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arXiv:2503.10146 · Physical review. B./Physical review. B

Nonequilibrium hysteretic phase transitions in periodically light-driven superconductors

Huanyu Zhang, Kazuaki Takasan, Naoto Tsuji

Published Nov 26, 2025• 0 citations
arXivHTMLPDF

Abstract

We find nonequilibrium phase transitions accompanied by multiple (nested) hysteresis behaviors in superconductors coupled to baths under a time-periodic light driving. The transitions are demonstrated with a full phase diagram in the domain of the driving amplitude and frequency by means of the Floquet many-body theory. In the weak-driving regime with a frequency smaller than half of the superconducting gap, excited quasiparticles are accumulated at the far edges of the bands, realizing a distribution reminiscent of the Eliashberg effect, which suddenly becomes unstable in the strong-driving regime due to multiphoton-assisted tunneling across the gap mediated by the in-gap Floquet sidebands. We also show that superconductivity is enhanced in the weak-driving regime without effective cooling, which is attributed to the modulation of the spectrum due to Floquet sidebands.

DOI
10.1103/m6f9-w9nz

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We find nonequilibrium phase transitions accompanied by multiple (nested) hysteresis behaviors in superconductors coupled to baths under a time-periodic light driving. The transitions are demonstrated with a full phase diagram in the domain of the driving amplitude and frequency by means of the Floquet many-body theory. In the weak-driving regime with a frequency smaller than half of the superconducting gap, excited quasiparticles are accumulated at the far edges of the bands, realizing a distribution reminiscent of the Eliashberg effect, which suddenly becomes unstable in the strong-driving regime due to multiphoton-assisted tunneling across the gap mediated by the in-gap Floquet sidebands. We also show that superconductivity is enhanced in the weak-driving regime without effective cooling, which is attributed to the modulation of the spectrum due to Floquet sidebands.
We perform a systematic analysis of the influence of phonon driving on the superconducting Hol- stein model coupled to heat baths by studying both the transient dynamics and the nonequilibrium steady state (NESS) in the weak and strong electron-phonon coupling regimes. Our study is based on the nonequilibrium dynamical mean-field theory, and for the NESS we present a Floquet formu- lation adapted to electron-phonon systems. The analysis of the phonon propagator suggests that the effective attractive interaction can be strongly enhanced in the parametric resonant regime because of the Floquet side bands. While this may be expected to enhance the superconductivity (SC), our fully self-consistent calculations, which include the effects of heating and nonthermal distributions, show that the parametric phonon driving generically results in a suppression or complete melting of the SC order. In the strong coupling regime, the NESS always shows a suppression of the SC gap, the SC order parameter and the superfluid density as a result of the driving, and this tendency is most prominent at the parametric resonance. Using the real-time nonequilibrium DMFT formalism, we also study the dynamics towards the NESS, which shows that the heating effect dominates the transient dynamics, and SC is weakened by the external modulations, in particular at the parametric resonance. In the weak coupling regime, we find that the SC fluctuations above the transition tem- perature are generally weakened under the driving. The strongest suppression occurs again around the parametric resonance because of the efficient energy absorption.
We consider a superconductor in which the density of states at the Fermi level or the pairing interaction is driven periodically with a frequency larger than the superconducting gap in the collisionless regime. We show by numerical and analytical computations that a subset of quasiparticle excitations enter into resonance and perform synchronous Rabi oscillations leading to cyclic population inversion with a frequency that depends on the amplitude of the drive. As a consequence a different ``Rabi-Higgs'' mode emerges. Turning off the drive at different times and modulating the strength allows access to all known dynamical phases of the order parameter: persistent oscillations, oscillations with damping and overdamped dynamics. We discuss physical realizations of the drive and methods to detect the dynamics.
The optical manipulation of phonon degrees of freedom can change the effective interactions in solids and potentially enhance superconductivity. However, heating and nonthermal energy distributions need to be considered to understand the ultimate effects of such a driving on ordered states. Using nonequilibrium dynamical mean field theory in the Kadanoff-Baym and Floquet implementation, the authors systematically discuss the effects of parametric phonon driving on conventional superconductivity. Both the transient dynamics of isolated systems and the nonequilibrium steady states in driven-dissipative systems are considered. While the phonon-mediated attractive interaction can be enhanced in certain driving regimes because of Floquet phonon sidebands, the heating and nonthermal distribution effects dominate and generically result in a suppression of superconductivity.
A saddle point plus fluctuation analysis of the periodically driven half-filled two-dimensional Hubbard model is performed. For drive frequencies below the equilibrium gap, we find discontinuous transitions to time-dependent solutions. A highly excited, generically nonthermal distribution of magnons occurs even for drive frequencies far above the gap. Above a critical drive amplitude, the low-energy magnon distribution diverges as the frequency tends to zero and antiferromagnetism is destroyed, revealing the generic importance of collective mode excitations arising from a nonequilibrium drive.
Abstract Non-equilibrium engineering is becoming a seminal way for realising novel quantum phases that are unimaginable in equilibrium. In particular, Floquet theory applied to quantum mechanics revealed that we can even control the band topology in semimetallic/insulating systems, while the straightforward application to topological superconductivity fails for typical superconductors because the supercondicting gap function does not couple to the electromagnetic field in a direct manner. Here we show that we can overcome this difficulty by taking account of correlation effects. Namely, we study how a d-wave superconductivity is changed when illuminated by circularly-polarised light (CPL) in the repulsive Hubbard model in the strong-coupling regime. We adopt the Floquet formalism for the Gutzwiller-projected effective Hamiltonian with the time-periodic Schrieffer-Wolff transformation. We find that CPL induces a topological superconductivity with a d + id pairing, which arises from the chiral spin coupling and the three-site term generated by the CPL. The latter term remains significant even for low frequencies and low intensities of the CPL. This is clearly reflected in the obtained phase diagram against the laser intensity and temperature for various frequencies red-detuned from the Hubbard U, with the transient dynamics also examined. The phenomenon revealed here can open a novel, dynamical way to induce a topological superconductivity.
Abstract Periodically driven systems provide a novel route to control the topology of quantum materials. In particular, Floquet theory allows an effective band description of periodically-driven systems through the Floquet Hamiltonian. Here, we study the time evolution of d-wave superconductors irradiated with intense circularly-polarized laser light. We consider the Floquet t–J model with time-periodic interactions, and investigate its mean-field dynamics by formulating the time-dependent Gutzwiller approximation. We observe the development of the idxy-wave pairing amplitude along with the original dx2−y2{d}_{{x}^{2}-{y}^{2}}dx2−y2​ d x 2 − y 2 -wave order upon gradual increasing of the field amplitude. We further numerically construct the Floquet Hamiltonian for the steady state, with which we identify the system as the fully-gapped d + id superconducting phase with a nonzero Chern number. We explore the low-frequency regime where the perturbative approaches in the previous studies break down, and find that the topological gap of an experimentally-accessible size can be achieved at much lower laser intensities.