Interactions govern the emergence of collective behaviour in classical and quantum many-body systems. While conservative interactions are well known to generate nonlinear phenomena ranging from self-trapping to pattern formation, it remains largely unexplored whether purely dissipative -- i.e., non-Hermitian -- interactions can give rise to similarly rich dynamics and nontrivial system states. Here, we experimentally realise tuneable non-Hermitian interactions in two coupled condensates of light confined within a dye-filled double-well microcavity. Local coupling to molecular reservoirs generates the effective dissipative photon interactions. We show that the interplay between coherent tunnelling and interactions stabilises limit-cycle oscillations, a hallmark of nonlinear dynamics traditionally associated with Hermitian nonlinearities. By tuning the reservoir coupling, we map out the dynamical phase diagram comprising stable fixed points and limit cycles, thereby demonstrating direct control over the interaction strength. Our experimentally validated model reveals both supercritical and subcritical Hopf bifurcations, giving rise to hysteresis, bistability and excitability. These results validate dissipative interactions as a mechanism for organising collective nonlinear dynamics in driven-dissipative systems and pave the way towards exploring nonequilibrium many-body physics through controlled dissipation.
Interactions govern the emergence of collective behaviour in classical and quantum many-body systems. While conservative interactions are well known to generate nonlinear phenomena ranging from self-trapping to pattern formation, it remains largely unexplored whether purely dissipative -- i.e., non-Hermitian -- interactions can give rise to similarly rich dynamics and nontrivial system states. Here, we experimentally realise tuneable non-Hermitian interactions in two coupled condensates of light confined within a dye-filled double-well microcavity. Local coupling to molecular reservoirs generates the effective dissipative photon interactions. We show that the interplay between coherent tunnelling and interactions stabilises limit-cycle oscillations, a hallmark of nonlinear dynamics traditionally associated with Hermitian nonlinearities. By tuning the reservoir coupling, we map out the dynamical phase diagram comprising stable fixed points and limit cycles, thereby demonstrating direct control over the interaction strength. Our experimentally validated model reveals both supercritical and subcritical Hopf bifurcations, giving rise to hysteresis, bistability and excitability. These results validate dissipative interactions as a mechanism for organising collective nonlinear dynamics in driven-dissipative systems and pave the way towards exploring nonequilibrium many-body physics through controlled dissipation.
Quantum mechanics is fundamentally governed by the Schrödinger equation, which is linear in the wave function. Nevertheless, quantum systems can exhibit highly nonlinear behavior in their observable dynamics. Such nonlinearities can emerge from many-body interactions, nonlinear coupling mechanisms, or the interplay between coherent evolution and dissipation. In the collective limit, microscopic quantum interactions can give rise to qualitatively new macroscopic behavior. Open quantum systems provide a rich setting for such phenomena, as environmental coupling introduces dissipation and fluctuations that compete with coherent dynamics and can alter the steady states and dynamical phases of a system. Combined with nonlinear interactions, this competition can produce behavior with no direct counterpart in conventional linear light--matter systems. In this thesis, I investigate such collective phenomena through nonlinear two-photon light--matter interactions and engineered quantum reservoirs. I first investigate the driven--dissipative two-photon Dicke model and demonstrate the emergence of a dissipative superradiant phase transition. The quadratic light--matter interaction introduces distinct stability requirements in the presence of dissipation. In particular, two-photon loss stabilizes the superradiant phase, allowing its steady states and critical behavior to be characterized. I next investigate photon blockade and transient quadrature-squeezed radiation in the two-photon Tavis--Cummings model. I show that two-photon interactions collectively enhance photon blockade and squeezing, in contrast to the conventional one-photon model, where the effective nonlinearity diminishes in the collective limit. Finally, I consider collective behavior induced by reservoir engineering. Two spatially separated open quantum systems without direct coherent interaction can undergo a nonlocal quantum phase transition when coupled to correlated quantum reservoirs. Remarkably, the transition is hidden from local observables and emerges only through nonlocal correlations and collective observables. Together, these results demonstrate how nonlinear interactions and engineered dissipation can reshape collective behavior in open quantum systems.
We study the dynamics of two ensembles of atoms (or equivalently, atomic clocks) coupled to a bad cavity and pumped incoherently by a Raman laser. Our main result is the nonequilibrium phase diagram for this experimental setup in terms of two parameters: detuning between the clocks and the repump rate. There are three main phases: a trivial steady state (phase I), where all atoms are maximally pumped, a nontrivial steady state corresponding to monochromatic superradiance (phase II), and amplitude-modulated superradiance (phase III). Phases I and II are fixed points of the mean-field dynamics, while in most of phase III stable attractors are limit cycles. Equations of motion possess an axial symmetry and a Z2 symmetry with respect to the interchange of the two clocks. Either one or both of these symmetries are spontaneously broken in various phases. The trivial steady state loses stability via a supercritical Hopf bifurcation bringing about a Z2-symmetric limit cycle. The nontrivial steady state goes through a subcritical Hopf bifurcation responsible for coexistence of monochromatic and amplitude-modulated superradiance. Using Floquet analysis, we show that the Z2-symmetric limit cycle eventually becomes unstable and gives rise to two Z2-asymmetric limit cycles via a supercritical pitchfork bifurcation. Each of the above attractors has its own unique fingerprint in the power spectrum of the light radiated from the cavity. In particular, limit cycles in phase III emit frequency combs---series of equidistant peaks, where the symmetry of the frequency comb reflects the symmetry of the underlying limit cycle. For typical experimental parameters, the spacing between the peaks is several orders of magnitude smaller than the monochromatic superradiance frequency, making the lasing frequency highly tunable.
Reduced abstract. This Thesis explores emergent cooperative phenomena in collective light-matter systems. We study ensembles of interacting quantum emitters coherently driven by a laser field and coupled to photonic structures, focusing on the hybrid description of emitters dressed by light. The interplay among quantum emitters, coherent driving, and photonic environments reveals a rich landscape of cooperative effects. While single-emitter dressing has been widely studied, we address collective phenomena in two non-identical emitters modelled as two-level systems. Strong interaction forms a dimer exhibiting superradiant and subradiant states, with two-photon resonances directly connecting ground and doubly excited states. This nonlinear process, central to the Thesis, enables new regimes of cooperative light-matter physics. Analytical studies show how interactions reshape observables such as emission intensity, photon statistics, and spectra, offering implications for quantum metrology. The sensitivity of two-photon processes to emitter distance and driving strength enables high-precision sensing and sub-wavelength imaging. Unexpectedly, we find that off-resonant virtual states may gain population through dissipation, redefining their role in open systems. To capture this, we develop a hierarchical adiabatic elimination method for metastable dynamics. We also analyze entanglement in emitters coupled to a lossy cavity, identifying five mechanisms, including the frequency-resolved Purcell effect introduced here. This selective enhancement stabilizes cooperative states and enables scalable entanglement. Our models, tailored to solid-state platforms such as quantum dots and molecular aggregates, address challenges like inhomogeneous broadening and decoherence, demonstrating the feasibility of harnessing cooperative light-matter effects for quantum technologies.
Self-sustained oscillations combine finite-amplitude stabilization with a neutral phase degree of freedom. We develop this bifurcation-based framework for driven-dissipative collective spins and show that the microscopic structure of the U(1)-covariant dissipation selects the background attractor, while the explicit U(1)-breaking channel governs its local bifurcation response. In the thermodynamic-limit mean-field dynamics, a single linear U(1)-covariant jump produces only polar fixed-point backgrounds, whereas nonlinear covariant dissipation provides amplitude-dependent saturation and stabilizes a finite-latitude self-sustained-oscillator manifold through a supercritical Hopf bifurcation. Under coherent U(1) breaking, exact resonance leads to a reversible double-zero degeneracy with vanishing critical frequency rather than a standard Hopf onset. Finite detuning unfolds this singularity into a genuine finite-frequency Hopf boundary, which exists only on the self-sustained-oscillator side and can be either supercritical or subcritical. By contrast, a single linear dissipative U(1)-breaking jump cannot generate a standard Hopf instability: when its phase-pinning invariant vanishes the azimuthal direction remains neutral, whereas otherwise the phase-locked fixed points have a purely real Jacobian spectrum. These results establish a general design principle: nonlinear covariant dissipation selects the selfsustained background, while the structure of the symmetry-breaking channel determines whether the resulting local response is double-zero, genuinely Hopf, or non-Hopf.
We propose a general mechanism for generating limit cycle (LC) oscillations by coupling a linear bosonic mode to a dissipative nonlinear bosonic mode. By analyzing the stability matrix, we show that LCs arise due to a supercritical Hopf bifurcation. We find that the existence of LCs is independent of the sign of the effective nonlinear interaction. The bosonic model can be realized in three-level systems interacting with a quantized light mode as realized in atom-cavity systems. Using such a platform, we experimentally observe LCs in an atom-cavity system with attractive optical pump lattice, thereby confirming our theoretical predictions for the minimal model and interactions needed to generate LCs for a class of driven-dissipative systems.
Understanding how strong correlations and dissipation combine to shape collective quantum excitations is a central challenge in many-body physics. We investigate the effect of dissipative light-matter coupling on strongly interacting exciton-polaritons in the presence of a biexciton resonance, which gives rise to polaron-polariton quasiparticles. We show that the interplay between many-body correlations and non-Hermitian coupling generates anomalous dispersion relations and exceptional points in the polaron-polariton spectrum. The location and coexistence of exceptional points are controlled by the dissipative coupling and the relative decay rates of the excitonic and photonic constituents, allowing them to emerge across different polaron-polariton branches. These results identify dissipative polaron-polaritons as a versatile platform for exploring non-Hermitian many-body physics with tunable light-matter quasiparticles.