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arXiv:1811.01515 · Physical Review A

Driven-dissipative dynamics of atomic ensembles in a resonant cavity: Nonequilibrium phase diagram and periodically modulated superradiance

Aniket Patra, B. L. Altshuler, Emil A. Yuzbashyan

Published Mar 1, 2019• 17 citations
arXivHTMLPDF

Abstract

We study the dynamics of two ensembles of atoms (or equivalently, atomic clocks) coupled to a bad cavity and pumped incoherently by a Raman laser. Our main result is the nonequilibrium phase diagram for this experimental setup in terms of two parameters: detuning between the clocks and the repump rate. There are three main phases: a trivial steady state (phase I), where all atoms are maximally pumped, a nontrivial steady state corresponding to monochromatic superradiance (phase II), and amplitude-modulated superradiance (phase III). Phases I and II are fixed points of the mean-field dynamics, while in most of phase III stable attractors are limit cycles. Equations of motion possess an axial symmetry and a ${\mathbb{Z}}_{2}$ symmetry with respect to the interchange of the two clocks. Either one or both of these symmetries are spontaneously broken in various phases. The trivial steady state loses stability via a supercritical Hopf bifurcation bringing about a ${\mathbb{Z}}_{2}$-symmetric limit cycle. The nontrivial steady state goes through a subcritical Hopf bifurcation responsible for coexistence of monochromatic and amplitude-modulated superradiance. Using Floquet analysis, we show that the ${\mathbb{Z}}_{2}$-symmetric limit cycle eventually becomes unstable and gives rise to two ${\mathbb{Z}}_{2}$-asymmetric limit cycles via a supercritical pitchfork bifurcation. Each of the above attractors has its own unique fingerprint in the power spectrum of the light radiated from the cavity. In particular, limit cycles in phase III emit frequency combs---series of equidistant peaks, where the symmetry of the frequency comb reflects the symmetry of the underlying limit cycle. For typical experimental parameters, the spacing between the peaks is several orders of magnitude smaller than the monochromatic superradiance frequency, making the lasing frequency highly tunable.

DOI
10.1103/physreva.99.033802

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We study the dynamics of two ensembles of atoms (or equivalently, atomic clocks) coupled to a bad cavity and pumped incoherently by a Raman laser. Our main result is the nonequilibrium phase diagram for this experimental setup in terms of two parameters: detuning between the clocks and the repump rate. There are three main phases: a trivial steady state (phase I), where all atoms are maximally pumped, a nontrivial steady state corresponding to monochromatic superradiance (phase II), and amplitude-modulated superradiance (phase III). Phases I and II are fixed points of the mean-field dynamics, while in most of phase III stable attractors are limit cycles. Equations of motion possess an axial symmetry and a Z2{\mathbb{Z}}_{2}Z2​ symmetry with respect to the interchange of the two clocks. Either one or both of these symmetries are spontaneously broken in various phases. The trivial steady state loses stability via a supercritical Hopf bifurcation bringing about a Z2{\mathbb{Z}}_{2}Z2​-symmetric limit cycle. The nontrivial steady state goes through a subcritical Hopf bifurcation responsible for coexistence of monochromatic and amplitude-modulated superradiance. Using Floquet analysis, we show that the Z2{\mathbb{Z}}_{2}Z2​-symmetric limit cycle eventually becomes unstable and gives rise to two Z2{\mathbb{Z}}_{2}Z2​-asymmetric limit cycles via a supercritical pitchfork bifurcation. Each of the above attractors has its own unique fingerprint in the power spectrum of the light radiated from the cavity. In particular, limit cycles in phase III emit frequency combs---series of equidistant peaks, where the symmetry of the frequency comb reflects the symmetry of the underlying limit cycle. For typical experimental parameters, the spacing between the peaks is several orders of magnitude smaller than the monochromatic superradiance frequency, making the lasing frequency highly tunable.
Recent experimental advances in the field of cold-atom cavity QED provide a powerful tool for exploring nonequilibrium correlated quantum phenomena beyond conventional condensed-matter scenarios. We present the dynamical phase diagram of a driven Bose-Einstein condensate coupled with the light field of a cavity, with a transverse driving field red-detuned from atomic resonance. We identify regions in parameter space showing dynamical instabilities in the form of limit cycles, which evolve into chaotic behavior in the strong driving limit. Such limit cycles originate from the interplay between cavity dissipation and atom-induced resonance frequency shift, which modifies the phase of cavity mode and gives excessive negative feedback on the atomic density modulation, leading to instabilities of the superradiant scattering. We find interesting merging of the limit cycles related by a Z2{Z}_{2}Z2​ symmetry, and identify a limit cycle formed by purely atomic excitations. The effects of quantum fluctuations and atomic interactions are also investigated.
We study dynamical phases of a driven Bose-Einstein condensate coupled to the light field of a high-Q optical cavity. For high field seeking atoms at red detuning the system is known to show a transition from a spatially homogeneous steady state to a self-ordered regular lattice exhibiting superradiant scattering into the cavity. For blue atom pump detuning the particles are repelled from the maxima of the light-induced optical potential suppressing scattering. We show that this generates a new dynamical instability of the self-ordered phase, leading to the appearance of self-ordered stable limit cycles characterized by large amplitude self-sustained oscillations of both the condensate density and cavity field. The limit cycles evolve into chaotic behavior by period doubling. Large amplitude oscillations of the condensate are accompanied by phase slippage through soliton nucleation at a rate that increases in the chaotic regime. Different from a superfluid in a closed setup, this driven dissipative superfluid is not destroyed by the proliferation of solitons since kinetic energy is removed through cavity losses.
Pattern formation of atoms in high-finesse optical resonators results from the mechanical forces of light associated with superradiant scattering into the cavity mode. It occurs when the laser intensity exceeds a threshold value such that the pumping processes counteract the losses. We consider atoms driven by a laser and coupling with a mode of a standing-wave cavity and describe their dynamics with a Fokker-Planck equation, in which the atomic motion is semiclassical but the cavity field is a full quantum variable. The asymptotic state of the atoms is a thermal state, whose temperature is solely controlled by the detuning between the laser and the cavity frequency and by the cavity loss rate. From this result we derive the free energy and show that in the thermodynamic limit self-organization is a second-order phase transition. The order parameter is the field inside the resonator to which one can associate a magnetization in analogy to ferromagnetism, the control field is the laser intensity, but the steady state is intrinsically out of equilibrium. In the symmetry-broken phase, quantum noise induces jumps of the spatial density between two ordered patterns: We characterize the statistical properties of this temporal behavior at steady state and show that the thermodynamic properties of the system can be extracted by detecting the light at the cavity output. The results of our analysis are in full agreement with previous studies; we extend them by deriving a self-consistent theory which is valid also when the cavity field is in the shot-noise limit and elucidate the nature of the self-organization transition.
We study the effect of spontaneous emission and incoherent atomic pumping on the nonlinear semiclassical dynamics of the unbalanced Dicke model---a generalization of the Dicke model that features independent coupling strengths for the co- and counter-rotating interaction terms. As well as the ubiquitous superradiant behavior the Dicke model is well-known for, the addition of spontaneous emission combined with the presence of strong counter-rotating terms creates a laserlike behavior termed counter-lasing. These states appear in the semiclassical model as stable periodic orbits. We perform a comprehensive dynamical analysis of the appearance of counter-lasing in the unbalanced Dicke model subject to strong cavity dissipation, such that the cavity field can be adiabatically eliminated to yield an effective Lipkin-Meshkov-Glick (LMG) model. If the coupling strength of the corotating interactions is small, then the counter-lasing phase appears via a Hopf bifurcation of the deexcited state. We find that if the rate of spontaneous emission is small, this can lead to resurgent superradiant pulses. However, if the corotating coupling is larger, then the counter-lasing phase must emerge via the steady-state superradiant phase. Such a transition is the result of the competition of the coherent and incoherent processes that drive superradiance and counter-lasing, respectively. We observe a surprisingly complex transition between the two, associated with the formation of a chaotic attractor over a thin transitional parameter region.
We theoretically analyze superradiant emission of light from an ultracold gas of bosonic atoms confined in a bad cavity. A metastable dipolar transition of the atoms couples to the cavity field and is incoherently pumped, and the mechanical effects of cavity-atom interactions tend to order the atoms in the periodic cavity potential. By means of a mean-field model we determine the conditions on the cavity parameters and pump rate that lead to the buildup of a stable macroscopic dipole emitting coherent light. We show that this occurs when the superradiant decay rate and the pump rate exceed threshold values of the order of the photon recoil energy. Above these thresholds superradiant emission is accompanied by the formation of stable matter-wave gratings that diffract the emitted photons. Outside of this regime, instead, the optomechanical coupling can give rise to dephasing or chaos, for which the emitted light is respectively incoherent or chaotic. These behaviors exhibit the features of a dynamical phase transitions and emerge from the interplay between global optomechanical interactions, quantum fluctuations, and noise.
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