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arXiv:1803.10663 · New Journal of Physics

Dissipative cooling of spin chains by a bath of dipolar particles

M Robert-de-Saint-Vincent, P. Pedri, B. Laburthe-Tolra

Published Jul 5, 2018• 3 citations
arXivHTMLPDF

Abstract

We consider a spin chain of fermionic atoms in an optical lattice, interacting with each other by super-exchange interactions. We theoretically investigate the dissipative evolution of the spin chain when it is coupled by magnetic dipole–dipole interaction to a bath consisting of atoms with a strong magnetic moment. Dipolar interactions with the bath allow for a dynamical evolution of the collective spin of the spin chain. Starting from an uncorrelated thermal sample, we demonstrate that the dissipative cooling produces highly entangled low energy spin states of the chain in a timescale of a few seconds. In practice, the lowest energy singlet state driven by super-exchange interactions is efficiently produced. This dissipative approach is a promising alternative to cool spin-full atoms in spin-independent lattices. It provides direct thermalization of the spin degrees of freedom, while traditional approaches are plagued by the inherently long timescale associated to the necessary spatial redistribution of spins under the effect of super-exchange interactions.

DOI
10.1088/1367-2630/aad141

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We consider a spin chain of fermionic atoms in an optical lattice, interacting with each other by super-exchange interactions. We theoretically investigate the dissipative evolution of the spin chain when it is coupled by magnetic dipole–dipole interaction to a bath consisting of atoms with a strong magnetic moment. Dipolar interactions with the bath allow for a dynamical evolution of the collective spin of the spin chain. Starting from an uncorrelated thermal sample, we demonstrate that the dissipative cooling produces highly entangled low energy spin states of the chain in a timescale of a few seconds. In practice, the lowest energy singlet state driven by super-exchange interactions is efficiently produced. This dissipative approach is a promising alternative to cool spin-full atoms in spin-independent lattices. It provides direct thermalization of the spin degrees of freedom, while traditional approaches are plagued by the inherently long timescale associated to the necessary spatial redistribution of spins under the effect of super-exchange interactions.
We study the classic problem concerning the dissipative dynamics of a system of two interacting spin-1/21/21/2 particles, coupled to a thermal bath. In particular, we consider the case of a resonant excitation of the initial single-spin coherences and examine the consequences of the interplay between this excitation and the spin-spin dipolar coupling. Using a fluctuation-regulated Quantum Master Equation (frQME) [Phys. Rev. A 97, 063837 (2018)] we show that the relevant dissipator consists of cross-terms between the drive and the dipolar Hamiltonian, apart from regular self-terms responsible for ordinary relaxation effects. The drive-dipole cross-correlations provide for a novel second-order coupling of single and two-spin observables in the Zeeman basis, which cannot be classified as a dissipative effect. We show that the presence of these unique second-order non-dissipative terms lead to the well-known spin-locked steady-states in dipolar spin-ensembles. Importantly, the mathematical form of the steady-state magnetization in the spin-locked phase, obtained from our theory, matches with the prediction of the traditional spin-temperature based methods used to describe such phenomena.
We investigate how two spatially separated qubits coupled to a common heat bath can be entangled by purely dissipative dynamics. We identify a dynamical time scale associated with the lifetime of the dissipatively generated entanglement and show that it can be much longer than either the typical single-qubit decoherence time or the time scale on which a direct exchange interaction can entangle the qubits. We give an approximate analytical expression for the long-time evolution of the qubit concurrence and propose an ion trap scheme in which such dynamics should be observable.
Understanding quantum thermalization through entanglement build up in isolated quantum systems addresses fundamental questions on how unitary dynamics connects to statistical physics. Spin systems made of long-range interacting atoms offer an ideal experimental platform to investigate this question. Here, we study the spin dynamics and approach towards local thermal equilibrium of a macroscopic ensemble of S = 3 chromium atoms pinned in a three dimensional optical lattice and prepared in a pure coherent spin state, under the effect of magnetic dipole-dipole interactions. Our isolated system thermalizes under its own dynamics, reaching a steady state consistent with a thermal ensemble with a temperature dictated from the system's energy. The build up of quantum correlations during the dynamics is supported by comparison with an improved numerical quantum phase-space method. Our observations are consistent with a scenario of quantum thermalization linked to the growth of entanglement entropy.
Understanding quantum thermalization through entanglement build-up in isolated quantum systems addresses fundamental questions on how unitary dynamics connects to statistical physics. Here, we study the spin dynamics and approach towards local thermal equilibrium of a macroscopic ensemble of S = 3 spins prepared in a pure coherent spin state, tilted compared to the magnetic field, under the effect of magnetic dipole-dipole interactions. The experiment uses a unit filled array of 104 chromium atoms in a three dimensional optical lattice, realizing the spin-3 XXZ Heisenberg model. The buildup of quantum correlation during the dynamics, especially as the angle approaches pi/2, is supported by comparison with an improved numerical quantum phase-space method and further confirmed by the observation that our isolated system thermalizes under its own dynamics, reaching a steady state consistent with the one extracted from a thermal ensemble with a temperature dictated from the system's energy. This indicates a scenario of quantum thermalization which is tied to the growth of entanglement entropy. Although direct experimental measurements of the Renyi entropy in our macroscopic system are unfeasible, the excellent agreement with the theory, which can compute this entropy, does indicate entanglement build-up.
We investigate collective behaviour that appears in open, many-body systems of two- and four-level atoms. Here, ``open" refers to the system interacting with an external environment that causes dissipation. We derive a general open quantum master equation to describe the system dynamics only, independent of this environment. We identify processes such as coherent exchange of virtual photons and modified decay rates caused by long-range interactions between all pairs of atoms that scale with distance by inverse power laws. We explore excitation transport within a one-dimensional chain of atoms where the atomic transition dipoles are coupled to the free radiation field. When the interatomic spacing is smaller than or comparable to the wavelength of light associated with the photon emitted from a given transition, virtual photon exchange interactions facilitate excitation transport through the chain. Atomic systems coupled to an environment display dissipative dynamics, however subradiant transport is exhibited from a variety of initial states; spontaneous emission from the chain occurs at a rate much slower than that for an individual atom. In particular, we find a region within the decay spectrum that consists entirely of subradiant states with a corresponding linear dispersion relation in the interaction energy. Identifying this subspace allows for the dispersionless transport of wave packets over long distances with near-zero decay. Moreover, the group velocity of the wave packet and direction of the transport can be controlled via an external uniform magnetic field while preserving its subradiant character. We discuss a number of experimental considerations to justify the feasibility and robustness of this protocol. Initial state preparation is outlined, utilising external laser driving to excite the system into the single excitation sector. Furthermore, we consider positional disorder by explicitly accounting for the external atomic degrees of freedom -- position and momentum -- which allows us to model the positions of all atoms by a motional state representing the occupation of a lattice well with a given width. These discussions are made in the low-temperature limit, where the atomic motion is essentially frozen, and we identify that subradiant transport is indeed robust. Finally, we explore the experimental limits of interatomic spacing and imperfect filling within an experimentally achievable optical lattice. We calculate the photon emission rate -- an experimentally measurable quantity -- and compare the emission spectra to our analysis. By limiting parameters to those achieved experimentally, we observe a reduction, yet not an absence, of collective behaviour. The simplicity and versatility of this system, together with the robustness of subradiance against disorder, makes it relevant for a range of applications such as lossless energy transport and long-time light storage. The lifetime of an atomic excitation could be increased by a factor of thousands to millions for a chain of atoms under the conditions that we explore in this thesis.
The modular path integral methodology is used to extend the well-known spin-boson dynamics to finite-length quantum Ising chains, where each spin is coupled to a dissipative harmonic bath. The chain is initially prepared in the ferromagnetic phase where all spins are aligned, and the magnetization is calculated with spin-spin coupling parameters corresponding to the paramagnetic phase, mimicking a quantum quench experiment. The observed dynamics is found to depend significantly on the location of the tagged spin. In the absence of a dissipative bath, the time evolution displays irregular patterns that arise from multiple frequencies associated with the eigenvalues of the chain Hamiltonian. Coupling of each spin to a harmonic bath leads to smoother dynamics, with damping effects that are stronger compared to those observed in the spin-boson model and more prominent in interior spins, a consequence of additional damping from the spin environment. Interior spins exhibit a transition from underdamped oscillatory to overdamped monotonic dynamics as the temperature, spin-bath, or spin-spin coupling is increased. In addition to these behaviors, a new dynamical pattern emerges in the evolution of edge spins with strong spin-spin coupling at low and intermediate temperatures, where the magnetization oscillates either above or below the equilibrium value.