Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

arXiv:1911.07607

Creation of long-lived states in interacting spins coupled to a thermal bath

Arnab Chakrabarti, Rangeet Bhattacharyya

Published Nov 18, 2019• 0 citations
arXivHTMLPDF

Abstract

We study the classic problem concerning the dissipative dynamics of a system of two interacting spin-$1/2$ particles, coupled to a thermal bath. In particular, we consider the case of a resonant excitation of the initial single-spin coherences and examine the consequences of the interplay between this excitation and the spin-spin dipolar coupling. Using a fluctuation-regulated Quantum Master Equation (frQME) [Phys. Rev. A 97, 063837 (2018)] we show that the relevant dissipator consists of cross-terms between the drive and the dipolar Hamiltonian, apart from regular self-terms responsible for ordinary relaxation effects. The drive-dipole cross-correlations provide for a novel second-order coupling of single and two-spin observables in the Zeeman basis, which cannot be classified as a dissipative effect. We show that the presence of these unique second-order non-dissipative terms lead to the well-known spin-locked steady-states in dipolar spin-ensembles. Importantly, the mathematical form of the steady-state magnetization in the spin-locked phase, obtained from our theory, matches with the prediction of the traditional spin-temperature based methods used to describe such phenomena.

Related papers

Emergence of prethermal states in a driven dissipative system through cross-correlated dissipation

Arnab Chakrabarti, Rangeet Bhattacharyya

Abstract Periodically driven closed quantum many-body systems are known to exhibit prethermal or quasi-steady-state dynamics. In this work, we theoretically show that such prethermal phases can appear in the dynamics of a dipolar two-spin-1/2 system coupled to a heat bath if the cross terms between the drive and dipolar interactions are taken into consideration. To this end, we use our recently reported fluctuation-regulated quantum master equation (Chakrabarti A. and Bhattacharyya R., Phys. Rev. A 97 (2018) 063837), to show that the predicted dynamics can successfully explain the experimentally observed features of the transient and prethermal regime.

Europhysics Letters (EPL)•May 12, 2023•4 citations

Dissipative cooling of spin chains by a bath of dipolar particles

M Robert-de-Saint-Vincent, P. Pedri, B. Laburthe-Tolra

We consider a spin chain of fermionic atoms in an optical lattice, interacting with each other by super-exchange interactions. We theoretically investigate the dissipative evolution of the spin chain when it is coupled by magnetic dipole–dipole interaction to a bath consisting of atoms with a strong magnetic moment. Dipolar interactions with the bath allow for a dynamical evolution of the collective spin of the spin chain. Starting from an uncorrelated thermal sample, we demonstrate that the dissipative cooling produces highly entangled low energy spin states of the chain in a timescale of a few seconds. In practice, the lowest energy singlet state driven by super-exchange interactions is efficiently produced. This dissipative approach is a promising alternative to cool spin-full atoms in spin-independent lattices. It provides direct thermalization of the spin degrees of freedom, while traditional approaches are plagued by the inherently long timescale associated to the necessary spatial redistribution of spins under the effect of super-exchange interactions.

arXiv:1803.10663•New Journal of Physics•Jul 5, 2018•3 citations

Bath-induced interactions and transient dynamics in open quantum systems at strong coupling: Effective Hamiltonian approach

Marlon Brenes, Brett Min, Nicholas Anto-Sztrikacs +2 more

Understanding the dynamics of dissipative quantum systems, particularly beyond the weak coupling approximation, is central to various quantum applications. While numerically exact methods provide accurate solutions, they often lack the analytical insight provided by theoretical approaches. In this study, we employ the recently developed method dubbed the effective Hamiltonian theory to understand the dynamics of system-bath configurations without resorting to a perturbative description of the system-bath coupling energy. Through a combination of mapping steps and truncation, the effective Hamiltonian theory offers both analytical insights into signatures of strong couplings in open quantum systems and a straightforward path for numerical simulations. To validate the accuracy of the method, we apply it to two canonical models: a single spin immersed in a bosonic bath and two noninteracting spins in a common bath. In both cases, we study the transient regime and the steady state limit at nonzero temperature and spanning system-bath interactions from the weak to the strong regime. By comparing the results of the effective Hamiltonian theory with numerically exact simulations, we show that although the former overlooks non-Markovian features in the transient equilibration dynamics, it correctly captures non-perturbative bath-generated couplings between otherwise non-interacting spins, as observed in their synchronization dynamics and correlations. Altogether, the effective Hamiltonian theory offers a powerful approach for understanding strong coupling dynamics and thermodynamics, capturing the signatures of such interactions in both relaxation dynamics and in the steady state limit.

arXiv:2403.03386•The Journal of Chemical Physics•Jun 25, 2024•12 citations

Non-equilibrium dynamics of dipole-coupled internal states in cold gases

Christopher D. Parmee

In this thesis, we consider the forms of non-equilibrium phenomena that can arise in atoms or polar molecules trapped in a deep optical lattice and coupled by dipolar internal degrees of freedom. We specifically focus on only two internal states, which results in the systems studied behaving as spin$-1/2$ models with long-range interactions. We first study a closed system with both static and resonant near-field dipole interactions under an external drive. By studying the uniform mean-field dynamics of the system, we find the dynamics are given by Rabi oscillations, with a bifurcation in the dynamics as a function of drive strength between small scale and large scale oscillations. Analysing the stability of these oscillations to small fluctuations reveals that interactions tend to cause the oscillations to decohere. However, we find parameter regimes where coherent oscillations can persist for high enough intensity drive. We then consider the effects of an environment on the non-equilibrium dynamics of the near-field dipole model. We find that within the mean-field approximation, an environment causes the system to relax to many novel steady state spin configurations, such as spin density waves, antiferromagnetism and long-time oscillations, as well as bistabilities between these phases. To assess the validity of the mean-field approximation, we compare our mean-field results to small quantum systems. We carry out a similar analysis on a system with far-field dipole interactions, where it is necessary to introduce nonlocal dissipation, which results in several decay modes into the environment. These decay modes lead to instabilities of many of the steady state phases that occurred in the near-field dipole system, leading to the emergence of more spin density wave and oscillatory phases. Finally, we examine the dynamics on the approach to steady state in a dissipative dipolar system by studying Rydberg atoms coupled to a photonic crystal waveguide, which mediates an effective dipole-dipole interaction between the atoms. We find that if two excitations exist in the system, then bound states can form, with nonlocal dissipation resulting in a momentum dependent decay rate of the bound states and also greater freedom in engineering the bound state energy dispersion.

•Apr 4, 2019•0 citations

Quantum master equation with dissipators regularized by thermal fluctuations

Arnab Chakrabarti, Rangeet Bhattacharyya

We report an alternate formulation of the quantum master equation (QME) to describe the dynamics of a quantum system weakly coupled to a heat bath, in the presence of weak external driving. A key feature of this approach is the introduction of an explicit Hamiltonian to model the thermal fluctuations in the heat bath. We show that the resulting time coarse-grained dynamical equation for the quantum system has dissipators with a natural regulator, which emerges from an ensemble average over the fluctuations. Importantly, such regularized dissipators arise from the second-order contributions of both the external drive as well as the system-environment coupling. We show that the second-order drive terms, regularized to time-scales set by the fluctuations, result in dynamic drive-induced frequency shifts as well as drive-dependent relaxation phenomena. Considering the specific case of an ensemble of two-level systems, subjected to a linearly polarized external drive, we derive the modified Bloch Equations with such drive-dependent shift and damping terms. The resulting drive-induced frequency shifts converge to the known forms of dynamic frequency shifts, such as the Bloch-Siegert shift or the dynamic Stark shift, in appropriate limits. The Kramers-Kronig pairs of these frequency shifts - manifest as drive-dependent damping terms in the modified Bloch Equations and help explain the Redfield limit of free-induction-decay (FID) rates as well as the non-Bloch decay of Rabi oscillations in isotropic medium. Our method predicts correct orders of magnitudes of non-Bloch decay rates in isotropic medium as well as their observed temperature dependence. The QME reported here, correctly describes all known aspects of the driven-dissipative dynamics up to second-order of an open quantum system with appropriate thermal signatures and as such is expected to provide deeper insights into the study of quantum information processing on real systems.

Physical Review A•Jun 18, 2018•15 citations

Dissipation Mechanisms and Dissipative Phase Transitions of two coupled Fully Connected Quantum Ising models

Bidyut Dey, Andrea Kazemi Nava, Domenico Giuliano

We study dissipative phase transitions in a system of two coupled fully-connected quantum Ising models interacting with an environment. The dynamics is governed by a Lindblad master equation combining coherent unitary evolution and incoherent dissipative processes, where the unitary part is described within a self-consistent mean-field framework effectively acting on the local Hilbert space of two coupled spins at each site. We analyze two fundamentally different classes of dissipators. In the first case, the jump operators are defined in the instantaneous eigenbasis of the mean-field Hamiltonian and satisfy a detailed-balance condition. In this setting, the relaxation dynamics depends strongly on the quench protocol: a parametric quench of the Hamiltonian leads to conventional relaxation, whereas a temperature quench gives rise to a dynamical phase transition characterized by nonanalytic behavior in time. Yet, in both cases, the system relaxes toward a steady state determined solely by the post-quench parameters and the bath temperature, which closely resembles a thermal Gibbs state of the mean-field Hamiltonian. As a result, the dissipative phase transition occurs at a critical point consistent with the corresponding equilibrium transition. In contrast, when the dissipators are realized via local spin raising and lowering operators, the steady state is genuinely nonequilibrium, leading to a significantly richer phase diagram. In particular, for sufficiently strong system-bath coupling, we observe a reentrant phase featuring a symmetry-broken region bounded by two continuous dissipative phase transitions. Our results evidence how the structure of dissipative processes controls the emergence of equilibrium-like versus genuinely nonequilibrium critical behavior in open quantum systems.

arXiv:2604.27072•Apr 29, 2026•0 citations
We study the classic problem concerning the dissipative dynamics of a system of two interacting spin-1/21/21/2 particles, coupled to a thermal bath. In particular, we consider the case of a resonant excitation of the initial single-spin coherences and examine the consequences of the interplay between this excitation and the spin-spin dipolar coupling. Using a fluctuation-regulated Quantum Master Equation (frQME) [Phys. Rev. A 97, 063837 (2018)] we show that the relevant dissipator consists of cross-terms between the drive and the dipolar Hamiltonian, apart from regular self-terms responsible for ordinary relaxation effects. The drive-dipole cross-correlations provide for a novel second-order coupling of single and two-spin observables in the Zeeman basis, which cannot be classified as a dissipative effect. We show that the presence of these unique second-order non-dissipative terms lead to the well-known spin-locked steady-states in dipolar spin-ensembles. Importantly, the mathematical form of the steady-state magnetization in the spin-locked phase, obtained from our theory, matches with the prediction of the traditional spin-temperature based methods used to describe such phenomena.
Abstract Periodically driven closed quantum many-body systems are known to exhibit prethermal or quasi-steady-state dynamics. In this work, we theoretically show that such prethermal phases can appear in the dynamics of a dipolar two-spin-1/2 system coupled to a heat bath if the cross terms between the drive and dipolar interactions are taken into consideration. To this end, we use our recently reported fluctuation-regulated quantum master equation (Chakrabarti A. and Bhattacharyya R., Phys. Rev. A 97 (2018) 063837), to show that the predicted dynamics can successfully explain the experimentally observed features of the transient and prethermal regime.
We consider a spin chain of fermionic atoms in an optical lattice, interacting with each other by super-exchange interactions. We theoretically investigate the dissipative evolution of the spin chain when it is coupled by magnetic dipole–dipole interaction to a bath consisting of atoms with a strong magnetic moment. Dipolar interactions with the bath allow for a dynamical evolution of the collective spin of the spin chain. Starting from an uncorrelated thermal sample, we demonstrate that the dissipative cooling produces highly entangled low energy spin states of the chain in a timescale of a few seconds. In practice, the lowest energy singlet state driven by super-exchange interactions is efficiently produced. This dissipative approach is a promising alternative to cool spin-full atoms in spin-independent lattices. It provides direct thermalization of the spin degrees of freedom, while traditional approaches are plagued by the inherently long timescale associated to the necessary spatial redistribution of spins under the effect of super-exchange interactions.
Understanding the dynamics of dissipative quantum systems, particularly beyond the weak coupling approximation, is central to various quantum applications. While numerically exact methods provide accurate solutions, they often lack the analytical insight provided by theoretical approaches. In this study, we employ the recently developed method dubbed the effective Hamiltonian theory to understand the dynamics of system-bath configurations without resorting to a perturbative description of the system-bath coupling energy. Through a combination of mapping steps and truncation, the effective Hamiltonian theory offers both analytical insights into signatures of strong couplings in open quantum systems and a straightforward path for numerical simulations. To validate the accuracy of the method, we apply it to two canonical models: a single spin immersed in a bosonic bath and two noninteracting spins in a common bath. In both cases, we study the transient regime and the steady state limit at nonzero temperature and spanning system-bath interactions from the weak to the strong regime. By comparing the results of the effective Hamiltonian theory with numerically exact simulations, we show that although the former overlooks non-Markovian features in the transient equilibration dynamics, it correctly captures non-perturbative bath-generated couplings between otherwise non-interacting spins, as observed in their synchronization dynamics and correlations. Altogether, the effective Hamiltonian theory offers a powerful approach for understanding strong coupling dynamics and thermodynamics, capturing the signatures of such interactions in both relaxation dynamics and in the steady state limit.
In this thesis, we consider the forms of non-equilibrium phenomena that can arise in atoms or polar molecules trapped in a deep optical lattice and coupled by dipolar internal degrees of freedom. We specifically focus on only two internal states, which results in the systems studied behaving as spin−1/2-1/2−1/2 models with long-range interactions. We first study a closed system with both static and resonant near-field dipole interactions under an external drive. By studying the uniform mean-field dynamics of the system, we find the dynamics are given by Rabi oscillations, with a bifurcation in the dynamics as a function of drive strength between small scale and large scale oscillations. Analysing the stability of these oscillations to small fluctuations reveals that interactions tend to cause the oscillations to decohere. However, we find parameter regimes where coherent oscillations can persist for high enough intensity drive. We then consider the effects of an environment on the non-equilibrium dynamics of the near-field dipole model. We find that within the mean-field approximation, an environment causes the system to relax to many novel steady state spin configurations, such as spin density waves, antiferromagnetism and long-time oscillations, as well as bistabilities between these phases. To assess the validity of the mean-field approximation, we compare our mean-field results to small quantum systems. We carry out a similar analysis on a system with far-field dipole interactions, where it is necessary to introduce nonlocal dissipation, which results in several decay modes into the environment. These decay modes lead to instabilities of many of the steady state phases that occurred in the near-field dipole system, leading to the emergence of more spin density wave and oscillatory phases. Finally, we examine the dynamics on the approach to steady state in a dissipative dipolar system by studying Rydberg atoms coupled to a photonic crystal waveguide, which mediates an effective dipole-dipole interaction between the atoms. We find that if two excitations exist in the system, then bound states can form, with nonlocal dissipation resulting in a momentum dependent decay rate of the bound states and also greater freedom in engineering the bound state energy dispersion.
We report an alternate formulation of the quantum master equation (QME) to describe the dynamics of a quantum system weakly coupled to a heat bath, in the presence of weak external driving. A key feature of this approach is the introduction of an explicit Hamiltonian to model the thermal fluctuations in the heat bath. We show that the resulting time coarse-grained dynamical equation for the quantum system has dissipators with a natural regulator, which emerges from an ensemble average over the fluctuations. Importantly, such regularized dissipators arise from the second-order contributions of both the external drive as well as the system-environment coupling. We show that the second-order drive terms, regularized to time-scales set by the fluctuations, result in dynamic drive-induced frequency shifts as well as drive-dependent relaxation phenomena. Considering the specific case of an ensemble of two-level systems, subjected to a linearly polarized external drive, we derive the modified Bloch Equations with such drive-dependent shift and damping terms. The resulting drive-induced frequency shifts converge to the known forms of dynamic frequency shifts, such as the Bloch-Siegert shift or the dynamic Stark shift, in appropriate limits. The Kramers-Kronig pairs of these frequency shifts - manifest as drive-dependent damping terms in the modified Bloch Equations and help explain the Redfield limit of free-induction-decay (FID) rates as well as the non-Bloch decay of Rabi oscillations in isotropic medium. Our method predicts correct orders of magnitudes of non-Bloch decay rates in isotropic medium as well as their observed temperature dependence. The QME reported here, correctly describes all known aspects of the driven-dissipative dynamics up to second-order of an open quantum system with appropriate thermal signatures and as such is expected to provide deeper insights into the study of quantum information processing on real systems.
We study dissipative phase transitions in a system of two coupled fully-connected quantum Ising models interacting with an environment. The dynamics is governed by a Lindblad master equation combining coherent unitary evolution and incoherent dissipative processes, where the unitary part is described within a self-consistent mean-field framework effectively acting on the local Hilbert space of two coupled spins at each site. We analyze two fundamentally different classes of dissipators. In the first case, the jump operators are defined in the instantaneous eigenbasis of the mean-field Hamiltonian and satisfy a detailed-balance condition. In this setting, the relaxation dynamics depends strongly on the quench protocol: a parametric quench of the Hamiltonian leads to conventional relaxation, whereas a temperature quench gives rise to a dynamical phase transition characterized by nonanalytic behavior in time. Yet, in both cases, the system relaxes toward a steady state determined solely by the post-quench parameters and the bath temperature, which closely resembles a thermal Gibbs state of the mean-field Hamiltonian. As a result, the dissipative phase transition occurs at a critical point consistent with the corresponding equilibrium transition. In contrast, when the dissipators are realized via local spin raising and lowering operators, the steady state is genuinely nonequilibrium, leading to a significantly richer phase diagram. In particular, for sufficiently strong system-bath coupling, we observe a reentrant phase featuring a symmetry-broken region bounded by two continuous dissipative phase transitions. Our results evidence how the structure of dissipative processes controls the emergence of equilibrium-like versus genuinely nonequilibrium critical behavior in open quantum systems.