics in highly coherent qubits, leading to their correlated bit-flip errors. Our findings not only deepen our understanding of qubit error mechanisms but also provide valuable insights into potential error-mitigation strategies for achieving fault tolerance by decoupling superconducting qubits from their mechanical environments. We also present a novel scheme for operating a cQED system in a regime where the cavity is largely displaced. We find that a qubit drive at the bare cavity frequency can effectively displace the cavity field while minimizing the cavity-drive-induced dephasing and the ac Stark shift. Furthermore, we demonstrate that standard cQED protocols, such as qubit control, readout, and cavity single-photon generation, remain compatible with largely displaced cavity fields, even beyond the critical photon number. These findings open new pathways for exploring cQED dynamics in large-photon-number regimes, including the study of nonlinear phenomena in microwave cavities, the saturation of two-level system baths for extending the coherence of microwave quantum states, and the acceleration of the dispersive readout. Finally, mechanical resonators have emerged as integral components in quantum computing for storing and transducing quantum information. Low-frequency mechanical resonators, with extremely low energy dissipation rates, are particularly interesting for extending the lifetimes of stored quantum information. However, integrating low-frequency mechanical resonators with qubits is challenging because their small energy gaps make coherent energy exchange and ground-state preparation difficult. In this thesis, we report the first steps towards the characterization of a hybrid quantum device, consisting of a Transmon qubit and a circuit optomechanical system, both coupled to a 3D microwave cavity.
In this PhD thesis, we will present the theoretical and experimental work that led to the realization of a radio-frequency circuit quantum electrodynamics system (RFcQED). In chapter 2, we provide a detailed derivation of the Hamiltonian of circuit QED formulated in the context of the Rabi model, and extract expressions for the cross-Kerr interaction. The resulting requirements for the coupling rate in RFcQED are discussed, one of them being the need to dramatically increase the coupling rate compared to typical circuit QED device. In chapter 3 we cover two experimental approaches to increasing the coupling in a circuit QED system, one making use of a high impedance resonator, the second utilizing a large coupling capacitor. In chapter 4, we combine these two approaches to implement RFcQED. Through strong dispersive coupling, we could measure individual photons in a megahertz resonator, demonstrate quantum control by cooling the resonator to the ground state or preparing Fock states, and finally observe with nanosecond resolution the re-thermalization of these states. In chapter 5 we present QuCAT or Quantum Circuit Analyzer Tool in Python, a software package that can be used for the design of circuit QED systems such as the one presented in this thesis. In chapter 6 we discuss how certain interplays between general relativity and quantum mechanics cannot be described using our current laws of physics. In particular, we show how radio-frequency mechanical oscillators are perfect candidates to perform experiments in this regime. In chapter 7 we present the prospects for coupling such mechanical oscillator to weakly anharmonic superconducting circuits such as the transmon qubit or RFcQED systems.
This thesis explores novel strategies for advancing superconducting quantum computing through a series of experimental investigations and device innovations. Grounded in the development of circuit quantum electrodynamics, the work addresses the challenges posed by the limitations of coherent control, coherence time and scaling of superconducting qubits. Focusing on transmon qubits, the thesis first reviews the foundational principles of circuit quantum electrodynamics and the critical role of the transmon in achieving robust qubit performance. Three experimental studies form the core of this work. The first study demonstrates a universal quantum gate set for strongly coupled transmons. By exploiting the residual ZZ interaction, the work introduces a novel two-axis gate protocol for single-qubit operations and implements both CZ and CNOT gates with high fidelities, highlighting the potential for fast, low-error quantum operations in the strong coupling regime. The second study investigates a dual-rail qubit architecture using parametrically coupled transmons, showcasing a hardware-efficient approach to quantum error correction. This experiment converts single-photon loss errors into detectable erasures and leverages mid-circuit detection to enhance qubit coherence, thereby advancing fault-tolerant quantum computing schemes in the NISQ era. The final study focuses on the development of merged-element transmons (MET) and their FinMET variants. By integrating the Josephson junction and shunt capacitor into a single trilayer device, these innovations achieve a dramatic reduction in device footprint while addressing loss channels through advanced materials engineering, ultimately paving the way for scalable, high-coherence quantum circuits. Collectively, these contributions demonstrate significant progress in quantum gate design, error mitigation, and qubit architecture, offering promising routes toward the realization of largescale, fault-tolerant quantum computers