Abstract We demonstrate novel implementations of high-precision optical magnetometers which allow for spatially-selective and spatially-resolved in situ measurements using cold atomic clouds. These are realised by using shaped dispersive probe beams combined with spatially-resolved balanced homodyne detection. Two magnetometer sequences are discussed: a vectorial magnetometer, which yields sensitivities two orders of magnitude better compared to a previous realisation and a Larmor magnetometer capable of measuring absolute magnetic fields. We characterise the dependence of single-shot precision on the size of the analysed region for the vectorial magnetometer and provide a lower bound for the measurement precision of magnetic field gradients for the Larmor magnetometer. Finally, we give an outlook on how dynamic trapping potentials combined with selective probing can be used to realise enhanced quantum simulations in quantum gas microscopes.
Abstract We demonstrate novel implementations of high-precision optical magnetometers which allow for spatially-selective and spatially-resolved in situ measurements using cold atomic clouds. These are realised by using shaped dispersive probe beams combined with spatially-resolved balanced homodyne detection. Two magnetometer sequences are discussed: a vectorial magnetometer, which yields sensitivities two orders of magnitude better compared to a previous realisation and a Larmor magnetometer capable of measuring absolute magnetic fields. We characterise the dependence of single-shot precision on the size of the analysed region for the vectorial magnetometer and provide a lower bound for the measurement precision of magnetic field gradients for the Larmor magnetometer. Finally, we give an outlook on how dynamic trapping potentials combined with selective probing can be used to realise enhanced quantum simulations in quantum gas microscopes.
This thesis covers experimental work conducted within two distinct fields of cold-atom physics. The first part describes an experiment capable of spatially-selective dispersive measurements of a cold-atomic system in part or in whole, by virtue of a digital micromirror device (DMD). Atom clouds are trapped in optical tweezers made and controlled by an acousto-optical deflector. Two types of high-precision magnetometers are realised. One is vectorial and reaches a single-shot precision of dB = (100, 200) µG for the field components parallel and transversal to the probe light, exceeding a previous realisation by two orders of magnitude. The other is a scalar magnetometer based on Larmor precession and reaches dB = 30 µG, putting it on equal footing with other state-of-the-art cold-atom magnetometers. The second part is devoted to the characterisation and the first results of a new quantum gas microscope experiment. It features a 0.69 NA microscope objective for high-resolution fluorescence imaging of individual atoms trapped in deep optical lattices. The imaging system is shown to perform near the diffraction limit. By means of DMD-generated off-resonant tight optical tweezers, projected through the high-resolution optics, we can load only a few planes of a co-propagating 1D lattice. In a single realisation of the experiment we acquire multiple fluorescence images, where the objective is translated between images, bringing different planes of the optical lattices in focus. In this way we can tomographically reconstruct the atom distribution in 3D.
This thesis presents advancements in radio-frequency atomic magnetometry utilising cold atoms as sensors. While cold atom magnetometers demonstrate lower absolute sensitivity compared to conventional vapour cell systems due to reduced atom numbers, they offer exceptional spatial resolution at the micrometre scale. The experimental apparatus features a cold atom production system capable of reaching quantum degeneracy through a refined cooling sequence that involves optical molasses, magnetic trapping and evaporation, and optical evaporative cooling in the dipole trap, culminating in a 87Rb Bose-Einstein condensate. This work details the development and characterisation of magnetometer set-ups with progressively enhanced performance. The first magnetometer utilised atoms in the optical molasses phase as a sensor, achieving an AC sensitivity of 330 pT/√Hz with approximately 108 atoms at 20 μK. Comprehensive magnetometry optimisation methods were developed to enhance sensitivity. Following laboratory interruptions due to the COVID-19 pandemic, system rebuilding incorporated significant upgrades, including a new probe laser and gradient compensation systems. The improved magnetometer prototype achieved a substantially enhanced sensitivity of 0.72±0.33 pT/√Hz, approaching the fundamental sensitivity limit of the system. Using atoms in the magnetic trap as a sensor, a sensitivity of 1.85 pT/√Hz was demonstrated. The system was verified to be photon-shot noise limited. Investigations into a double-pass probe configuration showed that, while the measured sensitivity was similar to that of the single-pass (4.3 pT/√Hz compared to 3.1 pT/√Hz at a probe power of 6.4 μW measured at the detector), the rotation angle increased by a factor of 2.2, with significantly reduced noise levels. These findings suggest that multi-pass strategies hold promise for enhanced performance in future implementations. In addition, the first signal detection from a BEC magnetometer, achieving 4.5 nT/√Hz with only 95,000 atoms at 35 nK was demonstrated.
The development of an experimental apparatus to produce Bose-Einstein condensates (BECs) of ⁸⁷Rb atoms and their application to magnetometry are discussed. Optical detection of atomic Larmor precession is a widely explored method for high-sensitivity measurements of magnetic fields. In this context, short laser/atom interaction time, atomic thermal diffusion and decoherence effects are among the main limitations. In this thesis, we overcome such problems by using spin-polarised ⁸⁷Rb ultra-cold atoms as the sensing element. After the atoms are polarised, a resonant pulse of radio-frequency excites Larmor precession, which is sensitive to external magnetic fields. By measuring the perturbations of the radio-frequency induced spin precession, information on the magnetic fields of interest. This is achieved by monitoring the polarisation plane’s rotation of a linearly polarised resonant laser probe. In the first part of this thesis, the building and optimisation of a laser-cooling set up to obtain a BEC in a hybrid trap is reported. In order to achieve the Phase Space Density (PSD) required for BEC, several different stages of trapping and cooling are necessary. Each phase has been implemented and optimised. The first step consists in the magneto-optical trap (MOT). Here a velocity dependent damping force and a spatially dependent confining force give the largest changes in PSD. Then atoms are loaded into a hybrid trap obtained by overlapping a quadrupole magnetic potential and a far detuned optical crossed dipole trap. The final stage for the condensation consists of forced evaporative cooling, both via magnetic and optical evaporation. In the second part of the thesis, a general overview of the principles of optical atomic magnetometry is provided and the advantages of using ultra-cold atoms with respect to conventional thermal vapours are discussed. The implementation, operation and a preliminary characterisation of the ultra-cold atom magnetometer are described along with the preliminary results collected. Finally, a plan for future improvements of its sensitivity is presented.
People have been measuring magnetic fields since 200 BC, giving rise to the field of magnetometry. Recently there has been a drive to measure smaller fields with better resolution, resulting in the production of many different types of magnetometers, each with their own unique features. These magnetometers can have a diverse range of applications such as, GNSS free navigation, biomedical sensing, space and weather measurements, and material physics. When designing a magnetomoter there is a trade off between high sensitivity to magnetic fields and high spatial resolution. Currently, there is a unoccupied niche in direct current (DC) magnetometry, that requires a magnetic field sensitivity in the picotesla range and micron scale spatial resolution. Here, I introduce the Bose-Einstein condensate (BEC), which is a macroscopic quantum object, ideal for probing magnetic fields on the nanotesla to picotesla range, with micron scale resolution. This thesis discusses the use of a BEC microscope (BEC-M) to characterise mate- rials with novel applications in nanotechnology by producing 2D current density maps. To produce the atomic probe for microscopy, a BEC in the quasi-1D regime is carefully prepared, requiring an ultra high vacuum (UHV) environment along with custom designed trapping structures, to optically and magnetically confine the atoms. The sensitivity and resolution of the BEC-M makes it an ideal tool for characterising electrical properties of structures on the micron scale such as carbon nanotube (CNT) bundles and biological samples. Current network configuration in samples such as these, can be mapped via a raster scanning procedure. A measurement was made to identify current pathways in CNTs by measuring the atomic distribution of the ultra cold cloud and converting these images to magnetic field and current density maps.
Ultra-cold atoms have small kinetic energy and are therefore very sensitive to external fields that act on the atoms. By having fine control over the positioning of the ultra-cold atom cloud we can use the atom cloud as a sensor for magnetic fields. By imaging these atom clouds we can infer a spatial map of the magnetic field. This spatial map will have a resolution proportional to the distance between the source of the magnetic field and the atom cloud which can be on the order of 0:1 µm. In the first half of the thesis, we investigate the two colour magneto-optical trap. This is a simple technique that can lead to a multiplicative increase in the number of atoms in a magneto-optical trap with a simple change to the optical setup. Using the two colour magneto-optical trap we have observed an increase of 5 times in the number of trapped atoms. An increase in the number of atoms in a magneto-optical helps with later cooling processes that are not lossless such as evaporative cooling which in turn helps the realisation of the ultra-cold atom microscope. In the second half of the thesis, we demonstrate how a 2d current density can be recovered from a 2d magnetic field map generated by the ultra-cold atom microscope. We then go on to show the sensitivity and responsivity of a cold atom cloud and a Bose-Einstein condensate. We then use the results of the previous section to simulate the measurement of currents in a silver nanowire network. Properties of the silver nanowire network can be simulated and aid in showing the abilities and limitations of the ultra-cold atom microscope. We found that the ultra-cold atom microscope can directly measure currents in low-density silver nanowire networks. In a high-density silver nanowire network, the average distance between the wires becomes too small to resolve. Hot-spots, areas of high current density can still be identified using the ultra-cold atom microscope. The ultracold atom microscope could then be used as a tool to aid the research look to use silver nanowires in many industrial applications such as touch screens.
We demonstrate a sensitive spatially resolved magnetometer using a spinor Bose-Einstein condensate (BEC) of 87Rb atoms with increased probe fluence. By performing a probe parameter search using a two-polarization phase contrast imaging technique, we find that the probe-induced atom loss, a major constraint in optical magnetometry with high-density gas, can be reduced. We attain a sensitivity of 5.4(6) mrad for the phase measurement of Larmor precession using a measurement area of $1.4\ifmmode\times\else\texttimes\fi{}{10}^{2}\phantom{\rule{3.33333pt}{0ex}}\ensuremath{\mu}{\mathrm{m}}^{2}$ with a probe fluence of $4.1\ifmmode\times\else\texttimes\fi{}{10}^{5}\phantom{\rule{3.33333pt}{0ex}}\ensuremath{\mu}{\mathrm{m}}^{\ensuremath{-}2}$. A dc magnetic field sensitivity of 5.0(4)pT/Hz is attained with a probe fluence of $3.9\ifmmode\times\else\texttimes\fi{}{10}^{5}\phantom{\rule{4pt}{0ex}}\ensuremath{\mu}{\mathrm{m}}^{\ensuremath{-}2}$. The results should contribute to further enhancement of the sensitivity of a BEC magnetometer.