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arXiv:1909.12310 · Physical review. B./Physical review. B

Nonlinear dynamics of driven superconductors with dissipation

H. P. Ojeda Collado, Gonzalo Usaj, J. Lorenzana, C. A. Balseiro

Published Feb 6, 2020• 15 citations
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Abstract

In the absence of dissipation a periodically driven BCS superconductor can enter a coherent nonlinear regime of collective Rabi oscillations which last for arbitrary long times [Ojeda Collado et al., Phys. Rev. B 98, 214519 (2018)]. Here we show that dissipation effects introduce dramatic changes: (i) The collective Rabi mode becomes a transient. (ii) At long times a steady state is reached showing strong nonlinear effects for large enough drive strength. We identify the physical parameters governing the various crossovers and present a detailed computation of time- and angle-resolved photoemission spectroscopy (tr-ARPES) and time-resolved tunneling spectra aiming at detecting the collective Rabi oscillations and the steady-state nonlinearities. We show also that second harmonic generation is allowed for a drive which acts on the BCS coupling constant.

DOI
10.1103/physrevb.101.054502

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In the absence of dissipation a periodically driven BCS superconductor can enter a coherent nonlinear regime of collective Rabi oscillations which last for arbitrary long times [Ojeda Collado et al., Phys. Rev. B 98, 214519 (2018)]. Here we show that dissipation effects introduce dramatic changes: (i) The collective Rabi mode becomes a transient. (ii) At long times a steady state is reached showing strong nonlinear effects for large enough drive strength. We identify the physical parameters governing the various crossovers and present a detailed computation of time- and angle-resolved photoemission spectroscopy (tr-ARPES) and time-resolved tunneling spectra aiming at detecting the collective Rabi oscillations and the steady-state nonlinearities. We show also that second harmonic generation is allowed for a drive which acts on the BCS coupling constant.
We consider a superconductor in which the density of states at the Fermi level or the pairing interaction is driven periodically with a frequency larger than the superconducting gap in the collisionless regime. We show by numerical and analytical computations that a subset of quasiparticle excitations enter into resonance and perform synchronous Rabi oscillations leading to cyclic population inversion with a frequency that depends on the amplitude of the drive. As a consequence a different ``Rabi-Higgs'' mode emerges. Turning off the drive at different times and modulating the strength allows access to all known dynamical phases of the order parameter: persistent oscillations, oscillations with damping and overdamped dynamics. We discuss physical realizations of the drive and methods to detect the dynamics.
Within the time-dependent Gutzwiller approximation applied to the negative-UUU Hubbard model, we investigate the dynamics of a superconductor after an interaction quench for different values of the final interaction from weak to strong coupling. The equilibrium BCS-BEC crossover becomes a sharp transition in the out-of-equilibrium dynamics between weak- and strong-coupling dynamical phases. Two different frequencies (${\mathrm{\ensuremath{\Omega}}}_{J}<{\mathrm{\ensuremath{\Omega}}}_{U}$) dominate the order parameter dynamics. In the weak coupling phase, ${\mathrm{\ensuremath{\Omega}}}_{J}$ follows twice the asymptotic average value of the gap (${\mathrm{\ensuremath{\Omega}}}_{J}\ensuremath{\approx}2{\mathrm{\ensuremath{\Delta}}}_{\ensuremath{\infty}}$) and ${\mathrm{\ensuremath{\Omega}}}_{U}$ is much larger but hardy visible in the anomalous density. At long times the BCS dynamics is recovered but surprisingly differences remain during the transient phase. In the strong coupling phase, the dynamics decouples from the asymptotic value of the order parameter except at exactly half filling and close to the dynamical transition where ${\mathrm{\ensuremath{\Omega}}}_{U}\ensuremath{\approx}2{\mathrm{\ensuremath{\Delta}}}_{\ensuremath{\infty}}$. The out-of-equilibrium transient spectral density and optical conductivity are presented and discussed in relation to pump probe experiments. Both ${\mathrm{\ensuremath{\Omega}}}_{J}$ and ${\mathrm{\ensuremath{\Omega}}}_{U}$ give rise to a complex structure of self-driven slow Rabi oscillations which are visible in the nonequilibrium optical conductivity where also sidebands appear due to the modulation of the double occupancy by superconducting amplitude oscillations. Analogous results apply to CDW and SDW systems. Our results show that in systems with long coherence times, pump-probe experiments allow us to characterize the regime (BCS vs preformed pairs) through very specific out-of-equilibrium fingerprints.
We present a systematic study of the dynamical phase diagram of a periodically driven BCS system as a function of drive strength and frequency. Three different driving mechanisms are considered and compared: oscillating density of states, oscillating pairing interaction, and oscillating external paring field. We identify the locus in parameter space of parametric resonances and four dynamical phases: Rabi-Higgs, gapless, synchronized Higgs, and time-crystal phases. We demonstrate that the main features of the phase diagram are quite robust to different driving protocols and discuss the order of the transitions. By mapping the BCS problem to a collection of nonlinear and interacting classical oscillators, we shed light on the origin of time-crystal phases and parametric resonances appearing for subgap excitations.
We perform time resolved photoelectron spectroscopy measurements of optimally doped $\tn{Bi}_2\tn{Sr}_2\tn{CaCu}_2\tn{O}_{8+δ}$ (Bi-2212) and $\tn{Bi}_2\tn{Sr}_{2-x}\tn{La}_{x}\tn{Cu}\tn{O}_{6+δ}$ (Bi-2201). The electrons dynamics show that inelastic scattering by nodal quasiparticles decreases when the temperature is lowered below the critical value of the superconducting phase transition. This drop of electronic dissipation is astonishingly robust and survives to photoexcitation densities much larger than the value sustained by long-range superconductivity. The unconventional behaviour of quasiparticle scattering is ascribed to superconducting correlations extending on a length scale comparable to the inelastic path. Our measurements indicate that strongly driven superconductors enter in a regime without phase coherence but finite pairing amplitude. The latter vanishes near to the critical temperature and has no evident link with the pseudogap observed by Angle Resolved Photoelectron Spectroscopy (ARPES).
The BCS model of an isolated superconductor initially prepared in a nonequilibrium state predicts the existence of interesting dynamical phenomena in the time-dependent order parameter as decaying oscillations, persistent oscillations, and overdamped dynamics. To make contact with real systems remains an open challenge as one needs to introduce dissipation due to the environment in a self-consistent computation. Here, we reach this goal with the use of the Keldysh formalism to treat the effect of a thermal bath. We show that, contrary to the dissipationless case, all dynamical phases reach the equilibrium order parameter in a characteristic time that depends on the coupling with the bath. Remarkably, as time evolves, the overdamped phase shows a fast crossover where the superconducting order parameter recovers to reach a state with a well-developed long range order that tends towards equilibrium with the damped Higgs mode oscillations. Our results provide a benchmark for the description of the dynamics of real out-of-equilibrium superconductors relevant for quantum technological applications.
Recent experiments on cuprates have shown the possibility of opening a gap above the superconducting critical temperature, in the so-called phase-fluctuating state, by enhancing the phase coherence of preformed Cooper pairs. Quench-drive spectroscopy, an implementation of 2D coherent spectroscopy, has emerged as a powerful tool for investigating out-of-equilibrium superconductors and their collective modes. In this paper, we enrich the quench-drive scheme by developing a systematic generalization to study the nonlinear response of d -wave incoherent Cooper pairs in a symmetry-resolved manner. In particular, we not only show that it is possible to obtain a third-harmonic signal from fully incoherent pairs with an equilibrium vanishing order parameter, but we also characterize the full flourishing 2D spectrum of the generated nonlinear response. The results provide a deeper theoretical insight on recent experimental results, opening the door to a symmetry-driven design of future experiments on unconventional and enhanced superconductors. Published by the American Physical Society 2024