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Supperradiant and Lasing States in Driven-Dissipative Dicke Models

Peter Kirton, Jonathan Keeling

Published Oct 17, 2017• 0 citations
OpenAlex

Abstract

We present the non-equilibrium phase diagram of a model which can demonstrate both Dicke--Hepp--Lieb superradiance and regular lasing by varying the coherent and incoherent driving terms. We find that the regions in the phase diagram corresponding to superradiance and standard lasing are always separated by a normal region. We analyse the behaviour of the system using a combination of exact numerics based on permutation symmetry of the density matrix for small to intermediate numbers of molecules, and second order cumulant equations for large numbers of molecules. We find that the nature of the photon distribution in the superradiant and lasing states are very similar, but the emission spectrum is very different. We also show that in the presence of both coherent and incoherent driving, a period-doubling route to a chaotic state occurs.

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We present the non-equilibrium phase diagram of a model which can demonstrate both Dicke--Hepp--Lieb superradiance and regular lasing by varying the coherent and incoherent driving terms. We find that the regions in the phase diagram corresponding to superradiance and standard lasing are always separated by a normal region. We analyse the behaviour of the system using a combination of exact numerics based on permutation symmetry of the density matrix for small to intermediate numbers of molecules, and second order cumulant equations for large numbers of molecules. We find that the nature of the photon distribution in the superradiant and lasing states are very similar, but the emission spectrum is very different. We also show that in the presence of both coherent and incoherent driving, a period-doubling route to a chaotic state occurs.
We present the non-equilibrium phase diagram of a model which can demonstrate both Dicke-Hepp-Lieb superradiance and regular lasing by varying the coherent and incoherent driving terms We find that the regions in the phase diagram corresponding to superradiance and standard lasing are always separated by a normal region. We analyse the behaviour of the system using a combination of exact numerics based on permutation symmetry of the density matrix for small to intermediate numbers of molecules, and second order cumulant equations for large numbers of molecules. We find that the nature of the photon distribution in the superradiant and lasing states are very similar, but the emission spectrum is very different. We also show that in the presence of both coherent and incoherent driving, a period-doubling route to a chaotic state occurs.
We present the non-equilibrium phase diagram of a model which can demonstrate both Dicke–Hepp–Lieb superradiance and regular lasing by varying the coherent and incoherent driving terms We find that the regions in the phase diagram corresponding to superradiance and standard lasing are always separated by a normal region. We analyse the behaviour of the system using a combination of exact numerics based on permutation symmetry of the density matrix for small to intermediate numbers of molecules, and second order cumulant equations for large numbers of molecules. We find that the nature of the photon distribution in the superradiant and lasing states are very similar, but the emission spectrum is very different. We also show that in the presence of both coherent and incoherent driving, a period-doubling route to a chaotic state occurs.
We study the effect of spontaneous emission and incoherent atomic pumping on the nonlinear semiclassical dynamics of the unbalanced Dicke model---a generalization of the Dicke model that features independent coupling strengths for the co- and counter-rotating interaction terms. As well as the ubiquitous superradiant behavior the Dicke model is well-known for, the addition of spontaneous emission combined with the presence of strong counter-rotating terms creates a laserlike behavior termed counter-lasing. These states appear in the semiclassical model as stable periodic orbits. We perform a comprehensive dynamical analysis of the appearance of counter-lasing in the unbalanced Dicke model subject to strong cavity dissipation, such that the cavity field can be adiabatically eliminated to yield an effective Lipkin-Meshkov-Glick (LMG) model. If the coupling strength of the corotating interactions is small, then the counter-lasing phase appears via a Hopf bifurcation of the deexcited state. We find that if the rate of spontaneous emission is small, this can lead to resurgent superradiant pulses. However, if the corotating coupling is larger, then the counter-lasing phase must emerge via the steady-state superradiant phase. Such a transition is the result of the competition of the coherent and incoherent processes that drive superradiance and counter-lasing, respectively. We observe a surprisingly complex transition between the two, associated with the formation of a chaotic attractor over a thin transitional parameter region.
This paper presents a theoretical examination of the non-equilibrium phase diagram of quantum emitters in a plasmonic cavity. The authors generalize driven-dissipative Dicke model to account for the coherent and dissipative interactions between the quantum emitters and the surface plasmon cavity mode. Depending on the interaction strength, the normal, superradiant, regular lasing, and lasing without inversion states are identified. Their signatures in the photon emission spectra are demonstrated.
Control and manipulation of quantum engineered systems allows for the utilization of time-dependent parametric modulations for accessing novel out-of-equilibrium phenomena. In the absence of such driving, the dissipative Dicke model exhibits a fascinating out-of-equilibrium many-body phase transition as a function of a coupling between a driven photonic cavity and numerous two-level atoms. We study the effect of a parametric modulation of this coupling and discover a rich phase diagram as a function of the modulation strength. We find that in addition to the established normal and super-radiant phases, a new phase with pulsed superradiance, which we term dynamical normal phase, appears when the system is parametrically driven. Employing different methods, we characterize the different phases and the transitions between them. Specific heed is paid to the role of dissipation in determining the phase boundaries. Our analysis paves the road for the experimental study of dynamically stabilized phases of interacting light and matter.
In 1973 Klaus Hepp and Elliott Lieb showed that a tightly confined ensemble of atoms placed in a quantised single-mode optical cavity will have their emission of light enhanced by constructive interference of emission events if the photons emitted are indistinguishable. This effect, known as superradiance, has proven difficult to realise experimentally due to the strong light-matter coupling required to produce such behaviour. However, over the last decade there have been several successful realisations which engineer superradiance by driving Raman transitions between atomic ground states of multilevel atoms. In this case, superradiance emerges via a quantum phase transition mediated by the laser driving power. In this work, we consider a generalisation of this model referred to as the unbalanced Dicke model. It has recently been implemented experimentally and is characterised by two lasers driving two distinct Raman transitions. We show that, in the semiclassical limit of a large number of atoms, the unbalanced Dicke model exhibits a wealth of nonlinear dynamics which describe novel dynamical phases of matter. Examples of nonlinear behaviour observed are pitchfork, saddle-node, and Hopf bifurcations, as well as two types of chaos. We explore the quantum mechanical manifestations of these bifurcations and additional physical effects which appear in the presence of quantum fluctuations. In this way, the model creates a playground in which to explore the onset of classical nonlinear dynamics from an open quantum system.