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arXiv:1808.01287 · Physical review. B./Physical review. B

Population inversion and dynamical phase transitions in a driven superconductor

H. P. Ojeda Collado, J. Lorenzana, Gonzalo Usaj, C. A. Balseiro

Published Dec 27, 2018• 22 citations
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Abstract

We consider a superconductor in which the density of states at the Fermi level or the pairing interaction is driven periodically with a frequency larger than the superconducting gap in the collisionless regime. We show by numerical and analytical computations that a subset of quasiparticle excitations enter into resonance and perform synchronous Rabi oscillations leading to cyclic population inversion with a frequency that depends on the amplitude of the drive. As a consequence a different ``Rabi-Higgs'' mode emerges. Turning off the drive at different times and modulating the strength allows access to all known dynamical phases of the order parameter: persistent oscillations, oscillations with damping and overdamped dynamics. We discuss physical realizations of the drive and methods to detect the dynamics.

DOI
10.1103/physrevb.98.214519

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Ympäristön synnyttämät pysyvät Rabi-oskillaatiot kubitissa

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Decoherence is a quantum-mechanical phenomenon severely limiting quantum information processing and storage capability in quantum computers. Decoherence refers to mechanisms that cause transfer of information from a quantum system to its bath. Typically, in theoretical and experimental considerations of different systems containing superconducting qubits, the coupling strength between a qubit and its bath has been assumed to be constant in time. In this case, many standard results in the dynamics of two-level systems follow. For example, due to decoherence, driven Rabi oscillations in a qubit have a characteristic decay time. In addition, the oscillations may take place at any phase. However, by considering time-dependent coupling to the bath, these phenomena may be absent. In this thesis, we demonstrate with numerical simulations of a time-dependent Lindblad master equation persistent Rabi oscillations in a qubit driven by a coherent drive tone. The persistent Rabi oscillations are induced by modulating the coupling of the qubit to the bath with a sinusoidal temporal shape. We observe that the temporal modulation enforces a limit cycle on the evolution of the dressed qubit state with a fixed phase relative to the phase of the sinusoidal modulation regardless of the initial state of the system. Through a synchronization-like phenomenon, the frequency of the Rabi oscillation adapts to match the frequency of the modulation. We determine the effect of different system parameters on the limit cycle and study how the amplitude of the persistent oscillation depends on the coupling modulation parameters. We also observe a similar effect in the freely evolving qubit precession. In addition, the qubit acts as a non-linear mixer, resulting in different linear combinations of the original modulation waveform appearing in the bath-induced Rabi oscillations. We also introduce a design for a physical system where our simulations can be verified experimentally.

•Mar 12, 2019•0 citations
We consider a superconductor in which the density of states at the Fermi level or the pairing interaction is driven periodically with a frequency larger than the superconducting gap in the collisionless regime. We show by numerical and analytical computations that a subset of quasiparticle excitations enter into resonance and perform synchronous Rabi oscillations leading to cyclic population inversion with a frequency that depends on the amplitude of the drive. As a consequence a different ``Rabi-Higgs'' mode emerges. Turning off the drive at different times and modulating the strength allows access to all known dynamical phases of the order parameter: persistent oscillations, oscillations with damping and overdamped dynamics. We discuss physical realizations of the drive and methods to detect the dynamics.
We present a systematic study of the dynamical phase diagram of a periodically driven BCS system as a function of drive strength and frequency. Three different driving mechanisms are considered and compared: oscillating density of states, oscillating pairing interaction, and oscillating external paring field. We identify the locus in parameter space of parametric resonances and four dynamical phases: Rabi-Higgs, gapless, synchronized Higgs, and time-crystal phases. We demonstrate that the main features of the phase diagram are quite robust to different driving protocols and discuss the order of the transitions. By mapping the BCS problem to a collection of nonlinear and interacting classical oscillators, we shed light on the origin of time-crystal phases and parametric resonances appearing for subgap excitations.
In the absence of dissipation a periodically driven BCS superconductor can enter a coherent nonlinear regime of collective Rabi oscillations which last for arbitrary long times [Ojeda Collado et al., Phys. Rev. B 98, 214519 (2018)]. Here we show that dissipation effects introduce dramatic changes: (i) The collective Rabi mode becomes a transient. (ii) At long times a steady state is reached showing strong nonlinear effects for large enough drive strength. We identify the physical parameters governing the various crossovers and present a detailed computation of time- and angle-resolved photoemission spectroscopy (tr-ARPES) and time-resolved tunneling spectra aiming at detecting the collective Rabi oscillations and the steady-state nonlinearities. We show also that second harmonic generation is allowed for a drive which acts on the BCS coupling constant.
Fermi gas with time-dependent pairing interaction hosts several different dynamical states. Coupling between the collective BCS pairing mode and individual Cooper pair states can make the latter either synchronize or dephase. We describe transition from phase-locked undamped oscillations to Landau-damped dephased oscillations in the collisionless, dissipationless regime as a function of coupling strength. In the dephased regime, we find a second transition at which the long-time asymptotic pairing amplitude vanishes. Using a combination of numerical and analytical methods we establish a continuous (type II) character of both transitions.
We find nonequilibrium phase transitions accompanied by multiple (nested) hysteresis behaviors in superconductors coupled to baths under a time-periodic light driving. The transitions are demonstrated with a full phase diagram in the domain of the driving amplitude and frequency by means of the Floquet many-body theory. In the weak-driving regime with a frequency smaller than half of the superconducting gap, excited quasiparticles are accumulated at the far edges of the bands, realizing a distribution reminiscent of the Eliashberg effect, which suddenly becomes unstable in the strong-driving regime due to multiphoton-assisted tunneling across the gap mediated by the in-gap Floquet sidebands. We also show that superconductivity is enhanced in the weak-driving regime without effective cooling, which is attributed to the modulation of the spectrum due to Floquet sidebands.
This thesis reports on theoretical investigations of the ultrafast nonequilibrium dynamics in superconductors. In particular, two nonequilibrium scenarios are modeled by combining several analytical and numerical methods: transient superconducting phase transition and collective excitations of a superconducting condensate. In the first part of the thesis the possibility to induce singlet superconducting correlations far from equilibrium is explored by applying time-dependent Lanczos algorithm to the one-dimensional extended Hubbard model. Here, the system is driven into a nonequilibrium state by (i) interaction quench and (ii) quench by pulse. In both cases the buildup of the superconducting correlations is studied in view of several correlation functions. Moreover, a transient Meissner effect, which reflects fingerprints of the induced superconductivity, is observed in calculations of the important for experiments time-dependent optical conductivity. In addition, the differences between nonequilibrium dynamics of the extended Hubbard model initiated by interaction quench and by pulse quench are discussed in detail. The second part is devoted to the excitation of collective modes in a superconductor out of equilibrium. First of all, focus is given to the properties of collective modes close to equilibrium conditions, where a linearized response can be expected. Within the framework of the (Nambu-) matrix kinetic theory in the clean limit a comprehensive gauge-invariant description of the collective modes associated with phase fluctuations of the order parameter is analytically formulated for the generalized case of two- band superconducting systems. Particular emphasis is on the application to the recently discovered noncentrosymmetric superconductors. A detailed analysis of the collective modes includes specification of the gauge mode (common to all superconductors) and the Leggett mode (collective fluctuations of the interband phase difference), and investigation of their subtle interplay in view of validity of the charge conservation law and the participation in the Anderson-Higgs mechanism. Further, the nonequilibrium excitation of the superconducting gaps for the case of two-band superconductors with singlet pairing correlations is investigated in a view of optical pump-probe experiments. For this purpose a semi-numerical method based on the density- matrix theory is formulated. In this case additional amplitude (Higgs) modes were identified, which allow to directly detect the properties of the superconducting condensates as a function of time. Moreover, a new interplay between the phase (Leggett) and amplitude (Higgs) modes is studied in detail. In particular it was found that the nonadiabatic excitation process leads to strong coupling between both modes. Finally, based on calculations of the time-dependent optical conductivity the prediction is made that the coupled Higgs and Leggett modes can be clearly visible in the pump-probe absorption spectra.
Decoherence is a quantum-mechanical phenomenon severely limiting quantum information processing and storage capability in quantum computers. Decoherence refers to mechanisms that cause transfer of information from a quantum system to its bath. Typically, in theoretical and experimental considerations of different systems containing superconducting qubits, the coupling strength between a qubit and its bath has been assumed to be constant in time. In this case, many standard results in the dynamics of two-level systems follow. For example, due to decoherence, driven Rabi oscillations in a qubit have a characteristic decay time. In addition, the oscillations may take place at any phase. However, by considering time-dependent coupling to the bath, these phenomena may be absent. In this thesis, we demonstrate with numerical simulations of a time-dependent Lindblad master equation persistent Rabi oscillations in a qubit driven by a coherent drive tone. The persistent Rabi oscillations are induced by modulating the coupling of the qubit to the bath with a sinusoidal temporal shape. We observe that the temporal modulation enforces a limit cycle on the evolution of the dressed qubit state with a fixed phase relative to the phase of the sinusoidal modulation regardless of the initial state of the system. Through a synchronization-like phenomenon, the frequency of the Rabi oscillation adapts to match the frequency of the modulation. We determine the effect of different system parameters on the limit cycle and study how the amplitude of the persistent oscillation depends on the coupling modulation parameters. We also observe a similar effect in the freely evolving qubit precession. In addition, the qubit acts as a non-linear mixer, resulting in different linear combinations of the original modulation waveform appearing in the bath-induced Rabi oscillations. We also introduce a design for a physical system where our simulations can be verified experimentally.