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arXiv:2201.12775 · Physical Review Research

Lasing and counter-lasing phase transitions in a cavity-QED system

Kevin C. Stitely, Andrus Giraldo, Bernd Krauskopf, A. S. Parkins

Published May 6, 2022• 14 citations
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Abstract

We study the effect of spontaneous emission and incoherent atomic pumping on the nonlinear semiclassical dynamics of the unbalanced Dicke model---a generalization of the Dicke model that features independent coupling strengths for the co- and counter-rotating interaction terms. As well as the ubiquitous superradiant behavior the Dicke model is well-known for, the addition of spontaneous emission combined with the presence of strong counter-rotating terms creates a laserlike behavior termed counter-lasing. These states appear in the semiclassical model as stable periodic orbits. We perform a comprehensive dynamical analysis of the appearance of counter-lasing in the unbalanced Dicke model subject to strong cavity dissipation, such that the cavity field can be adiabatically eliminated to yield an effective Lipkin-Meshkov-Glick (LMG) model. If the coupling strength of the corotating interactions is small, then the counter-lasing phase appears via a Hopf bifurcation of the deexcited state. We find that if the rate of spontaneous emission is small, this can lead to resurgent superradiant pulses. However, if the corotating coupling is larger, then the counter-lasing phase must emerge via the steady-state superradiant phase. Such a transition is the result of the competition of the coherent and incoherent processes that drive superradiance and counter-lasing, respectively. We observe a surprisingly complex transition between the two, associated with the formation of a chaotic attractor over a thin transitional parameter region.

DOI
10.1103/physrevresearch.4.023101

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We study the effect of spontaneous emission and incoherent atomic pumping on the nonlinear semiclassical dynamics of the unbalanced Dicke model---a generalization of the Dicke model that features independent coupling strengths for the co- and counter-rotating interaction terms. As well as the ubiquitous superradiant behavior the Dicke model is well-known for, the addition of spontaneous emission combined with the presence of strong counter-rotating terms creates a laserlike behavior termed counter-lasing. These states appear in the semiclassical model as stable periodic orbits. We perform a comprehensive dynamical analysis of the appearance of counter-lasing in the unbalanced Dicke model subject to strong cavity dissipation, such that the cavity field can be adiabatically eliminated to yield an effective Lipkin-Meshkov-Glick (LMG) model. If the coupling strength of the corotating interactions is small, then the counter-lasing phase appears via a Hopf bifurcation of the deexcited state. We find that if the rate of spontaneous emission is small, this can lead to resurgent superradiant pulses. However, if the corotating coupling is larger, then the counter-lasing phase must emerge via the steady-state superradiant phase. Such a transition is the result of the competition of the coherent and incoherent processes that drive superradiance and counter-lasing, respectively. We observe a surprisingly complex transition between the two, associated with the formation of a chaotic attractor over a thin transitional parameter region.
In recent years there have been significant advances in the study of many-body interactions between atoms and light confined to optical cavities.One model that has received widespread attention of late is the Dicke model, which under certain conditions exhibits a quantum phase transition to a state in which the atoms collectively emit light into the cavity mode, known as superradiance.We consider a generalization of this model that features independently controllable strengths of the corotating and counter-rotating terms of the interaction Hamiltonian.We study this system in the semiclassical (mean field) limit, i.e., neglecting the role of quantum fluctuations.Under this approximation, the model is described by a set of nonlinear differential equations, which determine the system's semiclassical evolution.By taking a dynamical systems approach, we perform a comprehensive analysis of these equations to reveal an abundance of complex dynamics.Examples of the phenomena that we observe are the emergence of superradiant oscillations arising due to Hopf bifurcations, and the appearance of a pair of chaotic attractors arising from period-doubling cascades, followed by their collision to form a single, larger chaotic attractor via a sequence of infinitely many homoclinic bifurcations.Moreover, we find that a flip of the collective spin can result in the sudden emergence of chaotic dynamics.Overall, we provide a comprehensive road map of the possible dynamics that arise in the unbalanced, open Dicke model in the form of a phase diagram in the plane of the two interaction strengths.Hence, we lay out the foundations to make further advances in the study of the fingerprint of semiclassical chaos when considering the master equation of the unbalanced Dicke model, thus, providing the possibility of studying a manifestation of quantum chaos in a specific, experimentally realizable system.
In 1973 Klaus Hepp and Elliott Lieb showed that a tightly confined ensemble of atoms placed in a quantised single-mode optical cavity will have their emission of light enhanced by constructive interference of emission events if the photons emitted are indistinguishable. This effect, known as superradiance, has proven difficult to realise experimentally due to the strong light-matter coupling required to produce such behaviour. However, over the last decade there have been several successful realisations which engineer superradiance by driving Raman transitions between atomic ground states of multilevel atoms. In this case, superradiance emerges via a quantum phase transition mediated by the laser driving power. In this work, we consider a generalisation of this model referred to as the unbalanced Dicke model. It has recently been implemented experimentally and is characterised by two lasers driving two distinct Raman transitions. We show that, in the semiclassical limit of a large number of atoms, the unbalanced Dicke model exhibits a wealth of nonlinear dynamics which describe novel dynamical phases of matter. Examples of nonlinear behaviour observed are pitchfork, saddle-node, and Hopf bifurcations, as well as two types of chaos. We explore the quantum mechanical manifestations of these bifurcations and additional physical effects which appear in the presence of quantum fluctuations. In this way, the model creates a playground in which to explore the onset of classical nonlinear dynamics from an open quantum system.
We present the non-equilibrium phase diagram of a model which can demonstrate both Dicke-Hepp-Lieb superradiance and regular lasing by varying the coherent and incoherent driving terms We find that the regions in the phase diagram corresponding to superradiance and standard lasing are always separated by a normal region. We analyse the behaviour of the system using a combination of exact numerics based on permutation symmetry of the density matrix for small to intermediate numbers of molecules, and second order cumulant equations for large numbers of molecules. We find that the nature of the photon distribution in the superradiant and lasing states are very similar, but the emission spectrum is very different. We also show that in the presence of both coherent and incoherent driving, a period-doubling route to a chaotic state occurs.
We theoretically analyze superradiant emission of light from an ultracold gas of bosonic atoms confined in a bad cavity. A metastable dipolar transition of the atoms couples to the cavity field and is incoherently pumped, and the mechanical effects of cavity-atom interactions tend to order the atoms in the periodic cavity potential. By means of a mean-field model we determine the conditions on the cavity parameters and pump rate that lead to the buildup of a stable macroscopic dipole emitting coherent light. We show that this occurs when the superradiant decay rate and the pump rate exceed threshold values of the order of the photon recoil energy. Above these thresholds superradiant emission is accompanied by the formation of stable matter-wave gratings that diffract the emitted photons. Outside of this regime, instead, the optomechanical coupling can give rise to dephasing or chaos, for which the emitted light is respectively incoherent or chaotic. These behaviors exhibit the features of a dynamical phase transitions and emerge from the interplay between global optomechanical interactions, quantum fluctuations, and noise.
We present the non-equilibrium phase diagram of a model which can demonstrate both Dicke--Hepp--Lieb superradiance and regular lasing by varying the coherent and incoherent driving terms. We find that the regions in the phase diagram corresponding to superradiance and standard lasing are always separated by a normal region. We analyse the behaviour of the system using a combination of exact numerics based on permutation symmetry of the density matrix for small to intermediate numbers of molecules, and second order cumulant equations for large numbers of molecules. We find that the nature of the photon distribution in the superradiant and lasing states are very similar, but the emission spectrum is very different. We also show that in the presence of both coherent and incoherent driving, a period-doubling route to a chaotic state occurs.
We study a generalization of a recently introduced Dicke trimer model [Phys. Rev. Lett. 128, 163601, Phys. Rev. Research 5, L042016], which allows for cavity losses and unbalanced light-matter interactions (in which rotating and counter-rotating terms can be tuned independently). We find that in the extreme unbalanced limit, the U(1)U(1)U(1) symmetry of the Tavis-Cummings model is restored, qualitatively altering the critical phenomena in the superradiant phase due to the presence of a zero-energy mode. To analyze this general regime, we develop a semiclassical theory based on a re-quantization technique. This theory also provides further physical insight on a recently reported anomalous finite critical fluctuations in the time-reversal broken regime. Moving to the open-Dicke case, by introducing local dissipation to the cavities, we observe the emergence of a rich range of nonequilibrium phases characterized by trivial and non-trivial dynamical signatures. In the former case, we identify, when time-reversal symmetry is present, a new stationary phase that features superradiant states in two of the three cavities and a normal state in the other cavity. In the latter case, we observe the emergence of dynamical phases in which the system exhibits superradiant oscillations, characterized by periodic or chaotic phase space patterns. The landscape of transitions associated with these dynamical phases features a wide range of qualitatively different behaviours such as Hopf bifurcations, anomalous Hopf bifurcations, collisions between basins of attraction, and exterior crises. We highlight how the two-critical-scalings feature of the closed model is robust under dissipation while the phenomenon of anomalous finite critical fluctuations becomes a mean-field scaling in the open model.