This thesis presents advancements in radio-frequency atomic magnetometry utilising cold atoms as sensors. While cold atom magnetometers demonstrate lower absolute sensitivity compared to conventional vapour cell systems due to reduced atom numbers, they offer exceptional spatial resolution at the micrometre scale. The experimental apparatus features a cold atom production system capable of reaching quantum degeneracy through a refined cooling sequence that involves optical molasses, magnetic trapping and evaporation, and optical evaporative cooling in the dipole trap, culminating in a 87Rb Bose-Einstein condensate. This work details the development and characterisation of magnetometer set-ups with progressively enhanced performance. The first magnetometer utilised atoms in the optical molasses phase as a sensor, achieving an AC sensitivity of 330 pT/√Hz with approximately 108 atoms at 20 μK. Comprehensive magnetometry optimisation methods were developed to enhance sensitivity. Following laboratory interruptions due to the COVID-19 pandemic, system rebuilding incorporated significant upgrades, including a new probe laser and gradient compensation systems. The improved magnetometer prototype achieved a substantially enhanced sensitivity of 0.72±0.33 pT/√Hz, approaching the fundamental sensitivity limit of the system. Using atoms in the magnetic trap as a sensor, a sensitivity of 1.85 pT/√Hz was demonstrated. The system was verified to be photon-shot noise limited. Investigations into a double-pass probe configuration showed that, while the measured sensitivity was similar to that of the single-pass (4.3 pT/√Hz compared to 3.1 pT/√Hz at a probe power of 6.4 μW measured at the detector), the rotation angle increased by a factor of 2.2, with significantly reduced noise levels. These findings suggest that multi-pass strategies hold promise for enhanced performance in future implementations. In addition, the first signal detection from a BEC magnetometer, achieving 4.5 nT/√Hz with only 95,000 atoms at 35 nK was demonstrated.
This thesis presents advancements in radio-frequency atomic magnetometry utilising cold atoms as sensors. While cold atom magnetometers demonstrate lower absolute sensitivity compared to conventional vapour cell systems due to reduced atom numbers, they offer exceptional spatial resolution at the micrometre scale. The experimental apparatus features a cold atom production system capable of reaching quantum degeneracy through a refined cooling sequence that involves optical molasses, magnetic trapping and evaporation, and optical evaporative cooling in the dipole trap, culminating in a 87Rb Bose-Einstein condensate. This work details the development and characterisation of magnetometer set-ups with progressively enhanced performance. The first magnetometer utilised atoms in the optical molasses phase as a sensor, achieving an AC sensitivity of 330 pT/√Hz with approximately 108 atoms at 20 μK. Comprehensive magnetometry optimisation methods were developed to enhance sensitivity. Following laboratory interruptions due to the COVID-19 pandemic, system rebuilding incorporated significant upgrades, including a new probe laser and gradient compensation systems. The improved magnetometer prototype achieved a substantially enhanced sensitivity of 0.72±0.33 pT/√Hz, approaching the fundamental sensitivity limit of the system. Using atoms in the magnetic trap as a sensor, a sensitivity of 1.85 pT/√Hz was demonstrated. The system was verified to be photon-shot noise limited. Investigations into a double-pass probe configuration showed that, while the measured sensitivity was similar to that of the single-pass (4.3 pT/√Hz compared to 3.1 pT/√Hz at a probe power of 6.4 μW measured at the detector), the rotation angle increased by a factor of 2.2, with significantly reduced noise levels. These findings suggest that multi-pass strategies hold promise for enhanced performance in future implementations. In addition, the first signal detection from a BEC magnetometer, achieving 4.5 nT/√Hz with only 95,000 atoms at 35 nK was demonstrated.
The development of an experimental apparatus to produce Bose-Einstein condensates (BECs) of ⁸⁷Rb atoms and their application to magnetometry are discussed. Optical detection of atomic Larmor precession is a widely explored method for high-sensitivity measurements of magnetic fields. In this context, short laser/atom interaction time, atomic thermal diffusion and decoherence effects are among the main limitations. In this thesis, we overcome such problems by using spin-polarised ⁸⁷Rb ultra-cold atoms as the sensing element. After the atoms are polarised, a resonant pulse of radio-frequency excites Larmor precession, which is sensitive to external magnetic fields. By measuring the perturbations of the radio-frequency induced spin precession, information on the magnetic fields of interest. This is achieved by monitoring the polarisation plane’s rotation of a linearly polarised resonant laser probe. In the first part of this thesis, the building and optimisation of a laser-cooling set up to obtain a BEC in a hybrid trap is reported. In order to achieve the Phase Space Density (PSD) required for BEC, several different stages of trapping and cooling are necessary. Each phase has been implemented and optimised. The first step consists in the magneto-optical trap (MOT). Here a velocity dependent damping force and a spatially dependent confining force give the largest changes in PSD. Then atoms are loaded into a hybrid trap obtained by overlapping a quadrupole magnetic potential and a far detuned optical crossed dipole trap. The final stage for the condensation consists of forced evaporative cooling, both via magnetic and optical evaporation. In the second part of the thesis, a general overview of the principles of optical atomic magnetometry is provided and the advantages of using ultra-cold atoms with respect to conventional thermal vapours are discussed. The implementation, operation and a preliminary characterisation of the ultra-cold atom magnetometer are described along with the preliminary results collected. Finally, a plan for future improvements of its sensitivity is presented.
Spinor Bose-Einstein condensates (BECs) are multi-component superfluids with magnetic interactions, formed from dilute gases of atoms in the Zeeman sublevels mF of a single hyperfine ground state F. Spinor BECs are inherently magnetic quantum objects, and exhibit a multitude of features such as spin domains, magnon excitations, and distinct magnetic phases. At the heart of the magnetic nature of a spinor BEC is the spin-dependent collisional interaction c, which determines the overall magnetic behaviour of the superfluid. In conjunction with the quadratic Zeeman shift q, the magnitude and sign of c give rise to an intricate magnetic phase diagram. The magnetic phase of a spinor BEC is tunable, and c and q are the knobs. In addition to realising quantum simulators of magnetism, spinor BECs are also precise magnetic sensors. Atomic magnetometry measures the Larmor precession frequency of atoms, which is proportional to the magnetic field strength. The sensitivity of an atomic magnetometer is principally dependent on the duration of the measurement (interrogation time) and number of atoms participating in the measurement. BECs are highly suitable as atomic magnetometers, allowing for long interrogation times and high atomic density, with microscopic sensor volumes. The latter is an important consideration, as measurement of small magnetic sources demand equally microscopic sensors. Established forms of magnetometry (such as warm vapour magnetometers) use large sensing volumes and are not trivially miniaturised. The exquisite sensitivity of a spinor BEC to magnetic fields becomes a liability when one studies low energy (~ 1 Hz) spinor physics over long evolution times (100 ms) in a typical laboratory environment. To first order, the spin-collisional interaction is independent of the magnetic field. However, spatially inhomogeneous magnetic fields are problematic, exerting mechanical forces on the magnetically sensitive spin components, suppressing spin collisions and possibly introducing relaxation mechanisms that confound the observation of intrinsic equilibration. Precise characterisation of magnetic field gradients and their cancellation is thus of paramount importance. In this thesis, the interaction of a spinor BEC with its environment is studied. The construction, operation and optimisation of a BEC machine is described in detail, as well as the quantum state preparation and control techniques used. Spin-mixing collisions were studied by observing population oscillations, the characteristic hallmark of such coherent phenomena. The observed population dynamics showed strong evidence of the deleterious effects of magnetic field gradients. A series of experiments were performed using spin-echo pulse sequences to decouple the evolving spinor condensate from the inhomogeneous magnetic environment with encouraging results, but which posed further questions. The fidelity of spin-echo pulses in the strong radiative coupling regime was also studied. Spinor condensates were then employed as sensitive magnetometers to characterise the magnetic landscape they inhabit. A new method of measuring magnetic field gradients was developed, using a pair of spinor BECs separated in space that are simultaneously addressed by a Ramsey interferometry sequence. Combined with a re-orientable magnetic bias field, the resulting gradiometer was used to measure the magnetic field gradient tensor in vacuo. This scheme can be extended to realise a high-precision vector co-magnetometer, with spatiotemporal sensitivity comparable to established forms of magnetometry. Vector light shifts (VLSs) are optically-induced energy shifts that result in effective magnetic fields, which in our case originate from the laser beams used to trap the atoms. The VLS vanishes for purely linearly polarised light, which is experimentally difficult to obtain in vacuo. Small elliptical polarisation imperfections originating from birefringent optics and the glass vacuum cell result in a non-zero shift that contaminates magnetometry measurements. The VLS is spatially varying due to the intensity gradient of the trapping light. Due to gravitational sag of the trapping potential, the spatial variation of the VLS is accentuated, resulting in an effective magnetic field gradient that contributes to dephasing and component separation. The simultaneous Ramsey interferometry experiments are then adapted to measure the VLS-induced Zeeman shift and diagnose its elimination. Up to 99.96% of the VLS is eliminated using this method, and extensions to the technique are described.
This thesis describes the progress achieved towards two goals. One is the construction of a compact magneto-optical trap (MOT) apparatus, used both as a standalone undergraduate laboratory experiment and as part of a public engagement demonstration of cold atom physics. The setup, which utilises a dichroic atomic vapour laser lock (DAVLL) system plus homemade sideband generation electronics, is capable of trapping and cooling up to 8x10⁷ ⁸⁵Rb atoms in a standard six-beam laser cooling scheme. The second goal is the loading of an ultracold ensemble of ⁸⁷Rb atoms into novel optical trap geometries using a phase-only liquid crystal spatial light modulator (LC SLM) for applications to atomtronics and quantum simulation. Details of a double vacuum chamber apparatus, designed to produce the first Bose-Einstein condensates (BECs) at St Andrews, are provided. The setup incorporates a hybrid trap evaporative cooling scheme towards quantum degeneracy and reliably produces BECs of 1.9 10⁵ ⁸⁷Rb atoms. Two computational techniques, developed during the course of this project, are presented with the aim of creating flexible, smooth holographic optical traps. The first method illuminates a single SLM with overlapped, co-propagating light beams of different wavelengths to create a composite optical pattern for atom manipulation. The second uses conjugate gradient minimisation to create exceptionally high fidelity light patterns in both amplitude and phase for light in the output plane. These techniques, combined with the implementation of a light sheet into the experimental setup, are used to trap atoms in both a ring profile and in a set of narrow waveguides connected with a tunnelling barrier.
We report on a radio frequency magnetometer employing a Bose–Einstein condensate of 87Rb atoms held in a dipole trap. An AC sensitivity of 296 pT/Hz is achieved at a probing volume of 3.2×10−8 cm3, leading to a volume-normalized sensitivity of 53 fT/Hz cm−3. At larger probing volumes with the atoms released from the magnetic trap used in the initial phase of the evaporation sequence, the AC sensitivity is improved to 1.4 pT/Hz, allowing a two-mode approach for applications requiring improved sensitivity. Immediate application in high-resolution electromagnetic induction imaging is expected when compared to performance of other induction-based imaging platforms.
Ultra-cold atoms have become indispensable in quantum sensing, quantum computing, and quantum communication applications, as well as in fundamental sciences. In quantum sensing, they enable precision measurements with outstanding sensitivities that can be of great benefit in navigation, geodesy, and fundamental physics applications. The sensitivity of the atom interferometers used herefore typically scales with the square of the interrogation time. Therefore, in atom interferometric measurements, one seeks ensembles that feature a particularly low internal kinetic energy and can thus be detected after a long time-of-flight. The lowest values are achieved using Bose-Einstein condensates in conjunction with delta-kick collimation, a technique for the collimation of the atomic wave function. Bose-Einstein condensation can be achieved using a multi-stage laser cooling scheme, followed by evaporative cooling, which finally brings the temperature down to the critical temperature, typically in the nanokelvin regime. In addition to the low thermal spread, microgravity enables particularly long observation times, as it avoids limitations of the interrogation time due to vacuum chamber constraints, which are present when falling freely under the influence of gravity. Additionally, microgravity enables measurements that are not possible under normal gravity conditions, such as buoyancy-free miscibility studies, truly uniform potentials, and advanced cold atom quantum memories, which are projected to feature unprecedented time-bandwidth products. For the preparation of a Bose-Einstein condensate, two techniques are widely used in science, namely magnetic traps and optical dipole traps. For microgravity missions, magnetic traps on atom chips have been used in nearly all setups so far due to their particularly low SWAP budget and high cold atom flux. In contrast, ground-based experiments often prefer optical traps due to their higher versatility, full optical access, and the absence of surfaces in proximity to the atoms, which is fundamental for precision measurements. Additionally, optical traps enable the manipulation of intra- and inter-species scattering lengths using Feshbach resonances. Compared to atom chip traps, they also feature an intrinsically better symmetry of the trapping potential, in theory leading to fewer aberrations in matter-wave optics. The latter could enable the generation of ensembles in the yet unreached femtokelvin regime using delta-kick collimation with fewer perturbations. This thesis is about the realization of a 1064nm optical dipole trap set up for the microgravity environment of the Bremen Drop Tower. It aims to highlight the advantages of optical traps in conjunction with microgravity and prepare optical trapping technology for use in future microgravity and space missions. The thesis describes the experimental setup, the direct loading process, the characterization of the optical potential, and the optimization and investigation of the evaporative cooling in the optical dipole trap. For the evaporation process, the influence of gravity is comprehensively investigated through analytical calculations and microgravity tests. Bose-Einstein condensation is demonstrated, proving the achievement of condensation through absorption imaging of the spatial distribution, tests on the free evolution of the ensemble, and investigation of the phase-space densities achieved. Up to (74 ± 4)% condensation of an ensemble featuring (30 000 ± 13 000) atoms at a kinetic temperature of (37 ± 3) nK is demonstrated. The evaporation shows high efficiency down to a 3 s evaporation time, while a critical phase-space density can be achieved within (1.29 ± 0.07) s using an even faster evaporation ramp. This opens the door to fundamental physics experiments on Bose-Einstein condensates in microgravity, as well as applications pursuing atomic ensembles with exceptionally low expansion velocities.
Abstract We demonstrate novel implementations of high-precision optical magnetometers which allow for spatially-selective and spatially-resolved in situ measurements using cold atomic clouds. These are realised by using shaped dispersive probe beams combined with spatially-resolved balanced homodyne detection. Two magnetometer sequences are discussed: a vectorial magnetometer, which yields sensitivities two orders of magnitude better compared to a previous realisation and a Larmor magnetometer capable of measuring absolute magnetic fields. We characterise the dependence of single-shot precision on the size of the analysed region for the vectorial magnetometer and provide a lower bound for the measurement precision of magnetic field gradients for the Larmor magnetometer. Finally, we give an outlook on how dynamic trapping potentials combined with selective probing can be used to realise enhanced quantum simulations in quantum gas microscopes.